Nanowire Photoelectrochemistry

Deng, Jiao; Su, Yude; Liu, Dong; Yang, Peidong; Liu, Bin; Liu, Chong

doi:10.1021/acs.chemrev.9b00232

Nanowire Photoelectrochemistry

Journal Article · Tue Jul 23 00:00:00 EDT 2019 · Chemical Reviews

DOI:https://doi.org/10.1021/acs.chemrev.9b00232· OSTI ID:1601204

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Univ. of California, Los Angeles, CA (United States)
Univ. of California, Berkeley, CA (United States)
Nanyang Technological Univ. (Singapore)
Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Kavli Energy NanoScience Institute, Berkeley, CA (United States)

Recent applications of photoelectrochemistry at the semiconductor/liquid interface provide a renewable route of mimicking natural photosynthesis and yielding chemicals from sunlight, water, and air. Nanowires, defined as one-dimensional nanostructures, exhibit multiple unique features for photoelectrochemical applications and promise better performance as compared to their bulk counterparts. Here, this article reviews the use of semiconductor nanowires in photoelectrochemistry. After introducing fundamental concepts essential to understanding nanowires and photoelectrochemistry, the review considers answers to the following questions: (1) How can we interface semiconductor nanowires with other building blocks for enhanced photoelectrochemical responses? (2) How are nanowires utilized for photoelectrochemical half reactions? (3) What are the techniques that allow us to obtain fundamental insights of photoelectrochemistry at single-nanowire level? (4) What are the design strategies for an integrated nanosystem that mimics a closed cycle in artificial photosynthesis? This framework should help readers evaluate the salient features of nanowires for photoelectrochemical applications, promoting the sustainable development of solar-powered chemical plants that will benefit our society in the long run.

View Accepted Manuscript (DOE)

Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: Singapore Ministry of Education Academic Research Fund (AcRF); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC02-05CH11231

OSTI ID:: 1601204

Journal Information:: Chemical Reviews, Journal Name: Chemical Reviews Journal Issue: 15 Vol. 119; ISSN 0009-2665

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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