High-quality mesoporous graphene particles as high-energy and fast-charging anodes for lithium-ion batteries

Mo, Runwei; Li, Fan; Tan, Xinyi; Xu, Pengcheng; Tao, Ran; Shen, Gurong; Lu, Xing; Liu, Fang; Shen, Li; Xu, Bin; Xiao, Qiangfeng; Wang, Xiang; Wang, Chongmin; Li, Jinlai; Wang, Ge; Lu, Yunfeng

doi:10.1038/s41467-019-09274-y

Title: High-quality mesoporous graphene particles as high-energy and fast-charging anodes for lithium-ion batteries

Journal Article · Mon Apr 01 00:00:00 EDT 2019 · Nature Communications

DOI:https://doi.org/10.1038/s41467-019-09274-y· OSTI ID:1518474

Mo, Runwei ^[1]; Li, Fan ^[1]; Tan, Xinyi ^[1]; Xu, Pengcheng ^[1]; Tao, Ran ^[1]; Shen, Gurong ^[1]; Lu, Xing ^[1]; Liu, Fang ^[1]; Shen, Li ^[1]; Xu, Bin ^[2]; Xiao, Qiangfeng ^[3]; Wang, Xiang ^[4];

^[4]; Li, Jinlai ^[5]; Wang, Ge ^[6]; Lu, Yunfeng ^[1]

Univ. of California, Los Angeles, CA (United States)
Jilin Univ., Changchun (China)
General Motors Research and Development Center, Warren, MI (United States)
Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
ENN Group, Hebei (China)
Univ. of Science and Technology Beijing, Beijing (China)

The application of graphene for electrochemical energy storage has received tremendous attention; however, challenges remain in synthesis and other aspects. Here we report the synthesis of high-quality, nitrogen-doped, mesoporous graphene particles through chemical vapor deposition with magnesium-oxide particles as the catalyst and template. Such particles possess excellent structural and electrochemical stability, electronic and ionic conductivity, enabling their use as high-performance anodes with high reversible capacity, outstanding rate performance (e.g., 1,138 mA h g^-1 at 0.2 C or 440 mA h g^-1 at 60 C with a mass loading of 1 mg cm^-2), and excellent cycling stability (e.g., >99% capacity retention for 500 cycles at 2 C with a mass loading of 1 mg cm^-2). Interestingly, thick electrodes could be fabricated with high areal capacity and current density (e.g., 6.1 mA h cm^-2 at 0.9 mA cm^-2), providing an intriguing class of materials for lithium-ion batteries with high energy and power performance.

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Research Organization:: Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC05-76RL01830

OSTI ID:: 1518474

Report Number(s):: PNNL-SA-143544

Journal Information:: Nature Communications, Vol. 10, Issue 1; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 104 works

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