skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Geometrically Tunable Beamed Light Emission from a Quantum‐Dot Ensemble Near a Gradient Metasurface

Journal Article · · Advanced Optical Materials
 [1];  [1];  [2];  [1];  [2]; ORCiD logo [1]
  1. Department of Electrical and Computer Engineering and Photonics Center Boston University 8 Saint Mary's Street Boston MA 02215 USA
  2. Department of Biomedical Engineering and Division of Materials Science and Engineering Boston University 8 St. Mary's St. Boston MA 02215 USA

Abstract Optical metasurfaces have been widely investigated in recent years as a means to tailor the wavefronts of externally incident light for passive device applications. At the same time, their use in active optoelectronic devices such as light emitters is far less established. This work explores their ability to control the radiation properties of a nearby continuous ensemble of randomly oriented incoherent dipole sources via near‐field interactions. Specifically, a film of colloidal quantum dots is deposited on a plasmonic metasurface consisting of a 1D array of metallic nanoantennas on a metal film. The array is designed to introduce a linear phase profile upon reflection, and a bi‐periodic nanoparticle arrangement is introduced to ensure adequate sampling of the desired phase gradient. Highly directional radiation patterns are correspondingly obtained from the quantum dots at an enhanced emission rate. The underlying radiation mechanism involves the near‐field excitation of surface plasmon polaritons at the metal film, and their selective diffractive scattering by the metasurface into well‐collimated beams along predetermined geometrically tunable directions. These results underscore the distinctive ability of metasurfaces to control radiation properties directly at the source level, which is technologically significant for the continued miniaturization and large‐scale integration of optoelectronic devices.

Sponsoring Organization:
USDOE
OSTI ID:
1601012
Journal Information:
Advanced Optical Materials, Journal Name: Advanced Optical Materials Vol. 8 Journal Issue: 8; ISSN 2195-1071
Publisher:
Wiley Blackwell (John Wiley & Sons)Copyright Statement
Country of Publication:
Germany
Language:
English
Citation Metrics:
Cited by: 7 works
Citation information provided by
Web of Science

References (35)

On-chip beam-steering photonic-crystal lasers journal May 2010
Plasmonic off-axis unidirectional beaming of quantum-well luminescence journal December 2013
Flat optics with designer metasurfaces journal February 2014
Enhanced Spontaneous Emission by Quantum Boxes in a Monolithic Optical Microcavity journal August 1998
Light-emitting metasurfaces journal July 2019
Coupling localized and extended plasmons to improve the light extraction through metal films journal January 2007
Enhancement and Quenching of Single-Molecule Fluorescence journal March 2006
Non-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion journal August 2015
Plasmonic Enhancement of Molecular Fluorescence journal February 2007
Spontaneous emission extraction and Purcell enhancement from thin-film 2-D photonic crystals journal January 1999
Fluorescence near interfaces: The role of photonic mode density journal April 1998
Shaping Photoluminescence Spectra with Magnetoelectric Resonances in All-Dielectric Nanoparticles journal January 2015
Spontaneous-emission control by photonic crystals and nanocavities journal August 2007
Large Enhancement of Fluorescence Efficiency from CdSe/ZnS Quantum Dots Induced by Resonant Coupling to Spatially Controlled Surface Plasmons journal August 2005
All-Dielectric Silicon Nanogap Antennas To Enhance the Fluorescence of Single Molecules journal July 2016
Unidirectional Emission of a Quantum Dot Coupled to a Nanoantenna journal August 2010
Enhanced near-green light emission from InGaN quantum wells by use of tunable plasmonic resonances in silver nanoparticle arrays journal January 2010
Bright Unidirectional Fluorescence Emission of Molecules in a Nanoaperture with Plasmonic Corrugations journal February 2011
III-nitride photonic-crystal light-emitting diodes with high extraction efficiency journal February 2009
Ultrafast spontaneous emission source using plasmonic nanoantennas journal July 2015
Circularly Symmetric Light Scattering from Nanoplasmonic Spirals journal May 2011
Lighting Up Multipolar Surface Plasmon Polaritons by Collective Resonances in Arrays of Nanoantennas journal December 2010
Quantum Dot Emission Driven by Mie Resonances in Silicon Nanostructures journal October 2017
Directional and Spectral Shaping of Light Emission with Mie-Resonant Silicon Nanoantenna Arrays journal January 2018
Recent advances in planar optics: from plasmonic to dielectric metasurfaces journal January 2017
Light Emission near a Gradient Metasurface journal January 2016
Control of LED Emission with Functional Dielectric Metasurfaces journal November 2019
Plasmonics for solid-state lighting: enhanced excitation and directional emission of highly efficient light sources journal May 2013
Plasmonic phase-gradient metasurface for spontaneous emission control journal November 2015
Efficient unidirectional polarization-controlled excitation of surface plasmon polaritons journal August 2014
Metalenses at visible wavelengths: past, present, perspectives: Metalenses at visible wavelengths: past, present, perspectives journal May 2017
Plasmonic beaming and active control over fluorescent emission journal April 2011
Gradient metasurfaces: a review of fundamentals and applications journal December 2017
High-Efficiency Broadband Anomalous Reflection by Gradient Meta-Surfaces journal February 2012
Enhancement of Single-Molecule Fluorescence Using a Gold Nanoparticle as an Optical Nanoantenna journal July 2006

Similar Records

Related Subjects