Magnetic and transport behaviors of non-centrosymmetric Nd7Ni2Pd

Pathak, Arjun K.; Mudryk, Y.; Provino, A.; Manfrinetti, P.; Pecharsky, V. K.

doi:10.1063/1.5129907

Title: Magnetic and transport behaviors of non-centrosymmetric Nd₇Ni₂Pd

Journal Article · Thu Jan 02 00:00:00 EST 2020 · AIP Advances

DOI:https://doi.org/10.1063/1.5129907· OSTI ID:1581590

^[1];

^[2]; Provino, A. ^[3]; Manfrinetti, P. ^[3]; Pecharsky, V. K. ^[2]

SUNY Buffalo State, Buffalo, NY (United States)
Ames Lab., and Iowa State Univ., Ames, IA (United States)
Univ. of Genova (Italy); Inst. SPIN-CNR, Genova (Italy)

Crystallographic, magnetic, electrical transport and thermodynamic properties of pseudo-binary Nd₇Ni₂Pd compound have been studied using temperature-dependent x-ray powder diffraction and physical property measurements. Compared to the ferromagnetic parent Nd₇Pd₃, the ground state of Nd₇Ni₂Pd is antiferromagnetic, and it exhibits strong metamagnetism. The measurements indicate two antiferromagnetic transitions in fields less than 8 kOe: a second-order paramagnetic to antiferromagnetic at T_N2 = 29 K and a weak first-order antiferromagnetic to antiferromagnetic transition at T_N1 = 24.5 K. Here, the compound becomes ferromagnetic in fields of 8 kOe and higher with T_C = 30 K. Temperature dependence of lattice parameters is anomalous, most prominently in the basal plane at ~30 K; however, there is no detectable structural distortion or clear volume discontinuity around 25 K, suggesting a significant weakening of the first-order transition when compared to the binary Nd₇Pd₃.

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Research Organization:: Ames Lab., Ames, IA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division

Grant/Contract Number:: AC02-07CH11358; 734303

OSTI ID:: 1581590

Alternate ID(s):: OSTI ID: 1580792

Report Number(s):: IS-J-10130; TRN: US2100761

Journal Information:: AIP Advances, Vol. 10, Issue 1; ISSN 2158-3226

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 1 work

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