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Title: Effect of Ni doping on vortex pinning in CaK ( F e 1 - x N i x ) 4 A s 4 single crystals

Journal Article · · Physical Review B
ORCiD logo [1];  [2];  [2]; ORCiD logo [3];  [2];  [2]
  1. Ames Lab. and Iowa State Univ., Ames, IA (United States); Centro Atómico Bariloche and Instituto Balseiro (Argentina)
  2. Ames Lab. and Iowa State Univ., Ames, IA (United States)
  3. Ames Lab. and Iowa State Univ., Ames, IA (United States); Univ. de Buenos Aires, Buenos Aires (Argentina)

We study the correlation between chemical composition and vortex dynamics in Ni-doped CaK(Fe1–xNix)4As4 (x = 0, 0.015, 0.025, 0.03, and 0.05) single crystals by performing measurements of the critical current densities Jc and the flux creep rates S. The magnetic relaxation of all the crystals is well described by the collective creep theory. The samples display a glassy exponent μ within the predictions for vortex bundles in a weak pinning scenario and relatively small characteristic pinning energy (U0 < 100K). The undoped crystals display modest Jc values at low temperatures and high magnetic fields applied along the c axis. Jc(T) dependences at high fields display an unusual peak. The enhancement in Jc(T) matches with an increase in U0 and the appearance of a second peak in the magnetization. As Ni doping increases, whereas there is a monotonic decrease in Tc there is a nonmonotonic change in Jc. Initially Jc increases, reaching a maximum value for x = 0.015, and then Jc decreases for x ≥ 0.025. This change in Jc(x) is coincident with the onset of antiferromagnetic order. The magnetic field dependence of Jc(H) also manifests a change in behavior between these x values. The analysis of the vortex dynamics for small and intermediate magnetic fields shows a gradual evolution in the glassy exponent μ with Ni content, x. As a result, this implies that there is no appreciable change in the mechanism that determines the vortex relaxation.

Research Organization:
Ames Lab., Ames, IA (United States)
Sponsoring Organization:
USDOE
Grant/Contract Number:
AC02-07CH11358; GBMF4411
OSTI ID:
1561964
Alternate ID(s):
OSTI ID: 1559358
Report Number(s):
IS-J-10028; PRBMDO; TRN: US2000672
Journal Information:
Physical Review B, Vol. 100, Issue 6; ISSN 2469-9950
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 11 works
Citation information provided by
Web of Science

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Cited By (2)

Enhancement of critical current density in CaKFe 4 As 4 single crystals through 3 MeV proton irradiation journal January 2020
Flux pinning and the vortex phase diagram in optimized CaKFe 4 As 4 single crystals fabricated by a one-step method journal February 2020