Suppression of ferromagnetic spin fluctuations in the filled skutterudite superconductor SrOs4As12 revealed by As75 NMR-NQR measurements

Ding, Q. -P.; Nishine, K.; Kawamura, Y.; Hayashi, J.; Sekine, C.; Furukawa, Y.

doi:10.1103/PhysRevB.100.054516

Title: Suppression of ferromagnetic spin fluctuations in the filled skutterudite superconductor ${SrOs}_{4} {As}_{12}$ revealed by ${}^{75}{As}$ NMR-NQR measurements

Journal Article · Mon Aug 26 00:00:00 EDT 2019 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.100.054516· OSTI ID:1560336

Ding, Q. -P. ^[1]; Nishine, K. ^[2]; Kawamura, Y. ^[2]; Hayashi, J. ^[2]; Sekine, C. ^[2];

^[1]

Ames Lab. and Iowa State Univ., Ames, IA (United States)
Muroran Inst. of Technology (Japan)

Motivated by the recent observation of ferromagnetic spin correlations in the filled skutterudite SrFe₄As₁₂ [Q.-P. Ding et al., Phys. Rev. B 98, 155149 (2018)], we have performed ⁷⁵As nuclear magnetic resonance (NMR) and nuclear quadrupole resonance (NQR) measurements to investigate the role of magnetic fluctuations in the newly discovered isostructural superconductor SrOs₄As₁₂ with a superconducting transition temperature of T_c ~ 4.8 K. Here, knight shift K determined by the NQR spectrum under a small magnetic field ( ≤ 0.5 T) is nearly independent of temperature, consistent with the temperature dependence of the magnetic susceptibility. The nuclear spin-lattice relaxation rate divided by temperature, 1/T₁T, is nearly independent of temperature above ~ 50 K and increases slightly with decreasing temperature below the temperature. The temperature dependence is reasonably explained by a simple model where a flat band structure with a small ledge near the Fermi energy is assumed. By comparing the present NMR data with those in SrFe₄As₁₂, we found that the values of | K | and 1/T₁T in SrFe₄As₁₂ are smaller than those in SrFe₄As₁₂, indicating no obvious ferromagnetic spin correlations in SrFe₄As₁₂. From the temperature dependence of 1/T₁T in the superconducting state, an s -wave superconductivity is realized.

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Research Organization:: Ames Lab., Ames, IA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-07CH11358; 23340092

OSTI ID:: 1560336

Alternate ID(s):: OSTI ID: 1558827

Report Number(s):: IS-J-10007; PRBMDO; TRN: US2000464

Journal Information:: Physical Review B, Vol. 100, Issue 5; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 2 works

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Title: Suppression of ferromagnetic spin fluctuations in the filled skutterudite superconductor ${SrOs}_{4} {As}_{12}$ revealed by ${}^{75}{As}$ NMR-NQR measurements