Low-temperature MnBi alloys: Electronic and magnetic properties, constitution, morphology and fabrication (Review article)

Antonov, V. N.; Antropov, V. P.

doi:10.1063/10.0000360

Title: Low-temperature MnBi alloys: Electronic and magnetic properties, constitution, morphology and fabrication (Review article)

Journal Article · Thu Jan 30 00:00:00 EST 2020 · Low Temperature Physics

DOI:https://doi.org/10.1063/10.0000360· OSTI ID:1599882

Antonov, V. N. ^[1]; Antropov, V. P. ^[2]

NAS of Ukraine, Kyiv (Ukraine). G. V. Kurdyumov Inst. for Metal Physics; Ames Lab., Ames, IA (United States)
Ames Lab., Ames, IA (United States)

The article reviews the rich phenomena of physical properties of MnBi. The diverse phenomena include strong spin-orbit interaction, anomalous temperature dependence of the coercivity and the magneto-crystalline anisotropy field, unique magneto-optical properties. Issues addressed include the nature of the electronic ground states of MnBi, the electronic and magnetic structures, Fermi surface, magneto-crystalline anisotropy, x-ray magnetic dichroism. The discussion includes key experiments, such as optical and magneto-optical spectroscopic measurements, de Haas-van Alphen (dHvA) measurements, x-ray photoemission and x-ray absorption spectroscopy measurements as well as x-ray magnetic circular dichroism. The effect of the spin-orbit (SO) interaction and Coulomb repulsion U were found to be crucial for the Fermi surface, cyclotron masses, magneto-optical properties, and x-ray magnetic circular dichroism. The microscopic origin of unique magneto-crystalline anisotropy and giant Kerr effect in MnBi is analyzed in detail. The huge Kerr effect in MnBi is caused by the combination of a sizable magnetic moment on manganese, the large spin-orbit coupling of bismuth, and a strong hybridization between the manganese 3d and the bismuth 6p states. The magneto-optically active states are mainly the 6p states of Bi. We show that the observed temperature dependence of the magneto-crystalline anisotropy can be explained taking into account the spin-orbit interaction together with strong Coulomb electron-electron interaction. The SO coupling of Bi is equally responsible for the large magneto-crystalline anisotropy energy as is the exchange splitting of Mn. The fabrication, morphology, and constitution of low-temperature MnBi alloys in bulk, thin films, and nanoparticles are discussed. The nanocomposite permanent magnetic materials based on MnBi, (Co, Fe) and Nd₂Fe₁₄B are also discussed.

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Research Organization:: Ames Lab., Ames, IA (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC02-07CH11358

OSTI ID:: 1599882

Report Number(s):: IS-J-10151; TRN: US2103766

Journal Information:: Low Temperature Physics, Vol. 46, Issue 1; ISSN 1063-777X

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 13 works

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Title: Low-temperature MnBi alloys: Electronic and magnetic properties, constitution, morphology and fabrication (Review article)

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