Progress on ternary oxide-based photoanodes for use in photoelectrochemical cells for solar water splitting

Lee, Dong Ki; Lee, Dongho; Lumley, Margaret A.; Choi, Kyoung-Shin

doi:10.1039/c8cs00761f

Progress on ternary oxide-based photoanodes for use in photoelectrochemical cells for solar water splitting

Journal Article · Fri Nov 30 04:00:00 EST 2018 · Chemical Society Reviews

DOI:https://doi.org/10.1039/c8cs00761f· OSTI ID:1611142

^[1]; ^[2]; Lumley, Margaret A. ^[2]; ^[2]

Univ. of Wisconsin, Madison, WI (United States); DOE/OSTI
Univ. of Wisconsin, Madison, WI (United States)

Solar water splitting using photoelectrochemical cells (PECs) has emerged as one of the most promising routes to produce hydrogen as a clean and renewable fuel source. Among various semiconductors that have been considered as photoelectrodes for use in PECs, oxide-based photoanodes are particularly attractive because of their stability in aqueous media in addition to inexpensive and facile processing compared to other types of semiconductors. However, they typically suffer from poor charge carrier separation and transport. In the past few years, there has been tremendous progress in developing ternary oxide-based photoelectrodes, specifically, photoanodes. The use of ternary oxides provides more opportunities to tune the composition and electronic structure of the photoelectrode compared to binary oxides, thus providing more freedom to tune the photoelectrochemical properties. In this article, we outline the important characteristics to analyze when evaluating photoanodes and review the major recent progress made on the development of ternary oxide-based photoanodes. For each system, we highlight the favorable and unfavorable features and summarize the strategies utilized to address the challenges associated with each material. Finally, by combining our analyses of all the photoanodes surveyed in this review, we provide possible future research directions for each compound and an outlook for constructing more efficient oxide-based PECs. Overall, this review will provide a critical overview of current ternary oxide-based photoanodes and will serve as a platform for the design of future oxide-based PECs.

View Accepted Manuscript (DOE)

Research Organization:: University of Wisconsin, Madison, WI (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0008707

OSTI ID:: 1611142

Alternate ID(s):: OSTI ID: 1484049

Journal Information:: Chemical Society Reviews, Journal Name: Chemical Society Reviews Journal Issue: 7 Vol. 48; ISSN 0306-0012

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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Unveiling new stable manganese based photoanode materials via theoretical high-throughput screening and experiments Noh, Juhwan; Kim, Sungwon; Gu, Geun ho Chemical Communications, Vol. 55, Issue 89 https://doi.org/10.1039/c9cc06736a	journal	January 2019
3D highly efficient photonic micro concave-pit arrays for enhanced solar water splitting Li, Ming; Chen, Le; Zhou, Chao Nanoscale, Vol. 11, Issue 39 https://doi.org/10.1039/c9nr05778a	journal	January 2019
Modulation of oxygen vacancy in tungsten oxide nanosheets for Vis-NIR light-enhanced electrocatalytic hydrogen production and anticancer photothermal therapy Liang, Haiyan; Xi, Hongjuan; Liu, Shaoqiong Nanoscale, Vol. 11, Issue 39 https://doi.org/10.1039/c9nr06222j	journal	January 2019
Nanostructured core–shell metal borides–oxides as highly efficient electrocatalysts for photoelectrochemical water oxidation Lu, Can; Jothi, Palani R.; Thersleff, Thomas Nanoscale, Vol. 12, Issue 5 https://doi.org/10.1039/c9nr09818f	journal	January 2020
Heterostructured Sn/SnO _2−x nanotube peapods with a strong plasmonic effect for photoelectrochemical water oxidation Li, Yueying; Wang, Jian-Gan; Hua, Wei Journal of Materials Chemistry A, Vol. 7, Issue 28 https://doi.org/10.1039/c9ta03848e	journal	January 2019
Optical absorption induced by small polaron formation in transition metal oxides: The case of Co 3 O 4 Smart, Tyler J.; Pham, Tuan Anh; Ping, Yuan Physical Review Materials, Vol. 3, Issue 10 https://doi.org/10.1103/physrevmaterials.3.102401	journal	October 2019

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