Frustrated magnetism from local moments in FeSe

Ruiz, Harrison; Wang, Yao; Moritz, Brian; Baum, Andreas; Hackl, Rudi; Devereaux, Thomas P.

doi:10.1103/physrevb.99.125130

Frustrated magnetism from local moments in FeSe

Journal Article · Fri Mar 15 00:00:00 EDT 2019 · Physical Review B

DOI:https://doi.org/10.1103/physrevb.99.125130· OSTI ID:1526705

Ruiz, Harrison ^[1]; Wang, Yao ^[2]; Moritz, Brian ^[3]; Baum, Andreas ^[4]; Hackl, Rudi ^[5]; Devereaux, Thomas P. ^[6]

Stanford Univ., Stanford, CA (United States); Stanford Univ., Menlo Park, CA (United States)
Stanford Univ., Menlo Park, CA (United States); Stanford Univ., Stanford, CA (United States); Harvard Univ., Cambridge, MA (United States)
Stanford Univ., Menlo Park, CA (United States); Univ. of North Dakota, Grand Forks, ND (United States)
Walther Meissner Institut, Garching (Germany); Technische Univ. Munchen, Garching (Germany)
Walther Meissner Institut, Garching (Germany)
Stanford Univ., Menlo Park, CA (United States)

We investigate properties of a spin-1 Heisenberg model with extended and biquadratic interactions, which captures crucial aspects of the low energy physics in FeSe. While we show that the model exhibits a rich phase diagram with four different magnetic ordering tendencies, we identify a parameter regime with strong competition between Néel, staggered dimer, and stripelike magnetic fluctuations, accounting for the physical properties of FeSe. We evaluate the spin and Raman responses using exact diagonalization. Through comparison with experiments we find enhanced magnetic frustration between Néel and collinear stripe ordering tendencies, which increases with increasing temperature. As a result, the explanation of these spectral behaviors with this frustrated spin model supports the idea of local spin interactions in FeSe.

View Accepted Manuscript (DOE)

Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC02-05CH11231; AC02-76SF00515

OSTI ID:: 1526705

Alternate ID(s):: OSTI ID: 1501698
OSTI ID: 1543136

Journal Information:: Physical Review B, Journal Name: Physical Review B Journal Issue: 12 Vol. 99; ISSN 2469-9950; ISSN PRBMDO

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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