Time-resolved XUV ARPES with tunable 24–33 eV laser pulses at 30 meV resolution

Sie, Edbert J.; Rohwer, Timm; Lee, Changmin; Gedik, Nuh

doi:10.1038/s41467-019-11492-3

Title: Time-resolved XUV ARPES with tunable 24–33 eV laser pulses at 30 meV resolution

Journal Article · Tue Aug 06 00:00:00 EDT 2019 · Nature Communications

DOI:https://doi.org/10.1038/s41467-019-11492-3· OSTI ID:1619647

; Rohwer, Timm; Lee, Changmin;

Abstract High harmonic generation of ultrafast laser pulses can be used to perform angle-resolved photoemission spectroscopy (ARPES) to map the electronic band structure of materials with femtosecond time resolution. However, currently it is difficult to reach high momenta with narrow energy resolution. Here, we combine a gas phase extreme ultraviolet (XUV) femtosecond light source, an XUV monochromator, and a time-of-flight electron analyzer to develop XUV-based time-resolved ARPES. Our technique can produce tunable photon energy between 24–33 eV with an unprecedented energy resolution of 30 meV and time resolution of 200 fs. This technique enables time-, energy- and momentum-resolved investigation of the nonequilibrium dynamics of electrons in materials with a full access to their first Brillouin zone. We evaluate the performance of this setup through exemplary measurements on various quantum materials, including WTe ₂ , WSe ₂ , TiSe ₂ , and Bi ₂ Sr ₂ CaCu ₂ O _8+δ .

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Research Organization:: Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)

Sponsoring Organization:: USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division; US Army Research Office (ARO); Gordon and Betty Moore Foundation (GBMF)

Grant/Contract Number:: GBMF4540

OSTI ID:: 1619647

Alternate ID(s):: OSTI ID: 1624182

Journal Information:: Nature Communications, Journal Name: Nature Communications Vol. 10 Journal Issue: 1; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United Kingdom

Language:: English

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Cited by: 46 works

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