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Antiferromagnetic ordering and dipolar interactions of YbAlO3

Journal Article · · Physical Review B
Here, we report low-temperature magnetic properties of the rare-earth perovskite material YbAlO3 . Results of elastic and inelastic neutron scattering experiment, magnetization measurements along with the crystalline electrical field (CEF) calculations, indicate that the ground state of Yb moments is a strongly anisotropic Kramers doublet, and the moments are confined in the ab plane, pointing at an angle of φ=±23.5° to the $$a$$ axis. With temperature decreasing below TN=0.88 K, Yb moments order into the coplanar but noncollinear antiferromagnetic (AFM) structure $AxGy$, where the moments are pointed along their easy axes. In addition, we highlight the importance of the dipole-dipole interaction, which selects the type of magnetic ordering and may be crucial for understanding magnetic properties of other rare-earth orthorhombic perovskites. Further analysis of the broad diffuse neutron scattering shows that one-dimensional interaction along the c axis is dominant and implies YbAlO3 as a new member of one-dimensional quantum magnets.
Research Organization:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
International Max Planck Research School for Chemistry and Physics of Quantum Materials (IMPRS-CPQM); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; Ukrainian Ministry of Education and Sciences
Grant/Contract Number:
AC05-00OR22725
OSTI ID:
1542224
Alternate ID(s):
OSTI ID: 1511765
Journal Information:
Physical Review B, Journal Name: Physical Review B Journal Issue: 19 Vol. 99; ISSN 2469-9950; ISSN PRBMDO
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

References (33)

Optical investigation of metamagnetic DyAlO3 journal April 1969
Antiferromagnetic ordering in the ytterbium aluminum perovskite YbAlO3 journal March 1981
Neutron diffraction study of weak antiferromagnetism in ytterbium orthoferrite journal August 1983
Theory of spin reorientation in rare-earth orthochromites and orthoferrites journal January 1974
Mantid—Data analysis and visualization package for neutron scattering and μ SR experiments
  • Arnold, O.; Bilheux, J. C.; Borreguero, J. M.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 764 https://doi.org/10.1016/j.nima.2014.07.029
journal November 2014
Laser-induced ultrafast spin reorientation in the antiferromagnet TmFeO3 journal June 2004
Multiferroics: a magnetic twist for ferroelectricity journal January 2007
Fractional spinon excitations in the quantum Heisenberg antiferromagnetic chain journal June 2013
Tomonaga–Luttinger liquid behavior and spinon confinement in YbAlO3 journal February 2019
Anisotropic magnetic entropy change in RFeO3 single crystals(R = Tb, Tm, or Y) journal January 2016
Structures et propriétés magnétiques des orthocobaltites de terres rares TCoO3 journal January 1970
Review of Recent Work on the Magnetic and Spectroscopic Properties of the Rare‐Earth Orthoferrites journal March 1969
The new cold neutron chopper spectrometer at the Spallation Neutron Source: Design and performance journal August 2011
The magnetic structures and transitions of a potential multiferroic orthoferrite ErFeO 3 journal April 2015
The cold neutron chopper spectrometer at the Spallation Neutron Source—A review of the first 8 years of operation journal September 2016
Spin-reorientation transitions in rare-earth magnets journal July 1976
Spin-liquid polymorphism in a correlated electron system on the threshold of superconductivity journal August 2015
Matrix Elements and Operator Equivalents Connected with the Magnetic Properties of Rare Earth Ions journal March 1952
Thermal changes of the crystal structure and the influence of thermo-chemical annealing on the optical properties of YbAlO 3 crystals journal January 2010
New field-driven spin reorientations in YbFeO 3 at 4.2 K journal February 1993
Magnetic excitations in the longitudinally amplitude modulated magnetic structure of PrNi 2 Si 2 journal October 2011
Investigation of Magnetic Interactions in TbAl O 3 by Optical Spectroscopy journal July 1968
Neutron-scattering studies of spin waves in rare-earth orthoferrites journal September 1974
Measurements of spin reorientation in YbFeO 3 and comparison with modified mean-field theory journal November 2005
Magnetic Symmetry of Rare-Earth Orthochromites and Orthoferrites journal December 1973
Inelastic neutron scattering studies of YFeO 3 journal January 2014
Magnetic ground state of the Ising-like antiferromagnet DyScO 3 journal October 2017
Decoupled spin dynamics in the rare-earth orthoferrite YbFeO 3 : Evolution of magnetic excitations through the spin-reorientation transition journal August 2018
Magnetic-Field-Induced Ferroelectric State in DyFeO 3 journal August 2008
Role of traps in photocoloration of Mn:YAlO_3 journal January 2001
Spin-reorientation transitions in rare-earth magnets [Perekhody spinovoi pereorientatsii v redkozemel'nykh magnetikakh] journal January 1976
Spin liquid polymorphism in a correlated electron system on the threshold of superconductivity text January 2015
DAVE: A Comprehensive Software Suite for the Reduction, Visualization, and Analysis of Low Energy Neutron Spectroscopic Data
  • Azuah, Richard Tumanjong; Kneller, Larry R.; Qiu, Yiming
  • Journal of Research of the National Institute of Standards and Technology, Vol. 114, Issue 6 https://doi.org/10.6028/jres.114.025
journal November 2009

Cited By (2)

Field-induced magnetic transition and spin fluctuations in the quantum spin-liquid candidate CsYbSe 2 journal December 2019
Low-temperature spin dynamics in the TmFeO 3 orthoferrite with a non-Kramers ion journal January 2020

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