Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

Observation of possible topological in-gap surface states in the Kondo insulator SmB6 by photoemission

Journal Article · · Nature Communications
DOI:https://doi.org/10.1038/ncomms4010· OSTI ID:1623931
 [1];  [2];  [3];  [4];  [4];  [3];  [3];  [3];  [3];  [3];  [3];  [3];  [2];  [4];  [2];  [3]
  1. Fudan Univ., Shanghai (China); DOE/OSTI
  2. Nanjing Univ. (China)
  3. Fudan Univ., Shanghai (China)
  4. University of Science and Technology of China, Hefei (China)

SmB6, a well-known Kondo insulator, exhibits a transport anomaly at low temperature. This anomaly is usually attributed to states within the hybridization gap. Recent theoretical work and transport measurements suggest that these in-gap states could be ascribed to topological surface states, which would make SmB6 the first realization of topological Kondo insulator. Here by performing angle-resolved photoemission spectroscopy experiments, we directly observe several dispersive states within the hybridization gap of SmB6. These states show negligible kz dependence, which indicates their surface origin. Furthermore, we perform photoemission circular dichroism experiments, which suggest that the in-gap states possess chirality of the orbital angular momentum. These states vanish simultaneously with the hybridization gap at around 150 K. Together, these observations suggest the possible topological origin of the in-gap states.

Research Organization:
Fudan Univ., Shanghai (China)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division
OSTI ID:
1623931
Journal Information:
Nature Communications, Journal Name: Nature Communications Journal Issue: 1 Vol. 4; ISSN 2041-1723
Publisher:
Nature Publishing GroupCopyright Statement
Country of Publication:
United States
Language:
English

References (31)

Heavy fermion semiconductors journal May 2000
Large low-temperature Hall effect and resistivity in mixed-valent Sm B 6 journal December 1979
Robust Surface Hall Effect and Nonlocal Transport in SmB6: Indication for an Ideal Topological Insulator text January 2012
Electronic structure of divalent hexaborides journal March 1996
Magnetic excitations in SmB6 single crystals journal May 1993
Gap state of SmB6 journal May 1993
Ultrahigh-resolution and angle-resolved photoemission study of SmB6 journal June 2002
Direct observation of pseudogap of SmB6 using ultrahigh-resolution photoemission spectroscopy journal March 2002
Advances in photoemission spectroscopy of f-electron materials journal June 2000
Surface electronic structure of the topological Kondo-insulator candidate correlated electron system SmB6 journal December 2013
Large low-temperature Hall effect and resistivity in mixed-valent Sm B 6 journal December 1979
Low-energy excitations of the correlation-gap insulator SmB 6 :ffA light-scattering study journal May 1997
4Electron self-trapping in intermediate-valent SmB 6 journal June 2000
Theory of topological Kondo insulators journal January 2012
Momentum-dependent hybridization gap and dispersive in-gap state of the Kondo semiconductor SmB 6 journal August 2012
Surface and bulk electronic structure of the strongly correlated system SmB 6 and implications for a topological Kondo insulator journal September 2013
Low-temperature surface conduction in the Kondo insulator SmB 6 journal November 2013
Topological Kondo Insulators journal March 2010
Observation of a Warped Helical Spin Texture in Bi 2 Se 3 from Circular Dichroism Angle-Resolved Photoemission Spectroscopy journal November 2011
Chiral Orbital-Angular Momentum in the Surface States of Bi 2 Se 3 journal January 2012
Limit Cycle and Anomalous Capacitance in the Kondo Insulator SmB 6 journal August 2012
Correlated Topological Insulators with Mixed Valence journal February 2013
Reversal of the Circular Dichroism in Angle-Resolved Photoemission from Bi 2 Te 3 journal May 2013
Magnetic and Semiconducting Properties of Sm B 6 journal February 1969
Sm B 6 : Kondo Insulator or Exotic Metal? journal February 1995
Kondo Hybridization and the Origin of Metallic States at the (001) Surface of SmB 6 journal December 2013
Colloquium: Topological insulators journal November 2010
Topological insulators and superconductors journal October 2011
SmB 6 : A Promising Candidate for a Topological Insulator journal December 2011
Topological Kondo Insulators journal March 2016
Surface electronic structure of the topological Kondo insulator candidate correlated electron system SmB6 text January 2013

Cited By (93)

Unconventional transformation of spin Dirac phase across a topological quantum phase transition journal April 2015
Author Correction: How to probe the spin contribution to momentum relaxation in topological insulators journal February 2018
Evidence for in-gap surface states on the single phase SmB6(001) surface journal October 2017
Racah materials: role of atomic multiplets in intermediate valence systems journal October 2015
On the Chemistry and Physical Properties of Flux and Floating Zone Grown SmB6 Single Crystals journal February 2016
Thin films of topological Kondo insulator candidate SmB 6 : Strong spin-orbit torque without exclusive surface conduction journal January 2018
Samarium hexaboride is a trivial surface conductor text January 2019
Emergent photovoltage on SmB6 surface upon bulk-gap evolution revealed by pump-and-probe photoemission spectroscopy text January 2015
Surface Kondo Effect and Non-Trivial Metallic State of the Kondo Insulator YbB12 text January 2016
Contrast Reversal in Scanning Tunneling Microscopy and Its Implications for the Topological Classification of SmB 6 journal January 2020
Magnetoresistance Anomaly in Topological Kondo Insulator SmB 6 Nanowires with Strong Surface Magnetism journal May 2018
Raman spectroscopic evidence of impurity‐induced structural distortion in SmB 6 journal July 2019
Investigation of High-Temperature Bulk Transport Characteristics and Skew Scattering in Samarium Hexaboride journal September 2019
Finite temperature physics of 1D topological Kondo insulator: Stable Haldane phase, emergent energy scale and beyond journal October 2018
Spin injection and inverse Edelstein effect in the surface states of topological Kondo insulator SmB6 journal November 2016
Additional energy scale in SmB6 at low-temperature journal December 2016
Direct observation of the spin texture in SmB6 as evidence of the topological Kondo insulator journal July 2014
One-dimensional edge state transport in a topological Kondo insulator journal November 2015
Möbius Kondo insulators journal April 2017
Non-trivial surface states of samarium hexaboride at the (111) surface journal May 2019
Magnetic field-tuned Fermi liquid in a Kondo insulator journal December 2019
Quantum materials for spin and charge conversion journal May 2018
Imaging emergent heavy Dirac fermions of a topological Kondo insulator journal November 2019
Perfect Andreev reflection due to the Klein paradox in a topological superconducting state journal June 2019
Breakdown of the strong multiplet description of the Sm2+ ion in the topological Kondo insulator SmB6: specific heat studies journal August 2019
Surface Hall Effect and Nonlocal Transport in SmB6: Evidence for Surface Conduction journal November 2013
CeRu4Sn6: a strongly correlated material with nontrivial topology journal December 2015
Robust topological surface state in Kondo insulator SmB 6 thin films journal December 2014
Single crystalline SmB 6 nanowires for self-powered, broadband photodetectors covering mid-infrared journal April 2018
Hybridization gap and Fano resonance in SmB 6 journal March 2014
Topological surface states interacting with bulk excitations in the Kondo insulator SmB 6 revealed via planar tunneling spectroscopy journal May 2016
Pressure-induced exotic states in rare earth hexaborides journal July 2016
Unusual diffusive effects on the ESR of Nd 3+ ions in the tunable topologically nontrivial semimetal YBiPt journal February 2016
Spin- and angle-resolved photoemission on the topological Kondo insulator candidate: SmB 6 journal July 2016
Single crystal growth and anisotropic physical properties of Sm 4 Co 3 Ga 16 journal July 2018
Interacting topological insulators: a review journal October 2018
Angle-resolved photoemission spectroscopy study of the Möbius Kondo insulator candidate CeRhSb journal July 2019
Resonant inelastic x-ray scattering investigation of the crystal-field splitting of Sm 3 + in SmB 6 journal December 2019
Consistency between ARPES and STM measurements on SmB 6 journal February 2020
Topological invariants, surface states, and interaction-driven phase transitions in correlated Kondo insulators with cubic symmetry journal February 2014
Strongly interacting Dirac liquid on the surface of a topological Kondo insulator journal August 2014
Exotic Kondo crossover in a wide temperature region in the topological Kondo insulator SmB 6 revealed by high-resolution ARPES journal August 2014
Surface theory of a family of topological Kondo insulators journal October 2014
In-gap collective mode spectrum of the topological Kondo insulator SmB 6 journal November 2014
Two-dimensional heavy fermions on the strongly correlated boundaries of Kondo topological insulators journal December 2014
New classes of three-dimensional topological crystalline insulators: Nonsymmorphic and magnetic journal April 2015
Magnetoresistance evidence of a surface state and a field-dependent insulating state in the Kondo insulator SmB 6 journal May 2015
Robust local and nonlocal transport in the topological Kondo insulator SmB 6 in the presence of a high magnetic field journal August 2015
Incomplete protection of the surface Weyl cones of the Kondo insulator SmB 6 : Spin exciton scattering journal August 2015
Magnetotransport measurements of the surface states of samarium hexaboride using Corbino structures journal September 2015
Fractionalized Fermi liquid on the surface of a topological Kondo insulator journal March 2016
Low-temperature conducting state in two candidate topological Kondo insulators: SmB 6 and Ce 3 Bi 4 Pt 3 journal July 2016
Breakdown of the Kondo insulating state in SmB 6 by introducing Sm vacancies journal August 2016
Anomalous three-dimensional bulk ac conduction within the Kondo gap of SmB 6 single crystals journal October 2016
Weak antilocalization and linear magnetoresistance in the surface state of SmB 6 journal November 2016
Effects of spin excitons on the surface states of SmB 6 : A photoemission study journal December 2016
Planar tunneling spectroscopy of the topological Kondo insulator SmB 6 journal May 2017
Understanding low-temperature bulk transport in samarium hexaboride without relying on in-gap bulk states journal May 2017
Reduction of the low-temperature bulk gap in samarium hexaboride under high magnetic fields journal June 2017
Tunable electronic structure and surface states in rare-earth monobismuthides with partially filled f shell journal August 2018
Physical properties of Sm x B 6 single crystals journal January 2019
Electrical detection of the surface spin polarization of the candidate topological Kondo insulator Sm B 6 journal June 2019
Emergence of a Coherent In-Gap State in the SmB 6 Kondo Insulator Revealed by Scanning Tunneling Spectroscopy journal March 2014
Interaction Driven Subgap Spin Exciton in the Kondo Insulator SmB 6 journal January 2015
Tuning Bulk and Surface Conduction in the Proposed Topological Kondo Insulator SmB 6 journal March 2015
Kondo Breakdown in Topological Kondo Insulators journal April 2015
Signature of Strong Spin-Orbital Coupling in the Large Nonsaturating Magnetoresistance Material WTe 2 journal October 2015
Kondo Breakdown and Quantum Oscillations in SmB 6 journal January 2016
Pressure-Resistant Intermediate Valence in the Kondo Insulator SmB 6 journal April 2016
Bulk Fermi Surface of Charge-Neutral Excitations in SmB 6 or Not: A Heat-Transport Study journal June 2016
Skyrme Insulators: Insulators at the Brink of Superconductivity journal August 2017
4 f Crystal Field Ground State of the Strongly Correlated Topological Insulator SmB 6 journal January 2018
Quantum Oscillations in Flux-Grown SmB 6 with Embedded Aluminum journal April 2019
Multiple topological Dirac cones in a mixed-valent Kondo semimetal: g -SmS journal August 2019
Microwave Meissner screening properties of proximity-coupled topological-insulator / superconductor bilayers journal December 2019
Correlation between Bulk Thermodynamic Measurements and the Low-Temperature-Resistance Plateau in SmB 6 journal July 2014
Observation of the Superconducting Proximity Effect in the Surface State of SmB 6 Thin Films journal August 2016
Heavy Weyl Fermion State in CeRu 4 Sn 6 journal March 2017
Colloquium : Topological band theory journal June 2016
Two-dimensional Fermi surfaces in Kondo insulator SmB 6 journal December 2014
$4f$ Crystal Field Ground State of the Strongly Correlated Topological Insulator $SmB_{6}$ text January 2018
Inorganic Boron-Based Nanostructures: Synthesis, Optoelectronic Properties, and Prospective Applications journal April 2019
Topological invariants, surface states, and interaction-driven phase transitions in correlated Kondo insulators with cubic symmetry text January 2013
Surface Theory of a Family of Topological Kondo Insulators text January 2014
Two-dimensional heavy fermions on the strongly correlated boundaries of Kondo topological insulators text January 2014
Spin Injection and Inverse Edelstein Effect in the Surface States of Topological Kondo Insulator SmB6 text January 2016
Reduction of the low-temperature bulk gap in samarium hexaboride under high magnetic fields text January 2016
Additional energy scale in SmB$_6$ at low temperature text January 2017
Skyrme insulators: insulators at the brink of superconductivity text January 2017
Tunable Electronic Structure and Surface States in Rare Earth Mono-Bismuthides with Partially Filled f Shell text January 2018
Interacting topological insulators: a review text January 2018
Investigation of high-temperature bulk transport characteristics and skew scattering in samarium hexaboride preprint January 2019
Multiple topological Dirac cones in a mixed-valent Kondo semimetal: g-SmS text January 2019

Similar Records

Anomalous three-dimensional bulk ac conduction within the Kondo gap of SmB6 single crystals
Journal Article · Fri Oct 21 00:00:00 EDT 2016 · Physical Review B · OSTI ID:1392878

Quantum phase transition and destruction of Kondo effect in pressurized SmB6
Journal Article · Tue Oct 24 00:00:00 EDT 2017 · Science Bulletin · OSTI ID:1431072

Robust topological surface state in Kondo insulator SmB{sub 6} thin films
Journal Article · Sun Nov 30 23:00:00 EST 2014 · Applied Physics Letters · OSTI ID:22402410