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Challenges and opportunities in attosecond and XFEL science

Journal Article · · Nature Reviews Physics
 [1];  [2];  [3];  [4];  [5];  [6];  [7]
  1. Stockholm Univ., Stockholm (Sweden)
  2. Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany); Hamburg Univ., Hamburg (Germany)
  3. Argonne National Lab and the Univ. of Chicago, Lemont, IL (United States)
  4. Sorbonne Univ., Paris (France)
  5. Weizmann Inst. of Science, Rehovot (Israel)
  6. Univ. of Connecticut, Storrs, CT (United States)
  7. Max Born Institute for Nonlinear Optics and Short Pulse Spectroscopy, Berlin (Germany); Technische Univ. Berlin, Berlin (Germany)
In 2009, the world’s first hard X-FEL brought a ten-billion-fold gain in X-ray peak brightness. This fuelled the avidly pursued, but still elusive, dream of single-shot imaging of non-crystalline samples with near-atomic resolution. The overarching concept of ‘diffract-before-destroy’ imaging is that a powerful burst of ultrafast X-rays can produce a coherent diffraction pattern of a nanoscale object — before the object explodes due to Coulomb repulsion caused by a massively parallel ionization of the atoms in the sample. A collection of snapshots of identical objects in random orientations then provide information from which a 3D structure can be retrieved.
Research Organization:
Argonne National Lab. (ANL), Argonne, IL (United States)
Sponsoring Organization:
USDOE Office of Science (SC)
Grant/Contract Number:
AC02-06CH11357
OSTI ID:
1514996
Journal Information:
Nature Reviews Physics, Journal Name: Nature Reviews Physics Journal Issue: 2 Vol. 1; ISSN 2522-5820
Publisher:
Springer NatureCopyright Statement
Country of Publication:
United States
Language:
English

References (7)

Ultrafast charge migration by electron correlation journal July 1999
Attosecond time–energy structure of X-ray free-electron laser pulses journal March 2018
Synthetic chiral light for efficient control of chiral light–matter interaction journal October 2019
Amplification of intense light fields by nearly free electrons journal April 2018
An electronic time scale in chemistry journal April 2006
Generating Single-Spike Hard X-Ray Pulses with Nonlinear Bunch Compression in Free-Electron Lasers journal October 2017
Attosecond dynamics through a Fano resonance: Monitoring the birth of a photoelectron journal November 2016

Cited By (4)

Symphony on strong field approximation journal October 2019
Probing Electronic Fluxes via Time-Resolved X-Ray Scattering journal January 2020
Symphony on strong field approximation text January 2019
Probing Electronic Fluxes via Time-Resolved X-ray Scattering text January 2019

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