Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

Effect of Electron Capture on Spectral Line Broadening in Hot Dense Plasmas

Journal Article · · Physical Review Letters
Accurate calculation of spectral line broadening is important for many hot, dense plasma applications. However, calculated line widths have significantly underestimated measured widths for Δn = 0 lines of Li-like ions, which is known as the isolated-line problem. In this Letter, scrutinization of the line-width derivation reveals that the commonly used expression neglects a potentially important contribution from electron-capture. Line-width calculations including this process are performed with two independent codes, both of which removed the discrepancies at temperatures below 10 eV. In conclusion, the revised calculations also suggest the remaining discrepancy scales more strongly with electron temperature than the atomic number as was previously suggested.
Research Organization:
Los Alamos National Laboratory (LANL), Los Alamos, NM (United States); Sandia National Laboratories (SNL-NM), Albuquerque, NM (United States)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA); USDOE Office of Science (SC), Fusion Energy Sciences (FES)
Grant/Contract Number:
89233218CNA000001; AC04-94AL85000; NA0003525
OSTI ID:
1618076
Alternate ID(s):
OSTI ID: 2346078
Report Number(s):
LA-UR--19-30252; SAND--2020-0489J; 682812
Journal Information:
Physical Review Letters, Journal Name: Physical Review Letters Journal Issue: 5 Vol. 124; ISSN 0031-9007; ISSN PRLTAO
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

References (36)

Broadening of the 3s–3p transition in NeVIII journal September 2003
Electron-impact broadening of the 3s–3p lines in low-Z Li-like ions journal September 2003
Stark Broadening Parameters of Analogous Spectral Lines Along the Lithium and Beryllium Isoelectronic Sequences journal February 1999
Electron broadening of isolated lines with stationary non-equilibrium level populations journal December 2005
Review of the 1st Spectral Line Shapes in Plasmas code comparison workshop journal September 2013
Relativistic opacities for astrophysical applications journal September 2015
Model uncertainties of local-thermodynamic-equilibrium K-shell spectroscopy journal September 2016
Experimental Stark Widths and Shifts for Spectral Lines of Neutral and Ionized Atoms (A Critical Review of Selected Data for the Period 1989 Through 2000) journal September 2002
Demonstration of thermonuclear conditions in magnetized liner inertial fusion experimentsa) journal May 2015
Diagnosing magnetized liner inertial fusion experiments on Za) journal May 2015
LABORATORY MEASUREMENTS OF WHITE DWARF PHOTOSPHERIC SPECTRAL LINES: H β journal June 2015
Atomic data for opacity calculations. VIII. Line-profile parameters for 42 transitions in Li-like and Be-like ions journal September 1988
Atomic data for opacity calculations: XII. Line-profile parameters for neutral atoms of He, C, N and O journal November 1989
Atomic data for opacity calculations. XIII. Line profiles for transitions in hydrogenic ions journal October 1990
Calculation of electron-impact ionization of lithium-like targets journal April 1995
Electron - atom scattering at low and intermediate energies using a pseudo-state/ R -matrix basis journal January 1996
Electron-impact excitation and ionization of journal June 1997
Opacities for stellar envelopes journal February 1994
General Impact Theory of Pressure Broadening journal November 1958
Variational Principles for Scattering Processes. I journal August 1950
The Formal Theory of Scattering journal July 1953
Full Coulomb calculation of Stark broadening in laser-produced plasmas journal July 1984
Stark broadening of spectral lines along the isoelectronic sequence of Li journal June 1992
Convergent close-coupling method for the calculation of electron scattering on hydrogenlike targets journal February 1994
Stark broadening of resonance transitions in B III journal April 1996
Absolute cross sections for excitation of the 2 s 2 S → 2 p 2 P transition in B 2 + and for electron-impact single ionization of B 2 + journal December 1998
Widths and shifts of spectral lines in He II ions produced by electron impact journal November 2012
Density-matrix correlations in the relaxation theory of electron broadening journal July 2018
Stark broadening of the B III 2 s − 2 p lines journal December 1997
Line shape measurement and isolated line width calculations: Quantal versus semiclassical methods journal November 1999
Standard line broadening impact theory for hydrogen including penetrating collisions journal October 2005
Systematic Study of L -Shell Opacity at Stellar Interior Temperatures journal June 2019
The Theory of Atomic Structure and Spectra book December 1981
The Second Workshop on Lineshape Code Comparison: Isolated Lines journal May 2014
Electron-Impact Widths and Shifts of B III 2p-2s Lines journal May 2014
The Third and Fourth Workshops on Spectral Line Shapes in Plasma Code Comparison: Isolated Lines journal May 2018