Imaging an aligned polyatomic molecule with laser-induced electron diffraction

Pullen, Michael G.; Wolter, Benjamin; Le, Anh-Thu; Baudisch, Matthias; Hemmer, Michaël; Senftleben, Arne; Schröter, Claus Dieter; Ullrich, Joachim; Moshammer, Robert; Lin, C. D.; Biegert, Jens

doi:10.1038/ncomms8262

Imaging an aligned polyatomic molecule with laser-induced electron diffraction

Journal Article · Wed Jun 24 00:00:00 EDT 2015 · Nature Communications

DOI:https://doi.org/10.1038/ncomms8262· OSTI ID:1623980

^[1]; Wolter, Benjamin ^[2]; Le, Anh-Thu ^[3]; Baudisch, Matthias ^[2]; Hemmer, Michaël ^[2]; Senftleben, Arne ^[4]; Schröter, Claus Dieter ^[5]; Ullrich, Joachim ^[6]; Moshammer, Robert ^[5]; Lin, C. D. ^[3]; Biegert, Jens ^[7]

Inst. de Ciencies Fotoniques (ICFO), Barcelona (Spain); DOE/OSTI
Inst. de Ciencies Fotoniques (ICFO), Barcelona (Spain)
Kansas State Univ., Manhattan, KS (United States)
Univ. Kassel (Germany)
Max-Planck-Inst. für Kernphysik, Heidelberg (Germany)
Max-Planck-Inst. für Kernphysik, Heidelberg (Germany); Physikalisch-Technische Bundesanstalt (PTB), Braunschweig (Germany)
Inst. de Ciencies Fotoniques (ICFO), Barcelona (Spain); Univ. of New Mexico, Albuquerque, NM (United States); Inst. Catalana de Recerca i Estudis Avançats (ICREA), Barcelona (Spain)

Laser-induced electron diffraction is an evolving tabletop method that aims to image ultrafast structural changes in gas-phase polyatomic molecules with sub-Ångstro¨m spatial and femtosecond temporal resolutions. Here we demonstrate the retrieval of multiple bond lengths from a polyatomic molecule by simultaneously measuring the C–C and C–H bond lengths in aligned acetylene. Our approach takes the method beyond the hitherto achieved imaging of simple diatomic molecules and is based on the combination of a 160 kHz mid-infrared few-cycle laser source with full three-dimensional electron–ion coincidence detection. Our technique provides an accessible and robust route towards imaging ultrafast processes in complex gas-phase molecules with atto- to femto-second temporal resolution.

View Accepted Manuscript (DOE)

Research Organization:: Kansas State Univ., Manhattan, KS (United States)

Sponsoring Organization:: Catalan Agencia de Gestio´ d’Ajuts Universitaris i de Recerca (AGAUR); European Commission; Fundació Cellex Barcelona; Laserlab-Europe; Ministerio de Economía y Competitividad (MINECO); USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division

Grant/Contract Number:: FG02-86ER13491

OSTI ID:: 1623980

Journal Information:: Nature Communications, Journal Name: Nature Communications Journal Issue: 1 Vol. 6; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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The Potential of EuPRAXIA@SPARC_LAB for Radiation Based Techniques Balerna, Antonella; Bartocci, Samanta; Batignani, Giovanni Condensed Matter, Vol. 4, Issue 1 https://doi.org/10.3390/condmat4010030	journal	March 2019
Dynamics of valence-shell electrons and nuclei probed by strong-field holography and rescattering Walt, Samuel G.; Ram, Niraghatam Bhargava; Atala, Marcos ETH Zurich https://doi.org/10.3929/ethz-b-000191079	text	January 2017
Interplay between Coulomb-focusing and non-dipole effects in strong-field ionization with elliptical polarization Daněk, Jiří; Klaiber, Michael; Hatsagortsyan, Karen Z. ETH Zurich https://doi.org/10.3929/ethz-b-000268933	text	January 2018
Attosecond physics at the nanoscale Ciappina, M. F.; Pérez-Hernández, J. A.; Landsman, A. S. arXiv https://doi.org/10.48550/arxiv.1607.01480	text	January 2016
Emergence of a higher energy structure in strong field ionization with inhomogeneous electric fields Ortmann, L.; Pérez-Hernández, J. A.; Ciappina, M. F. arXiv https://doi.org/10.48550/arxiv.1608.07394	text	January 2016
Interplay between Coulomb-focusing and non-dipole effects in strong-field ionization with elliptical polarization Maurer, J.; Willenberg, B.; Mayer, B. W. arXiv https://doi.org/10.48550/arxiv.1703.03283	preprint	January 2017
Robust transverse structures in rescattered photoelectron wavepackets and their observable consequences Bredtmann, Timm; Patchkovskii, Serguei arXiv https://doi.org/10.48550/arxiv.1810.12672	text	January 2018

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