Impact of nematicity on the relationship between antiferromagnetic fluctuations and superconductivity in FeSe0.91S0.09 under pressure

Rana, K.; Xiang, L.; Wiecki, P.; Ribeiro, R. A.; Lesseux, G. G.; Böhmer, A. E.; Bud'ko, S. L.; Canfield, P. C.; Furukawa, Y.

doi:10.1103/PhysRevB.101.180503

Title: Impact of nematicity on the relationship between antiferromagnetic fluctuations and superconductivity in ${{FeSe}_{0.91} S}_{0.09}$ under pressure

Journal Article · Wed May 06 00:00:00 EDT 2020 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.101.180503· OSTI ID:1617468

^[1];

^[1]; Wiecki, P. ^[2];

^[1];

^[1]; Böhmer, A. E. ^[2]; Bud'ko, S. L. ^[1]; Canfield, P. C. ^[1];

^[1]

Ames Lab., and Iowa State Univ., Ames, IA (United States)
Ames Lab., and Iowa State Univ., Ames, IA (United States); Karlsruhe Inst. of Technology (KIT) (Germany)

The sulfur-substituted FeSe system, ${FeSe}_{1 - x} S_{x}$ , provides a versatile platform for studying the relationship among nematicity, antiferromagnetism, and superconductivity. Herein, by nuclear magnetic resonance (NMR) and resistivity measurements up to 4.73 GPa on ${FeSe}_{0.91} S_{0.09}$ , we established the pressure- ( $p$ -) temperature ( $T$ ) phase diagram in which the nematic state is suppressed with pressure showing a nematic quantum phase transition (QPT) around $p = 0.5 GPa$ , two superconductivity (SC) regions separated by the QPT appear, and antiferromagnetic (AFM) phase emerges above $~ 3.3 GPa$ . From the NMR results up to 2.1 GPa, AFM fluctuations are revealed to be characterized by the stripe-type wave vector which remains the same for the two SC regions. Furthermore, the electronic state is discovered to change in character from non-Fermi liquid to Fermi liquid around the nematic QPT and persists up to $~ 2.1 GPa$ . In addition, although the AFM fluctuations correlate with $T_{c}$ in both SC states, demonstrating the importance of the AFM fluctuations for the appearance of SC in the system, we found that, when nematic order is absent, $T_{c}$ is strongly correlated with the AFM fluctuations whereas $T_{c}$ weakly depends on the AFM fluctuations when nematic order is present. Our findings on ${FeSe}_{0.91} S_{0.09}$ were shown to be applied to the whole ${FeSe}_{1 - x} S_{x}$ system and offer an insight into the relationship between AFM fluctuations and SC in Fe-based superconductors.

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Research Organization:: Ames Lab., Ames, IA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division

Grant/Contract Number:: AC02-07CH11358

OSTI ID:: 1617468

Report Number(s):: IS-J 10,212; PRBMDO; TRN: US2106746

Journal Information:: Physical Review B, Vol. 101, Issue 18; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 5 works

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Title: Impact of nematicity on the relationship between antiferromagnetic fluctuations and superconductivity in FeSe 0.91 S 0.09 under pressure

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Title: Impact of nematicity on the relationship between antiferromagnetic fluctuations and superconductivity in ${{FeSe}_{0.91} S}_{0.09}$ under pressure