skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Effects of Interface Induced Natural Strains on Magnetic Properties of FeRh

Journal Article · · Nanomaterials
DOI:https://doi.org/10.3390/nano9040574· OSTI ID:1571992
 [1];  [2];  [3];  [4]; ORCiD logo [1]
  1. Huazhong Univ. of Science and Technology, Wuhan (China)
  2. Pennsylvania State Univ., University Park, PA (United States)
  3. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS)
  4. Univ. of California, Berkeley, CA (United States)

FeRh is a unique alloy which shows temperature dependent phase transition magnetic properties. The lattice parameter (a) of this CsCl-type (B2) structure is 4.1712 Å. It undergoes a first order transition from antiferromagnetic (AFM) to ferromagnetic (FM) order at around 370K and hysteretic behavior while cooling and heating. This meta-magnetic transition of FeRh is accompanied by an isotropic expansion in the unit cell volume, which indicates strong coupling between magnetic and structural properties of FeRh. Consequently, the magnetic and transport properties, such as magnetoresistance (MR), are changed during the transition. Due to its unique thermo-magnetic behaviors, FeRh is very important for future spintronic devices. The structure could be applicable for MR devices such as memory, sensors, and many other applications. It is critical to understand how to systematically influence phase transition of FeRh from naturally applied strains. Here, we investigate magnetic properties of FeRh in different strain environments induced by the substrates with different lattice parameters. The study was performed using synchrotron radiation, temperature dependent magnetometry, and magnetic scanning probe microscopy in addition to Landau theory calculations. We found that the naturally induced strains could modulate the magnetic phase locally and globally. The presence of the segments from the nucleation of the ferromagnetic domains, with a very thin layer in the antiferromagnetic matrix and the domain growth, were observed gradually. Using the systematic phenomena, it could be used for immediate applications in the future generation of phase change random access memory (PC-RAM) devices.

Research Organization:
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; National Natural Science Foundation of China (NSFC)
Grant/Contract Number:
AC02-05CH11231
OSTI ID:
1571992
Journal Information:
Nanomaterials, Vol. 9, Issue 4; ISSN 2079-4991
Publisher:
MDPICopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 7 works
Citation information provided by
Web of Science

References (15)

Temperature and field hysteresis of the antiferromagnetic-to-ferromagnetic phase transition in epitaxial FeRh films journal December 2005
Mechanism of the Ferrimagnetic to Antiferromagnetic Transition in Mn 2 x Cr x Sb journal May 1964
Room-temperature antiferromagnetic memory resistor journal January 2014
Instability of the rhodium magnetic moment as the origin of the metamagnetic phase transition in α FeRh journal February 2003
Anomalously high entropy change in FeRh alloy journal February 1996
Effect of strain and thickness on the transition temperature of epitaxial FeRh thin-films journal October 2017
Large resistivity modulation in mixed-phase metallic systems journal January 2015
Model of Exchange-Inversion Magnetization journal October 1960
Interface-induced phenomena in magnetism journal June 2017
Theory of strain phase separation and strain spinodal: Applications to ferroelastic and ferroelectric systems journal July 2017
Lattice Parameter Change of FeRh Alloys due to Antiferromagnetic-Ferromagnetic Transformation journal January 1967
Antiferromagnetic-ferromagnetic phase transition in FeRh probed by x-ray magnetic circular dichroism journal May 2008
Large resistivity modulation in mixed-phase metallic systems text January 2015
Antiferromagnetic-ferromagnetic transition in FeRh journal August 1992
Room-temperature antiferromagnetic memory resistor text January 2015

Similar Records

Antiferromagnetic-ferromagnetic phase domain development in nanopatterned FeRh islands
Journal Article · Mon Oct 01 00:00:00 EDT 2018 · Physical Review Materials · OSTI ID:1571992

Magnetic modification at sub-surface of FeRh bulk by energetic ion beam irradiation
Journal Article · Thu May 07 00:00:00 EDT 2015 · Journal of Applied Physics · OSTI ID:1571992

Magnetic imaging and statistical analysis of the metamagnetic phase transition of FeRh with electron spins in diamond
Journal Article · Tue Jun 08 00:00:00 EDT 2021 · Journal of Applied Physics · OSTI ID:1571992