Anomalous electron transport in epitaxial NdNiO3 films

Ojha, Shashank Kumar; Ray, Sujay; Das, Tanmoy; Middey, S.; Sarkar, Sagar; Mahadevan, Priya; Wang, Zhen; Zhu, Yimei; Liu, Xiaoran; Kareev, M.; Chakhalian, J.

doi:10.1103/PhysRevB.99.235153

Title: Anomalous electron transport in epitaxial ${NdNiO}_{3}$ films

Journal Article · Thu Jun 27 00:00:00 EDT 2019 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.99.235153· OSTI ID:1561256

Ojha, Shashank Kumar ^[1]; Ray, Sujay ^[1]; Das, Tanmoy ^[1];

^[1]; Sarkar, Sagar ^[2]; Mahadevan, Priya ^[2]; Wang, Zhen ^[3];

^[3]; Liu, Xiaoran ^[4]; Kareev, M. ^[4]; Chakhalian, J. ^[4]

Indian Inst. of Science, Bengaluru (India)
S.N. Bose National Center for Basic Sciences, Kolkata (India)
Brookhaven National Lab. (BNL), Upton, NY (United States)
Rutgers Univ., Piscataway, NJ (United States)

The origin of simultaneous electronic, structural, and magnetic transitions in bulk rare-earth nickelates (RENiO₃) remains puzzling with multiple conflicting reports on the nature of these entangled phase transitions. Heterostructure engineering of these materials offers unique opportunity to decouple the metal-insulator transition (MIT) from the magnetic transition. Yet, the evolution of underlying electronic properties across these decoupled transitions remains largely unexplored. In order to address this, we have calculated Hall effect on a series of epitaxial ${NdNiO}_{3}$ films, spanning a variety of electronic and magnetic phases. We find that the MIT results in only a partially gapped Fermi surface, whereas the full insulating phase forms below the magnetic transition. Moreover, we also find a systematic reduction of the Hall coefficient R_H in the metallic phase of these films with epitaxial strain and also a surprising transition to a negative value at large compressive strain. The partially gapped, weakly insulating, paramagnetic phase is reminiscence of pseudogap behavior of high-T_c cuprates. The precursor metallic phase, which undergoes transition to the insulating phase, is a non-Fermi liquid with a temperature exponent n of resistivity of 1, whereas the exponent increases to 4/3 in the noninsulating samples. Such a nickelate phase diagram with sign reversal of R_H, a pseudogap phase, and non-Fermi-liquid behavior is intriguingly similar to high-T_c cuprates, giving crucial guidelines to engineer unconventional superconductivity in oxide heterostructures.

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Research Organization:: Brookhaven National Lab. (BNL), Upton, NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0012704; SC00012375; AC02-98CH10886; DOE DE-SC 00012375

OSTI ID:: 1561256

Alternate ID(s):: OSTI ID: 1529699

Report Number(s):: BNL-212072-2019-JAAM; PRBMDO; TRN: US2000610

Journal Information:: Physical Review B, Vol. 99, Issue 23; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 13 works

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Asymmetric orbital-lattice interactions in ultra-thin correlated oxide films Chakhalian, J.; Rondinelli, J. M.; Liu, Jian arXiv https://doi.org/10.48550/arxiv.1008.1373	text	January 2010
Dynamical Mean Field Theory of Nickelate Superlattices Han, M. J.; Wang, X.; Marianetti, C. A. arXiv https://doi.org/10.48550/arxiv.1105.0016	text	January 2011
Superconductivity in Iron Compounds Stewart, G. R. arXiv https://doi.org/10.48550/arxiv.1106.1618	text	January 2011
Electronic structure of nickelates: From two-dimensional heterostructures to three-dimensional bulk materials Hansmann, P.; Toschi, A.; Yang, Xiaoping arXiv https://doi.org/10.48550/arxiv.1111.1111	text	January 2011
Unusual temperature dependence of the spectral weight near the Fermi level of NdNiO3 thin films Schwier, E. F.; Scherwitzl, R.; Vydrova, Z. arXiv https://doi.org/10.48550/arxiv.1211.4922	text	January 2012
Pseudogap formation above the superconducting dome in iron-pnictides Shimojima, T.; Sonobe, T.; Malaeb, W. arXiv https://doi.org/10.48550/arxiv.1305.3875	text	January 2013
Heterointerface engineered electronic and magnetic phases of NdNiO3 thin films Liu, Jian; Kargarian, Mehdi; Kareev, Mikhail arXiv https://doi.org/10.48550/arxiv.1311.4611	text	January 2013
Intermediate Coupling Model of the Cuprates Das, Tanmoy; Markiewicz, R. S.; Bansil, A. arXiv https://doi.org/10.48550/arxiv.1407.5722	text	January 2014
Tuning the metal-insulator transition in NdNiO3 heterostructures via Fermi surface instability and spin-fluctuations Dhaka, R. S.; Das, Tanmoy; Plumb, N. C. arXiv https://doi.org/10.48550/arxiv.1505.04510	text	January 2015
Change of carrier density at the pseudogap critical point of a cuprate superconductor Badoux, S.; Tabis, W.; Laliberté, F. arXiv https://doi.org/10.48550/arxiv.1511.08162	text	January 2015
Bond disproportionation and dynamical charge fluctuations in the perovskite rare earth nickelates Green, Robert J.; Haverkort, Maurits W.; Sawatzky, George A. arXiv https://doi.org/10.48550/arxiv.1608.01645	text	January 2016
Mott Transition and Magnetism in Rare Earth Nickelates and its Fingerprint on the X-ray Scattering Haule, Kristjan; Pascut, Gheorghe L. arXiv https://doi.org/10.48550/arxiv.1703.08196	text	January 2017
Epitaxial strain modulated electronic properties of interface controlled nickelate superlattice Middey, S.; Meyers, D.; Ojha, Shashank Kumar arXiv https://doi.org/10.48550/arxiv.1807.00449	text	January 2018
Evolution of the Hall Coefficient and the Peculiar Electronic Structure of the Cuprate Superconductors Ando, Yoichi; Kurita, Y.; Komiya, Seiki arXiv https://doi.org/10.48550/arxiv.cond-mat/0401034	text	January 2004
Spin and charge ordering in self-doped Mott insulators Mizokawa, T.; Khomskii, D. I.; Sawatzky, G. A. arXiv https://doi.org/10.48550/arxiv.cond-mat/9908016	text	January 1999

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Mass divergence type metal-insulator transition in charge transfer rare-earth nickelates Santhosh Kumar, K.; Phanindra, E. V.; Rana, D. S. Physical Review B, Vol. 100, Issue 12 https://doi.org/10.1103/physrevb.100.125127	journal	September 2019
Conductivity noise across temperature driven transitions of rare-earth nickelate heterostructures Daptary, Gopi Nath; Kumar, Siddharth; Kareev, M. arXiv https://doi.org/10.48550/arxiv.1908.06413	text	January 2019