skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Pulse-duration dependence of the double-to-single ionization ratio of Ne by intense 780-nm and 800-nm laser fields: Comparison of simulations with experiments

Journal Article · · Physical Review A
 [1];  [1];  [1];  [2];  [2];  [3];  [4]
  1. Shantou University (China)
  2. Drake University, Des Moines, IO (United States)
  3. The University of Electro-Communications, Tokyo (Japan)
  4. Kansas State Univ., Manhattan, KS (United States)

Accurate ab initio calculations of the ratio of double-to-single ionization of Ne atoms in strong laser fields are difficult due to the many-electron nature of the target. Here, with accurate total cross sections carefully evaluated by using the state-of-the-art many-electron R-matrix theory for both electron-impact ionization and electron-impact excitation of Ne+, we simulate the total double-ionization yields of Ne2+ in strong laser fields at 780 and 800 nm for pulse durations in the range from 7.5 to 200 fs based on the improved quantitative rescattering model. The corresponding single-ionization yields of Ne+ are calculated within the nonadiabatic tunneling model of Perelomov, Popov, and Terent'ev. The ratio of double-to-single ionization of Ne is then obtained from the calculated double- and single-ionization yields. By normalizing the ratio to the one calculated from solving the time-dependent Schrödinger equation for a short few-cycle pulse, we make quantitative comparisons of our results with experimental data to show that our model predicts the experimental findings very well. Lastly, we analyze the pulse-duration dependence of the double-to-single ionization ratio.

Research Organization:
Kansas State Univ., Manhattan, KS (United States)
Sponsoring Organization:
National Science Foundation (NSF); National Natural Science Foundation of China (NSFC); JJapan Society for the Promotion of Science (JSPS); Scientific Research Foundation for the Returned Overseas Chinese Scholars; USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division; USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences, and Biosciences Division; Japan Society for the Promotion of Science KAKENHI
Grant/Contract Number:
FG02-86ER13491; PHY-1430245; PHY-1520970; PHY-1803844; 11274219; 16H04029; 16H04103; 17K05597
OSTI ID:
1610048
Alternate ID(s):
OSTI ID: 1505841
Journal Information:
Physical Review A, Vol. 99, Issue 4; ISSN 2469-9926
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 11 works
Citation information provided by
Web of Science

References (42)

Multiply Charged Ions Formed by Multiphoton Absorption Processes in the Continuum journal June 1982
Coulomb focusing in intense field atomic processes journal October 1996
Ratios of double to single ionization of He and Ne by strong 400-nm laser pulses using the quantitative rescattering theory journal January 2018
Direct and rescattered electrons in above-threshold detachment from negative ions journal November 2003
Production of high-charge states of Xe in a femtosecond laser pulse journal May 1999
Physics of correlated double ionization of atoms in intense laser fields: Quasistatic tunneling limit journal February 2001
Correlation dynamics between electrons and ions in the fragmentation of D 2 molecules by short laser pulses journal October 2003
Non-sequential multiple ionization of rare gas atoms in a Ti:Sapphire laser field journal March 1998
Two-dimensional electron momentum spectra of argon ionized by short intense lasers: Comparison of theory with experiment journal February 2007
Ultrastrong Field Ionization of Ne n + ( n 8 ) : Rescattering and the Role of the Magnetic Field journal June 2005
Double ionization in the perturbative and tunneling regimes journal August 1993
Few Cycle Dynamics of Multiphoton Double Ionization journal April 2001
Quantitative rescattering theory for laser-induced high-energy plateau photoelectron spectra journal March 2009
Elements of the quantitative rescattering theory journal April 2018
Correlated multiphoton double ionization of helium: The role of nonadiabatic tunneling and singlet recollision journal August 2001
Observation of nonsequential double ionization of helium with optical tunneling journal November 1992
Numerical simulation of the double-to-single ionization ratio for the helium atom in strong laser fields journal December 2015
Above threshold ionization beyond the high harmonic cutoff journal March 1993
Nonsequential Double Ionization of Helium journal March 1997
Quantitative rescattering theory for nonsequential double ionization of atoms by intense laser pulses journal January 2009
Theories of photoelectron correlation in laser-driven multiple atomic ionization journal July 2012
The B -spline R -matrix method for atomic processes: application to atomic structure, electron collisions and photoionization journal May 2013
Rescattering nonsequential ionization of Ne 3 + , Ne 4 + , Ne 5 + , Kr 5 + , Kr 6 + , Kr 7 + , and Kr 8 + in a strong, ultraviolet, ultrashort laser pulse journal October 2012
Momentum Distributions of Ne n + Ions Created by an Intense Ultrashort Laser Pulse journal January 2000
Nonsequential Double Ionization as a Completely Classical Photoelectric Effect journal March 2005
Single- and multiple-electron dynamics in the strong-field tunneling limit journal November 1998
Separation of Recollision Mechanisms in Nonsequential Strong Field Double Ionization of Ar: The Role of Excitation Tunneling journal July 2001
Electron-impact ionization cross-sections and ionization rate coefficients for atoms and ions from hydrogen to calcium journal June 1968
Analytical model for calibrating laser intensity in strong-field-ionization experiments journal February 2016
S -matrix analysis of ionization yields of noble gas atoms at the focus of Ti:sapphire laser pulses journal July 1999
Analysis of two-dimensional high-energy photoelectron momentum distributions in the single ionization of atoms by intense laser pulses journal October 2007
Plasma perspective on strong field multiphoton ionization journal September 1993
Roothaan-Hartree-Fock atomic wavefunctions journal September 1974
Rings in above-threshold ionization: A quasiclassical analysis journal February 1995
Strong Field Ionization Rate for Arbitrary Laser Frequencies journal November 2008
ATI as a source for multiply charged ion production in a laser field journal December 1995
Classical Effects of Laser Pulse Duration on Strong-Field Double Ionization journal November 2005
Interplay of electron correlation and intense field dynamics in the double ionization of helium journal March 1999
Experimental investigation of strong-field-ionization theories for laser fields from visible to midinfrared frequencies journal December 2017
Precision Measurement of Strong Field Double Ionization of Helium journal August 1994
Multiply charged ions induced by multiphoton absorption in rare gases at 0.53 μm journal May 1983
Recollision model for double ionization of atoms in strong laser fields journal June 2000

Cited By (1)

Wavelength-dependent nonsequential double ionization of magnesium by intense femtosecond laser pulses journal September 2019

Figures / Tables (6)