Thickness-dependent polarization-induced intrinsic magnetoelectric effects in La0.67Sr0.33MnO3/PbZr0.52Ti0.48O3 heterostructures

Yu, Xiaoqian; Wu, Lijun; Zhang, Bangmin; Zhou, Hua; Dong, Yongqi; Wu, Xiaohan; Kou, Ronghui; Yang, Ping; Chen, Jingsheng; Sun, Cheng-Jun; Zhu, Yimei; Chow, Gan Moog

doi:10.1103/PhysRevB.100.104405

Title: Thickness-dependent polarization-induced intrinsic magnetoelectric effects in $L a_{0.67} S r_{0.33} Mn O_{3} / PbZ r_{0.52} T i_{0.48} O_{3}$ heterostructures

Journal Article · Tue Sep 03 00:00:00 EDT 2019 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.100.104405· OSTI ID:1566881

^[1];

^[2]; Zhang, Bangmin ^[3]; Zhou, Hua ^[4]; Dong, Yongqi ^[4]; Wu, Xiaohan ^[1]; Kou, Ronghui ^[4]; Yang, Ping ^[1]; Chen, Jingsheng ^[1]; Sun, Cheng-Jun ^[4]; Zhu, Yimei ^[2];

^[1]

National Univ. of Singapore (Singapore)
Brookhaven National Lab. (BNL), Upton, NY (United States)
National Univ. of Singapore (Singapore); Sun Yat-Sen Univ., Guangdong (China)
Argonne National Lab. (ANL), Argonne, IL (United States)

The polarization of PbZr0.52Ti0.48O3 thin film is switched by changing film thickness through the competition between the strain relaxation-induced flexoelectric fields and the interfacial effects. Without an applied electric field, this reversal of polarization is exploited to control the magnetic properties of La0.67Sr0.33MnO3 by the competition/cooperation between the charge-mediated and the strain-mediated effects. Scanning transmission electron microscopy, polarized near-edge x-ray absorption spectroscopy, and half-integer diffraction measurements are employed to decode the intrinsic magnetoelectric effects in the La0.67Sr0.33MnO3/PbZr0.52Ti0.48O3 heterostructures. With PbZr0.52Ti0.48O3 films <48 nm, the polarization-driven carrier density modulation around the La0.67ST0.33MnO3/PbZr0.52Ti0.48O3 interface and the strain-mediated Mn 3d orbital occupancy work together to enhance the magnetism of 14-unit-cell La0.67Sr0.33MnO3 film; with PbZr0.52Ti0.48O3 layers >48 nm, the strain-induced change of bond length/angle of MnO6 accompanied with a modified spin configuration are responsible for the decrease in the Curie temperature and magnetization of 14-unit-cell La0.67Sr0.33MnO3 film.

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Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States); Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division

Grant/Contract Number:: SC0012704; AC02-06CH11357

OSTI ID:: 1566881

Alternate ID(s):: OSTI ID: 1560291; OSTI ID: 1572696

Report Number(s):: BNL-212151-2019-JAAM; PRBMDO; TRN: US2001012

Journal Information:: Physical Review B, Vol. 100, Issue 10; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 20 works

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Title: Thickness-dependent polarization-induced intrinsic magnetoelectric effects in $L a_{0.67} S r_{0.33} Mn O_{3} / PbZ r_{0.52} T i_{0.48} O_{3}$ heterostructures