Strong-field-induced bond rearrangement in triatomic molecules

Zhao, S.; Jochim, Bethany; Feizollah, Peyman; Rajput, Jyoti; Ziaee, F.; P., Kanaka Raju; Kaderiya, B.; Borne, K.; Malakar, Y.; Berry, Ben; Harrington, J.; Rolles, D.; Rudenko, A.; Carnes, K. D.; Wells, Eric; Ben-Itzhak, I.; Severt, T.

doi:10.1103/physreva.99.053412

Title: Strong-field-induced bond rearrangement in triatomic molecules

Journal Article · Wed May 15 00:00:00 EDT 2019 · Physical Review A

DOI:https://doi.org/10.1103/physreva.99.053412· OSTI ID:1610700

Zhao, S. ^[1]; Jochim, Bethany ^[2]; Feizollah, Peyman ^[2]; Rajput, Jyoti ^[3]; Ziaee, F. ^[2]; P., Kanaka Raju ^[2]; Kaderiya, B. ^[2]; Borne, K. ^[2]; Malakar, Y. ^[2]; Berry, Ben ^[2]; Harrington, J. ^[2]; Rolles, D. ^[2]; Rudenko, A. ^[2]; Carnes, K. D. ^[2]; Wells, Eric ^[1]; Ben-Itzhak, I. ^[2]; Severt, T. ^[2]

Augustana Univ., Sioux Falls, SD (United States)
Kansas State Univ., Manhattan, KS (United States)
Kansas State Univ., Manhattan, KS (United States); Univ. of Delhi (India)

A comparative study of bond rearrangement is reported for the double ionization of three triatomic molecules: carbon dioxide, carbonyl sulfide, and water (D₂O). Specifically, we study the formation of the molecular cation AC⁺ from the edge atoms of a triatomic molecular dication ABC²⁺ following double ionization by intense, short (23 fs, 790 nm) laser pulses. The comparison is made using the double ionization branching ratio of each molecule, thereby minimizing differences due to differing ionization rates. The rearrangement branching ratio is highest for water, which has a bent initial geometry, while CO₂ and OCS are linear molecules. The angular distribution of O₂⁺ fragments arising from CO₂ is essentially isotropic, while SO⁺ from OCS and $$D$$ $$^{+}_{2}$$ from D₂O are aligned with the laser polarization. In the CO₂ and D₂O cases, the angular distributions of the bond rearrangement channels are different from the angular distributions of the dominant dissociative double ionization channels CO⁺ + O⁺ and OD⁺ + D⁺. Only the angular distribution of SO+ from OCS is both aligned with the laser polarization and similar to the angular distribution of the largest dissociative channel, CO⁺ + S⁺. As a result, the mixed behavior observed from the angular distributions of the different molecules stands in contrast to the relative consistency of the magnitude of the bond rearrangement branching ratio.

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Research Organization:: Kansas State Univ., Manhattan, KS (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division; National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0002378; FG02-86ER13491; FG02-09ER16115; PHYS-175777; PHY-1723002

OSTI ID:: 1610700

Alternate ID(s):: OSTI ID: 1512820

Journal Information:: Physical Review A, Vol. 99, Issue 5; ISSN 2469-9926

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 16 works

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Strong-field control of H3+ production from methanol dications: Selecting between local and extended formation mechanisms Iwamoto, Naoki; Schwartz, Charles J.; Jochim, Bethany The Journal of Chemical Physics, Vol. 152, Issue 5 https://doi.org/10.1063/1.5129946	journal	February 2020

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