Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

Simultaneous Iron and Nickel Isotopic Analyses of Presolar Silicon Carbide Grains.

Journal Article · · Geochimica et Cosmochimica Acta
Aside from recording stellar nucleosynthesis, a few elements in presolar grains can also provide insights into the galactic chemical evolution (GCE) of nuclides. We have studied the carbon, silicon, iron, and nickel isotopic compositions of presolar silicon carbide (SiC) grains from asymptotic giant branch (AGB) stars to better understand GCE. Since only the neutron-rich nuclides in these grains have been heavily influenced by the parent star, the neutron-poor nuclides serve as GCE proxies. Using CHILI, a new resonance ionizationmass spectrometry (RIMS) instrument, we measured 74 presolar SiC grains for all iron and nickel isotopes. With the CHARISMA instrument, 13 presolar SiC grains were analyzed for iron isotopes. All grains were also measured by NanoSIMS for their carbon and silicon isotopic compositions. A comparison of the measured neutron-rich isotopes with models for AGB star nucleosynthesis shows that our measurements are consistent with AGB star predictions for low-mass stars between half-solar and solar metallicity. Furthermore, our measurements give an indication on the Ne-22(alpha, n)Mg-25 reaction rate. In terms of GCE, we find that the GCE-dominated iron and nickel isotope ratios, Fe-54/Fe-56 and Ni-60/Ni-58, correlate with their GCE-dominated counterpart in silicon, Si-29/Si-28. The measured GCE trends include the Solar System composition, showing that the Solar System is not a special case. However, as seen in silicon and titanium, many presolar SiC grains are more evolved for iron and nickel than the Solar System. This confirms prior findings and agrees with observations of large stellar samples that a simple age-metallicity relationship for GCE cannot explain the composition of the solar neighborhood. (C) 2017 Elsevier Ltd. All rights reserved.
Research Organization:
Argonne National Laboratory (ANL)
Sponsoring Organization:
National Aeronautic and Space Administration (NASA); USDOE Office of Science
DOE Contract Number:
AC02-06CH11357
OSTI ID:
1571246
Journal Information:
Geochimica et Cosmochimica Acta, Journal Name: Geochimica et Cosmochimica Acta Journal Issue: SI Vol. 221; ISSN 0016-7037
Country of Publication:
United States
Language:
English

References (52)

Iron and nickel isotope compositions of presolar silicon carbide grains from supernovae journal January 2018
Beta-decay rates of highly ionized heavy atoms in stellar interiors journal May 1987
The Evolution of a 25 M Star from the Main Sequence up to the Onset of the Iron Core Collapse journal August 1998
Trace-element concentrations in single circumstellar silicon carbide grains from the Murchison meteorite journal November 1995
Molecular Opacities for Low‐Mass Metal‐poor AGB Stars Undergoing the Third Dredge‐up journal September 2007
Presolar Grains from Novae journal April 2001
Iron and Nickel Isotopic Ratios in Presolar SiC Grains journal December 2008
CHILI – the Chicago Instrument for Laser Ionization – a new tool for isotope measurements in cosmochemistry journal August 2016
Galactic Evolution of Silicon Isotopes: Application to Presolar SiC Grains from Meteorites journal December 1996
Determination of the absolute isotopic composition and Atomic Weight of a reference sample of natural iron journal November 1992
Silicon and Carbon Isotopic Ratios in AGB Stars: SiC Grain Data, Models, and the Galactic Evolution of the Si Isotopes journal October 2006
Reaction rates for O-18(alpha, gamma)Ne-22, Ne-22(alpha, gamma)Mg-26, and Ne-22(alpha, n)Mg-25 in stellar helium burning and s-process nucleosynthesis in massive stars journal December 1994
The evolution of isotope ratios in the Milky Way Galaxy: The evolution of isotope ratios journal May 2011
A Presolar Galactic Merger Spawned the SiC‐Grain Mainstream journal November 2003
Neutron Capture in Low‐Mass Asymptotic Giant Branch Stars: Cross Sections and Abundance Signatures journal November 1999
Anomalous odd- to even-mass isotope ratios in resonance ionization with broad-band lasers journal August 1989
Low-Mass AGB Stellar Models for 0.003 ≤ Z ≤ 0.02: Basic Formulae for Nucleosynthesis Calculations journal January 2003
Absolute isotopic abundance ratios and atomic weight of a reference sample of nickel journal November 1989
Presolar SiC Grains of Type Y: Origin from Low‐Metallicity Asymptotic Giant Branch Stars journal January 2001
THE EFFECTS OF ROTATION ON s -PROCESS NUCLEOSYNTHESIS IN ASYMPTOTIC GIANT BRANCH STARS journal August 2013
The Geneva-Copenhagen survey of the Solar neighbourhood II: New uvby calibrations and rediscussion of stellar ages, the G dwarf problem, age-metallicity diagram, and heating mechanisms of the disk journal August 2007
SILICON CARBIDE GRAINS OF TYPE C PROVIDE EVIDENCE FOR THE PRODUCTION OF THE UNSTABLE ISOTOPE 32 Si IN SUPERNOVAE journal June 2013
Titanium isotopic compositions of well-characterized silicon carbide grains from Orgueil (CI): Implications for s-process nucleosynthesis journal August 2007
Observational evidence for mixing and dust condensation in core-collapse supernovae conference January 1997
Presolar SiC Grains of Type A and B: Their Isotopic Compositions and Stellar Origins journal September 2001
N 22 e ( α , n ) M 25 g : The Key Neutron Source in Massive Stars journal October 2001
The Galactic Evolution of Si, Ti, and O Isotopic Ratios journal July 1999
Solar System Abundances and Condensation Temperatures of the Elements journal July 2003
Radiative C-13 burning in asymptotic giant branch stars and s-processing journal February 1995
Confirmation of mass-independent Ni isotopic variability in iron meteorites journal December 2011
Constraints on Heterogeneous Galactic Chemical Evolution from Meteoritic Stardust journal January 2005
Galactic Chemical Evolution: Carbon through Zinc journal December 2006
Nucleosynthesis in Massive Stars with Improved Nuclear and Stellar Physics journal September 2002
60Fe–60Ni chronology of core formation in Mars journal March 2014
Constraining the 13 C neutron source in AGB stars through isotopic analysis of trace elements in presolar SiC journal August 2007
Nucleosynthesis in type Ia supernovae journal August 1997
Resonance ionization mass spectrometry for precise measurements of isotope ratios journal November 2009
Resonance ionization spectroscopy and one-atom detection journal October 1979
s process in low-mass asymptotic giant branch stars journal October 2006
Iron isotopic measurements in presolar silicate and oxide grains from the Acfer 094 ungrouped carbonaceous chondrite journal July 2015
The ionization potential of neutral iron, Fe I, by multistep laser spectroscopy journal January 1984
Analyzing individual presolar grains with CHARISMA journal September 2003
Si Isotopic Ratios in Mainstream Presolar SiC Grains Revisited journal December 1999
Evolution, Nucleosynthesis, and Yields of Low-Mass Asymptotic Giant Branch Stars at Different Metallicities journal April 2009
Completing the iron period: double-resonance, fluorescence-dip Rydberg spectroscopy and ionization potentials of titanium, vanadium, iron, cobalt, and nickel journal January 1990
Stardust in meteorites journal November 2011
Nucleosynthesis in Stars and the Chemical Enrichment of Galaxies journal August 2013
On the need for the Light Elements Primary Process (Lepp) journal March 2015
Condensation Chemistry of Circumstellar Grains journal January 1999
Correction of dead time effects in time‐of‐flight mass spectrometry
  • Stephan, T.; Zehnpfenning, J.; Benninghoven, A.
  • Journal of Vacuum Science & Technology A: Vacuum, Surfaces, and Films, Vol. 12, Issue 2 https://doi.org/10.1116/1.579255
journal March 1994
Evolution and Nucleosynthesis in Low‐Mass Asymptotic Giant Branch Stars. II. Neutron Capture and the s ‐Process journal April 1998
The branchings of the main s-process: their sensitivity to α-induced reactions on 13C and 22Ne and to the uncertainties of the nuclear network journal March 2015

Cited By (4)

New Constraints on the Major Neutron Source in Low-mass AGB Stars journal September 2018
New Constraints on the Abundance of 60 Fe in the Early Solar System journal April 2018
Resonance ionization of titanium: high useful yield and new autoionizing states journal January 2018
The Importance of the 13 C( α ,n) 16 O Reaction in Asymptotic Giant Branch Stars journal May 2018

Similar Records

Simultaneous iron and nickel isotopic analyses of presolar silicon carbide grains
Journal Article · Sun Dec 31 19:00:00 EST 2017 · Geochimica et Cosmochimica Acta · OSTI ID:1414366

Barium isotopes in individual presolar silicon carbide grains from the Murchison meteorite.
Journal Article · Mon Sep 01 00:00:00 EDT 2003 · Geochim. Cosmochim. Acta · OSTI ID:949642

Iron and nickel isotope compositions of presolar silicon carbide grains from supernovae
Journal Article · Sun May 28 20:00:00 EDT 2017 · Geochimica et Cosmochimica Acta · OSTI ID:1571449