Charge distribution guided by grain crystallographic orientations in polycrystalline battery materials

Xu, Zhengrui; Jiang, Zhisen; Kuai, Chunguang; Xu, Rong; Qin, Changdong; Zhang, Yan; Rahman, Muhammad Mominur; Wei, Chenxi; Nordlund, Dennis; Sun, Cheng-Jun; Xiao, Xianghui; Du, Xi-Wen; Zhao, Kejie; Yan, Pengfei; Liu, Yijin; Lin, Feng

doi:10.1038/s41467-019-13884-x

Charge distribution guided by grain crystallographic orientations in polycrystalline battery materials

Journal Article · Wed Jan 08 00:00:00 EST 2020 · Nature Communications

DOI:https://doi.org/10.1038/s41467-019-13884-x· OSTI ID:1619727

Xu, Zhengrui; Jiang, Zhisen; Kuai, Chunguang; ; Qin, Changdong; Zhang, Yan; Rahman, Muhammad Mominur; Wei, Chenxi; ; Sun, Cheng-Jun; ; ; ; ; ;

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States); Argonne National Laboratory (ANL), Argonne, IL (United States). Advanced Photon Source (APS); Brookhaven National Laboratory (BNL), Upton, NY (United States). National Synchrotron Light Source II (NSLS-II); SLAC National Accelerator Laboratory, Menlo Park, CA (United States). Stanford Synchrotron Radiation Lightsource (SSRL)

Sponsoring Organization:: National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC02-06CH11357; AC02-76SF00515; SC0012704

OSTI ID:: 1619727

Alternate ID(s):: OSTI ID: 1603289
OSTI ID: 1605379
OSTI ID: 1630079

Report Number(s):: BNL--213685-2020-JAAM; 83; PII: 13884

Journal Information:: Nature Communications, Journal Name: Nature Communications Journal Issue: 1 Vol. 11; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United Kingdom

Language:: English

References (50)

High‐Voltage Charging‐Induced Strain, Heterogeneity, and Micro‐Cracks in Secondary Particles of a Nickel‐Rich Layered Cathode Material Mao, Yuwei; Wang, Xuelong; Xia, Sihao Advanced Functional Materials, Vol. 29, Issue 18 https://doi.org/10.1002/adfm.201900247	journal	March 2019
Persistent State-of-Charge Heterogeneity in Relaxed, Partially Charged Li ₁₋ _x Ni _1/3 Co _1/3 Mn _1/3 O ₂ Secondary Particles Gent, William E.; Li, Yiyang; Ahn, Sungjin Advanced Materials, Vol. 28, Issue 31 https://doi.org/10.1002/adma.201601273	journal	May 2016
Revealing the Atomic Origin of Heterogeneous Li‐Ion Diffusion by Probing Na Xiao, Biwei; Wang, Kuan; Xu, Gui‐Liang Advanced Materials, Vol. 31, Issue 29 https://doi.org/10.1002/adma.201805889	journal	May 2019
Observation of Microstructural Evolution in Li Battery Cathode Oxide Particles by In Situ Electron Microscopy Miller, Dean J.; Proff, Christian; Wen, J. G. Advanced Energy Materials, Vol. 3, Issue 8 https://doi.org/10.1002/aenm.201300015	journal	May 2013
Nonequilibrium Pathways during Electrochemical Phase Transformations in Single Crystals Revealed by Dynamic Chemical Imaging at Nanoscale Resolution Yu, Young-Sang; Kim, Chunjoong; Liu, Yijin Advanced Energy Materials, Vol. 5, Issue 7 https://doi.org/10.1002/aenm.201402040	journal	December 2014
Microstructure‐Controlled Ni‐Rich Cathode Material by Microscale Compositional Partition for Next‐Generation Electric Vehicles Kim, Un‐Hyuck; Ryu, Hoon‐Hee; Kim, Jae‐Hyung Advanced Energy Materials, Vol. 9, Issue 15 https://doi.org/10.1002/aenm.201803902	journal	February 2019
Radially Oriented Single‐Crystal Primary Nanosheets Enable Ultrahigh Rate and Cycling Properties of LiNi _0.8 Co _0.1 Mn _0.1 O ₂ Cathode Material for Lithium‐Ion Batteries Xu, Xing; Huo, Hua; Jian, Jiyuan Advanced Energy Materials, Vol. 9, Issue 15 https://doi.org/10.1002/aenm.201803963	journal	February 2019
Understanding the Effect of Local Short-Range Ordering on Lithium Diffusion in Li1.3Nb0.3Mn0.4O2 Single-Crystal Cathode Kan, Wang Hay; Deng, Biao; Xu, Yahong Chem, Vol. 4, Issue 9 https://doi.org/10.1016/j.chempr.2018.05.008	journal	September 2018
Heterogeneous damage in Li-ion batteries: Experimental analysis and theoretical modeling Xu, Rong; Yang, Yang; Yin, Fei Journal of the Mechanics and Physics of Solids, Vol. 129 https://doi.org/10.1016/j.jmps.2019.05.003	journal	August 2019
Charge Heterogeneity and Surface Chemistry in Polycrystalline Cathode Materials Tian, Chixia; Xu, Yahong; Nordlund, Dennis Joule, Vol. 2, Issue 3 https://doi.org/10.1016/j.joule.2017.12.008	journal	March 2018
Chemomechanical interplay of layered cathode materials undergoing fast charging in lithium batteries Xia, Sihao; Mu, Linqin; Xu, Zhengrui Nano Energy, Vol. 53 https://doi.org/10.1016/j.nanoen.2018.09.051	journal	November 2018
Unraveling the Complex Delithiation Mechanisms of Olivine-Type Cathode Materials, LiFe _x Co _{1– x} PO ₄ Strobridge, Fiona C.; Liu, Hao; Leskes, Michal Chemistry of Materials, Vol. 28, Issue 11 https://doi.org/10.1021/acs.chemmater.6b00319	journal	May 2016
High-Energy Ni-Rich Li[Ni _x Co _y Mn _{1 –x–y} ]O ₂ Cathodes via Compositional Partitioning for Next-Generation Electric Vehicles Yoon, Chong S.; Park, Kang-Joon; Kim, Un-Hyuck Chemistry of Materials, Vol. 29, Issue 24 https://doi.org/10.1021/acs.chemmater.7b04047	journal	November 2017
Capacity Fading of Ni-Rich Li[Ni _x Co _y Mn _{1– x – y} ]O ₂ (0.6 ≤ x ≤ 0.95) Cathodes for High-Energy-Density Lithium-Ion Batteries: Bulk or Surface Degradation? Ryu, Hoon-Hee; Park, Kang-Joon; Yoon, Chong S. Chemistry of Materials, Vol. 30, Issue 3 https://doi.org/10.1021/acs.chemmater.7b05269	journal	January 2018
Mesoscale Chemomechanical Interplay of the LiNi _0.8 Co _0.15 Al _0.05 O ₂ Cathode in Solid-State Polymer Batteries Besli, Münir M.; Xia, Sihao; Kuppan, Saravanan Chemistry of Materials, Vol. 31, Issue 2 https://doi.org/10.1021/acs.chemmater.8b04418	journal	December 2018
Synchrotron X-ray Analytical Techniques for Studying Materials Electrochemistry in Rechargeable Batteries Lin, Feng; Liu, Yijin; Yu, Xiqian Chemical Reviews, Vol. 117, Issue 21 https://doi.org/10.1021/acs.chemrev.7b00007	journal	September 2017
Visualization of Inhomogeneous Reaction Distribution in the Model LiCoO ₂ Composite Electrode of Lithium Ion Batteries Nakamura, Takashi; Watanabe, Toshiki; Kimura, Yuta The Journal of Physical Chemistry C, Vol. 121, Issue 4 https://doi.org/10.1021/acs.jpcc.6b12133	journal	January 2017
Intergranular Cracking as a Major Cause of Long-Term Capacity Fading of Layered Cathodes Liu, Hao; Wolf, Mark; Karki, Khim Nano Letters, Vol. 17, Issue 6 https://doi.org/10.1021/acs.nanolett.7b00379	journal	May 2017
In situ Visualization of State-of-Charge Heterogeneity within a LiCoO ₂ Particle that Evolves upon Cycling at Different Rates Xu, Yahong; Hu, Enyuan; Zhang, Kai ACS Energy Letters, Vol. 2, Issue 5 https://doi.org/10.1021/acsenergylett.7b00263	journal	April 2017
Crystal Orientation Tuning of LiFePO ₄ Nanoplates for High Rate Lithium Battery Cathode Materials Wang, Li; He, Xiangming; Sun, Wenting Nano Letters, Vol. 12, Issue 11 https://doi.org/10.1021/nl3027839	journal	October 2012
Intercalation Pathway in Many-Particle LiFePO ₄ Electrode Revealed by Nanoscale State-of-Charge Mapping Chueh, William C.; El Gabaly, Farid; Sugar, Joshua D. Nano Letters, Vol. 13, Issue 3 https://doi.org/10.1021/nl3031899	journal	February 2013
Nanoscale Imaging of Lithium Ion Distribution During In Situ Operation of Battery Electrode and Electrolyte Holtz, Megan E.; Yu, Yingchao; Gunceler, Deniz Nano Letters, Vol. 14, Issue 3 https://doi.org/10.1021/nl404577c	journal	February 2014
Phase transformation mechanism in lithium manganese nickel oxide revealed by single-crystal hard X-ray microscopy Kuppan, Saravanan; Xu, Yahong; Liu, Yijin Nature Communications, Vol. 8, Issue 1 https://doi.org/10.1038/ncomms14309	journal	February 2017
Phase evolution for conversion reaction electrodes in lithium-ion batteries Lin, Feng; Nordlund, Dennis; Weng, Tsu-Chien Nature Communications, Vol. 5, Issue 1 https://doi.org/10.1038/ncomms4358	journal	February 2014
In operando tracking phase transformation evolution of lithium iron phosphate with hard X-ray microscopy Wang, Jiajun; Chen-Wiegart, Yu-chen Karen; Wang, Jun Nature Communications, Vol. 5, Issue 1 https://doi.org/10.1038/ncomms5570	journal	August 2014
Visualization of electrochemically driven solid-state phase transformations using operando hard X-ray spectro-imaging Li, Linsen; Chen-Wiegart, Yu-chen Karen; Wang, Jiajun Nature Communications, Vol. 6, Issue 1 https://doi.org/10.1038/ncomms7883	journal	April 2015
In-operando high-speed tomography of lithium-ion batteries during thermal runaway Finegan, Donal P.; Scheel, Mario; Robinson, James B. Nature Communications, Vol. 6, Issue 1 https://doi.org/10.1038/ncomms7924	journal	April 2015
Metal segregation in hierarchically structured cathode materials for high-energy lithium batteries Lin, Feng; Nordlund, Dennis; Li, Yuyi Nature Energy, Vol. 1, Issue 1 https://doi.org/10.1038/nenergy.2015.4	journal	January 2016
Reversible redox reactions in an epitaxially stabilized SrCoOx oxygen sponge Jeen, Hyoungjeen; Choi, Woo Seok; Biegalski, Michael D. Nature Materials, Vol. 12, Issue 11 https://doi.org/10.1038/nmat3736	journal	August 2013
Current-induced transition from particle-by-particle to concurrent intercalation in phase-separating battery electrodes Li, Yiyang; El Gabaly, Farid; Ferguson, Todd R. Nature Materials, Vol. 13, Issue 12 https://doi.org/10.1038/nmat4084	journal	September 2014
Three-dimensional localization of nanoscale battery reactions using soft X-ray tomography Yu, Young-Sang; Farmand, Maryam; Kim, Chunjoong Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-03401-x	journal	March 2018
Coupling of electrochemically triggered thermal and mechanical effects to aggravate failure in a layered cathode Yan, Pengfei; Zheng, Jianming; Chen, Tianwu Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-04862-w	journal	June 2018
Propagation topography of redox phase transformations in heterogeneous layered oxide cathode materials Mu, Linqin; Yuan, Qingxi; Tian, Chixia Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-05172-x	journal	July 2018
Trace doping of multiple elements enables stable battery cycling of LiCoO2 at 4.6 V Zhang, Jie-Nan; Li, Qinghao; Ouyang, Chuying Nature Energy, Vol. 4, Issue 7 https://doi.org/10.1038/s41560-019-0409-z	journal	June 2019
Rapid Mapping of Lithiation Dynamics in Transition Metal Oxide Particles with Operando X-ray Absorption Spectroscopy Nowack, Lea; Grolimund, Daniel; Samson, Vallerie Scientific Reports, Vol. 6, Issue 1 https://doi.org/10.1038/srep21479	journal	February 2016
Profiling the nanoscale gradient in stoichiometric layered cathode particles for lithium-ion batteries Lin, Feng; Nordlund, Dennis; Markus, Isaac M. Energy & Environmental Science, Vol. 7, Issue 9 https://doi.org/10.1039/C4EE01400F	journal	January 2014
An Li-rich oxide cathode material with mosaic spinel grain and a surface coating for high performance Li-ion batteries Liu, Hui; Du, Chunyu; Yin, Geping Journal of Materials Chemistry A, Vol. 2, Issue 37 https://doi.org/10.1039/C4TA02947J	journal	January 2014
A review of Ni-based layered oxides for rechargeable Li-ion batteries Xu, Jing; Lin, Feng; Doeff, Marca M. Journal of Materials Chemistry A, Vol. 5, Issue 3 https://doi.org/10.1039/C6TA07991A	journal	January 2017
A highly stabilized nickel-rich cathode material by nanoscale epitaxy control for high-energy lithium-ion batteries Kim, Junhyeok; Ma, Hyunsoo; Cha, Hyungyeon Energy & Environmental Science, Vol. 11, Issue 6 https://doi.org/10.1039/C8EE00155C	journal	January 2018
Empowering multicomponent cathode materials for sodium ion batteries by exploring three-dimensional compositional heterogeneities Rahman, Muhammad Mominur; Xu, Yahong; Cheng, Hao Energy & Environmental Science, Vol. 11, Issue 9 https://doi.org/10.1039/C8EE00309B	journal	January 2018
Chemomechanical behaviors of layered cathode materials in alkali metal ion batteries Xu, Zhengrui; Rahman, Muhammad Mominur; Mu, Linqin Journal of Materials Chemistry A, Vol. 6, Issue 44 https://doi.org/10.1039/C8TA06875E	journal	January 2018
Three-dimensional imaging of chemical phase transformations at the nanoscale with full-field transmission X-ray microscopy Meirer, Florian; Cabana, Jordi; Liu, Yijin Journal of Synchrotron Radiation, Vol. 18, Issue 5 https://doi.org/10.1107/S0909049511019364	journal	July 2011
TXM-Wizard : a program for advanced data collection and evaluation in full-field transmission X-ray microscopy Liu, Yijin; Meirer, Florian; Williams, Phillip A. Journal of Synchrotron Radiation, Vol. 19, Issue 2 https://doi.org/10.1107/S0909049511049144	journal	January 2012
A Reversible Solid-State Crystalline Transformation in a Metal Phosphide Induced by Redox Chemistry Souza, D. C. S. Science, Vol. 296, Issue 5575 https://doi.org/10.1126/science.1071079	journal	June 2002
Visualization and Quantification of Electrochemical and Mechanical Degradation in Li Ion Batteries Ebner, M.; Marone, F.; Stampanoni, M. Science, Vol. 342, Issue 6159 https://doi.org/10.1126/science.1241882	journal	October 2013
Capturing metastable structures during high-rate cycling of LiFePO4 nanoparticle electrodes Liu, H.; Strobridge, F. C.; Borkiewicz, O. J. Science, Vol. 344, Issue 6191 https://doi.org/10.1126/science.1252817	journal	June 2014
Origin and hysteresis of lithium compositional spatiodynamics within battery primary particles Lim, Jongwoo; Li, Yiyang; Alsem, Daan Hein Science, Vol. 353, Issue 6299 https://doi.org/10.1126/science.aaf4914	journal	August 2016
“Electrochemical Shock” of Intercalation Electrodes: A Fracture Mechanics Analysis Woodford, William H.; Chiang, Yet-Ming; Carter, W. Craig Journal of The Electrochemical Society, Vol. 157, Issue 10 https://doi.org/10.1149/1.3464773	journal	January 2010
Visualization of the State-of-Charge Distribution in a LiCoO ₂ Cathode by In Situ Raman Imaging Nishi, Toshio; Nakai, Hideki; Kita, Akinori Journal of The Electrochemical Society, Vol. 160, Issue 10 https://doi.org/10.1149/2.061310jes	journal	January 2013
Depth-Dependent Redox Behavior of LiNi _0.6 Mn _0.2 Co _0.2 O ₂ Tian, Chixia; Nordlund, Dennis; Xin, Huolin L. Journal of The Electrochemical Society, Vol. 165, Issue 3 https://doi.org/10.1149/2.1021803jes	journal	January 2018

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Charge distribution guided by grain crystallographic orientations in polycrystalline battery materials

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