Probing molecular bond-length using molecular-frame photoelectron angular distributions

Fukuzawa, Hironobu; Lucchese, Robert R.; Liu, Xiao-Jing; Sakai, Kentaro; Iwayama, Hiroshi; Nagaya, Kiyonobu; Kreidi, Katharina; Schöffler, Markus S.; Harries, James R.; Tamenori, Yusuke; Morishita, Yuichiro; Suzuki, Isao H.; Saito, Norio; Ueda, Kiyoshi

doi:10.1063/1.5091946

Title: Probing molecular bond-length using molecular-frame photoelectron angular distributions

Journal Article · Tue May 07 00:00:00 EDT 2019 · Journal of Chemical Physics

DOI:https://doi.org/10.1063/1.5091946· OSTI ID:1526599

^[1];

^[2]; Liu, Xiao-Jing ^[3]; Sakai, Kentaro ^[1]; Iwayama, Hiroshi ^[4]; Nagaya, Kiyonobu ^[5]; Kreidi, Katharina ^[6]; Schöffler, Markus S. ^[6];

^[7];

^[8]; Morishita, Yuichiro ^[9];

^[10];

^[9];

^[1]

Tohoku Univ., Sendai (Japan)
Tohoku Univ., Sendai (Japan); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Tohoku Univ., Sendai (Japan); ShanghaiTech Univ., Shanghai (China)
Kyoto Univ., Kyoto (Japan); Inst. of Molecular Science, Okazaki (Japan)
Kyoto Univ., Kyoto (Japan)
Goeth-Univ. Frankfurt am Main, Frankfurt (Germany)
Japan Synchrotron Radiation Research Inst., Hyogo (Japan); QST, Hyogo (Japan)
Japan Synchrotron Radiation Research Inst., Hyogo (Japan)
National Metrology Institute of Japan, Tsukuba (Japan)
National Metrology Institute of Japan, Tsukuba (Japan); Inst. of Material Structure Science, Tsukuba (Japan)

The molecular-frame photoelectron angular distributions (MFPADs) in O 1s photoemission from CO₂ molecule were measured. Patterns due to photoelectron diffractions were observed in the MFPADs. The polarization-averaged MFPADs were compared with theoretical calculation and were found to be useful in determining the molecular bond-length, which is a component to determine molecular structures.

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Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences, and Biosciences Division

Grant/Contract Number:: AC02-05CH11231

OSTI ID:: 1526599

Alternate ID(s):: OSTI ID: 1511080

Journal Information:: Journal of Chemical Physics, Vol. 150, Issue 17; ISSN 0021-9606

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 16 works

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A new route for enantio-sensitive structure determination by photoelectron scattering on molecules in the gas phase Fehre, K.; Novikovskiy, N. M.; Grundmann, S. arXiv https://doi.org/10.48550/arxiv.2101.03375	text	January 2021
Probing gaseous molecular structure by molecular-frame photoelectron angular distributions Fukuzawa, Hironobu; Yamada, Syuhei; Sakakibara, Yuta The Journal of Chemical Physics, Vol. 151, Issue 10 https://doi.org/10.1063/1.5115801	journal	September 2019
Improved molecular structure retrieval method for photoelectron holography Yu, Chengjian; Wang, Xu Physical Review A, Vol. 100, Issue 6 https://doi.org/10.1103/physreva.100.063422	journal	December 2019
Photoelectron Diffraction Imaging of a Molecular Breakup Using an X-Ray Free-Electron Laser Kastirke, Gregor; Schöffler, Markus S.; Weller, Miriam Deutsches Elektronen-Synchrotron, DESY, Hamburg https://doi.org/10.3204/pubdb-2020-02563	text	January 2020

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