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Quantum phase transition and ferromagnetism in C o1+x Sn

Journal Article · · Physical Review B
 [1];  [1];  [2];  [3];  [1];  [1];  [2];  [3];  [3];  [4];  [1]
  1. Univ. of Nebraska, Lincoln, NE (United States)
  2. IIT Mandi, Himachal Pradesh (India)
  3. Ames Lab., and Iowa State Univ., Ames, IA (United States)
  4. Univ. of Delaware, Newark, DE (United States)
The onset of ferromagnetism in cobalt-tin alloys is investigated experimentally and theoretically. The Co1+xSn alloys were prepared by rapid quenching from the melt and form a modified hexagonal NiAs-type crystal structure for 0.45 ≤ x ≤ 1. The magnetic behavior is described analytically and by density-functional theory using supercells and the coherent-potential approximation. The excess of Co concentration x, which enters the interstitial 2d sites in the hypothetical NiAs-ordered parent alloy CoSn, yields a Griffiths-like phase and, above a quantum critical point (xc ≈ 0.65), a quantum phase transition to ferromagnetic order. Quantum critical exponents are determined on the paramagnetic and ferromagnetic sides of the transition and related to the nature of the magnetism in itinerant systems with different types of chemical disorder.
Research Organization:
Ames Laboratory (AMES), Ames, IA (United States); Iowa State Univ., Ames, IA (United States); Univ. of Delaware, Newark, DE (United States); Univ. of Nebraska, Lincoln, NE (United States)
Sponsoring Organization:
National Science Foundation; National Science Foundation (NSF); USDOE Office of Science (SC)
Grant/Contract Number:
AC02-07CH11358; FG02-04ER46152; FG02-90ER45413
OSTI ID:
1609559
Alternate ID(s):
OSTI ID: 1700694
OSTI ID: 1518501
Report Number(s):
IS--J-9959
Journal Information:
Physical Review B, Journal Name: Physical Review B Journal Issue: 18 Vol. 99; ISSN 2469-9950; ISSN PRBMDO
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

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Cited By (2)

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Figures / Tables (14)