Emergent magnetism at the 3d-5d interface: SrMnO3/SrIrO3

Bhowal, Sayantika; Satpathy, Sashi

doi:10.1063/1.5050724

Title: Emergent magnetism at the 3d-5d interface: SrMnO3/SrIrO3

Journal Article · Thu Aug 16 00:00:00 EDT 2018 · AIP Conference Proceedings

DOI:https://doi.org/10.1063/1.5050724· OSTI ID:1544227

Bhowal, Sayantika ^[1]; Satpathy, Sashi ^[1]

Univ. of Missouri, Columbia, MO (United States). Dept. of Physics

Recent experiments have found new magnetic behaviors, which are different from the parent bulk materials, at the interfaces between 3d and 5d oxides such as SrMnO₃ (SMO) and SrIrO₃ (SIO). The system is of considerable interest due to the strong spin-orbit coupling in the 5d materials on one hand and the double exchange physics in SMO on the other, which belongs to the class of the colossal magnetoresistive (CMR) manganites. In order to gain insight into the physics of the system, we have performed density-functional studies on a selected interface structure, viz., the (SMO)₁(SIO)₁ superlattice, which has been experimentally grown and studied. Our density-functional results show that the interfacial magnetism is controlled by a net charge transfer at the interface from the SIO to the SMO side, turning both of them into ferromagnetic metal from the original antiferromagnetic insulating state in the bulk. The transferred electrons to the SMO side make it ferromagnetic through the Anderson-Hasegawa double exchange interaction, while the SIO part becomes ferromagnetic due to the doping of the half-filled Mott-Hubbard insulator as suggested by the Nagaoka Theorem. Our results are discussed in the context of the experiments for the same structure.

View Accepted Manuscript (DOE)

Cite

Export

Save

Research Organization:: Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). National Energy Research Scientific Computing Center (NERSC)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: FG02-00ER45818

OSTI ID:: 1544227

Journal Information:: AIP Conference Proceedings, Vol. none, Issue none

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

Citation Metrics:

Cited by: 5 works

Citation information provided by
Web of Science

References (27)

Generalized Gradient Approximation Made Simple Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868 https://doi.org/10.1103/PhysRevLett.77.3865	journal	October 1996
Magnetic effects at the interface between non-magnetic oxides Brinkman, A.; Huijben, M.; van Zalk, M. Nature Materials, Vol. 6, Issue 7, p. 493-496 https://doi.org/10.1038/nmat1931	journal	June 2007
High-pressure synthesis of orthorhombic SrIrO3 perovskite and its positive magnetoresistance Zhao, J. G.; Yang, L. X.; Yu, Y. Journal of Applied Physics, Vol. 103, Issue 10 https://doi.org/10.1063/1.2908879	journal	May 2008
Projector augmented-wave method Blöchl, P. E. Physical Review B, Vol. 50, Issue 24, p. 17953-17979 https://doi.org/10.1103/PhysRevB.50.17953	journal	December 1994
Interplay between spin-orbit coupling and Hubbard interaction in SrIrO $_{3}$ and related $Pbnm$ perovskite oxides Zeb, M. Ahsan; Kee, Hae-Young Physical Review B, Vol. 86, Issue 8 https://doi.org/10.1103/PhysRevB.86.085149	journal	August 2012
Simultaneous metal-insulator and antiferromagnetic transitions in orthorhombic perovskite iridate $S r_{0.94} I r_{0.78} O_{2.68}$ single crystals Zheng, H.; Terzic, J.; Ye, Feng Physical Review B, Vol. 93, Issue 23 https://doi.org/10.1103/PhysRevB.93.235157	journal	June 2016
Ferromagnetism in a Narrow, Almost Half-Filled $s$ Band Nagaoka, Yosuke Physical Review, Vol. 147, Issue 1 https://doi.org/10.1103/PhysRev.147.392	journal	July 1966
Electron Leakage and Double-Exchange Ferromagnetism at the Interface between a Metal and an Antiferromagnetic Insulator: ${CaRuO}_{3} / {CaMnO}_{3}$ Nanda, B. R. K.; Satpathy, S.; Springborg, M. S. Physical Review Letters, Vol. 98, Issue 21 https://doi.org/10.1103/PhysRevLett.98.216804	journal	May 2007
Metal-insulator transitions Imada, Masatoshi; Fujimori, Atsushi; Tokura, Yoshinori Reviews of Modern Physics, Vol. 70, Issue 4, p. 1039-1263 https://doi.org/10.1103/RevModPhys.70.1039	journal	October 1998
Engineering a Spin-Orbital Magnetic Insulator by Tailoring Superlattices Matsuno, J.; Ihara, K.; Yamamura, S. Physical Review Letters, Vol. 114, Issue 24 https://doi.org/10.1103/PhysRevLett.114.247209	journal	June 2015
Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set Kresse, G.; Furthmüller, J. Physical Review B, Vol. 54, Issue 16, p. 11169-11186 https://doi.org/10.1103/PhysRevB.54.11169	journal	October 1996
From ultrasoft pseudopotentials to the projector augmented-wave method Kresse, G.; Joubert, D. Physical Review B, Vol. 59, Issue 3, p. 1758-1775 https://doi.org/10.1103/PhysRevB.59.1758	journal	January 1999
Structure and properties of the high and low pressure forms of SrIrO3 Longo, J. M.; Kafalas, J. A.; Arnott, R. J. Journal of Solid State Chemistry, Vol. 3, Issue 2 https://doi.org/10.1016/0022-4596(71)90022-3	journal	May 1971
Band theory and Mott insulators: Hubbard U instead of Stoner I Anisimov, Vladimir I.; Zaanen, Jan; Andersen, Ole K. Physical Review B, Vol. 44, Issue 3, p. 943-954 https://doi.org/10.1103/PhysRevB.44.943	journal	July 1991
The physics of manganites: Structure and transport Salamon, Myron B.; Jaime, Marcelo Reviews of Modern Physics, Vol. 73, Issue 3 https://doi.org/10.1103/RevModPhys.73.583	journal	August 2001
Electronic and Magnetic Structure under Lattice Distortion in SrIrO ₃ /SrTiO ₃ Superlattice: A First-Principles Study Fan, Wei; Yunoki, Seiji Journal of Physics: Conference Series, Vol. 592 https://doi.org/10.1088/1742-6596/592/1/012139	journal	March 2015
Effects of Double Exchange in Magnetic Crystals de Gennes, P. -G. Physical Review, Vol. 118, Issue 1 https://doi.org/10.1103/PhysRev.118.141	journal	April 1960
A high-mobility electron gas at the LaAlO3/SrTiO3 heterointerface Ohtomo, A.; Hwang, H. Y. Nature, Vol. 427, Issue 6973 https://doi.org/10.1038/nature02308	journal	January 2004
Magnetic Structure of the Cubic Perovskite Type SrMnO ₃ Takeda, Takayoshi; Ōhara, Sōji Journal of the Physical Society of Japan, Vol. 37, Issue 1 https://doi.org/10.1143/JPSJ.37.275	journal	July 1974
Ab initiomolecular dynamics for liquid metals Kresse, G.; Hafner, J. Physical Review B, Vol. 47, Issue 1, p. 558-561 https://doi.org/10.1103/PhysRevB.47.558	journal	January 1993
Mott metal-insulator transition in the doped Hubbard-Holstein model Kurdestany, Jamshid Moradi; Satpathy, S. Physical Review B, Vol. 96, Issue 8 https://doi.org/10.1103/PhysRevB.96.085132	journal	August 2017
The Challenge of Unconventional Superconductivity Norman, M. R. Science, Vol. 332, Issue 6026 https://doi.org/10.1126/science.1200181	journal	April 2011
Charge Transfer in Iridate-Manganite Superlattices Okamoto, Satoshi; Nichols, John; Sohn, Changhee Nano Letters, Vol. 17, Issue 4 https://doi.org/10.1021/acs.nanolett.6b04107	journal	March 2017
Emerging magnetism and anomalous Hall effect in iridate–manganite heterostructures Nichols, John; Gao, Xiang; Lee, Shinbuhm Nature Communications, Vol. 7, Issue 1 https://doi.org/10.1038/ncomms12721	journal	September 2016
Gapless Spin Liquids on the Three-Dimensional Hyperkagome Lattice of ${Na}_{4} {Ir}_{3} O_{8}$ Lawler, Michael J.; Paramekanti, Arun; Kim, Yong Baek Physical Review Letters, Vol. 101, Issue 19 https://doi.org/10.1103/PhysRevLett.101.197202	journal	November 2008
Multiferroic and magnetoelectric materials Eerenstein, W.; Mathur, N. D.; Scott, J. F. Nature, Vol. 442, Issue 7104 https://doi.org/10.1038/nature05023	journal	August 2006
Origin of the Two-Dimensional Electron Gas Carrier Density at the ${LaAlO}_{3}$ on ${SrTiO}_{3}$ Interface Popović, Zoran S.; Satpathy, Sashi; Martin, Richard M. Physical Review Letters, Vol. 101, Issue 25, Article No. 256801 https://doi.org/10.1103/PhysRevLett.101.256801	journal	December 2008

Cited By (2)

Electric field tuning of the anomalous Hall effect at oxide interfaces Bhowal, Sayantika; Satpathy, Sashi npj Computational Materials, Vol. 5, Issue 1 https://doi.org/10.1038/s41524-019-0198-8	journal	May 2019
Electric field tuning of the anomalous Hall effect at oxide interfaces Bhowal, Sayantika; Satpathy, S. arXiv https://doi.org/10.48550/arxiv.1812.08950	preprint	January 2018

Similar Records

Electronic structure and anomalous Hall effect in the ferromagnetic 3d-5d superlattice SrMnO3/SrIrO3

Journal Article · Tue Jun 25 00:00:00 EDT 2019 · Physical Review B · OSTI ID:1544227

Bhowal, Sayantika; Satpathy, S.

Escalated Phase Separation Driven Enhanced Magnetoresistance in Manganite/Iridate Epitaxial Heterostructures

Journal Article · Wed Oct 25 00:00:00 EDT 2023 · Advanced Physics Research · OSTI ID:1544227

Roy, Pinku; Zhang, Di; Kunwar, Sundar; +4 more

Role of Structurally and Magnetically Modified Nanoclusters in Colossal Magnetoresistance

Journal Article · Tue Dec 27 00:00:00 EST 2011 · Proceedings of the National Academy of Sciences of the United States of America · OSTI ID:1544227

Tao, J; Niebieskikwiat, D; Jie, Q; +3 more

Related Subjects

71 CLASSICAL AND QUANTUM MECHANICS
GENERAL PHYSICS

Title: Emergent magnetism at the 3d-5d interface: SrMnO3/SrIrO3

Citation Formats

References (27)

Cited By (2)

Similar Records

Related Subjects