Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

Gold-patched graphene nano-stripes for high-responsivity and ultrafast photodetection from the visible to infrared regime

Journal Article · · Light, Science & Applications
 [1];  [2];  [2];  [2]
  1. Univ. of California, Los Angeles, CA (United States). Electrical Engineering Dept.; Univ. of California, Los Angeles, CA (United States)
  2. Univ. of California, Los Angeles, CA (United States). Electrical Engineering Dept.

Graphene is a very attractive material for broadband photodetection in hyperspectral imaging and sensing systems. However, its potential use has been hindered by tradeoffs between the responsivity, bandwidth, and operation speed of existing graphene photodetectors. Here, we present engineered photoconductive nanostructures based on gold-patched graphene nano-stripes, which enable simultaneous broadband and ultrafast photodetection with high responsivity. These nanostructures merge the advantages of broadband optical absorption, ultrafast photocarrier transport, and carrier multiplication within graphene nano-stripes with the ultrafast transport of photocarriers to gold patches before recombination. Through this approach, high-responsivity operation is realized without the use of bandwidth-limiting and speed-limiting quantum dots, defect states, or tunneling barriers. We demonstrate high-responsivity photodetection from the visible to infrared regime (0.6 A/W at 0.8 μm and 11.5 A/W at 20 μm), with operation speeds exceeding 50 GHz. Our results demonstrate improvement of the response times by more than seven orders of magnitude and an increase in bandwidths of one order of magnitude compared to those of higher-responsivity graphene photodetectors based on quantum dots and tunneling barriers.

Research Organization:
Univ. of California, Los Angeles (United States)
Sponsoring Organization:
USDOE Office of Science (SC)
Grant/Contract Number:
SC0016925
OSTI ID:
1510255
Journal Information:
Light, Science & Applications, Journal Name: Light, Science & Applications Journal Issue: 1 Vol. 7; ISSN 2047-7538
Publisher:
Nature Publishing GroupCopyright Statement
Country of Publication:
United States
Language:
English

References (62)

Infrared Photodetectors Based on CVD-Grown Graphene and PbS Quantum Dots with Ultrahigh Responsivity journal August 2012
Sub-10 nm Graphene Nanoribbon Array Field-Effect Transistors Fabricated by Block Copolymer Lithography journal June 2013
Ultrahigh electron mobility in suspended graphene journal June 2008
Optical spectroscopy of graphene: From the far infrared to the ultraviolet journal August 2012
Enhanced Graphene Photodetector with Fractal Metasurface journal December 2016
Microcavity-Integrated Graphene Photodetector journal May 2012
Graphene-Antenna Sandwich Photodetector journal June 2012
Strong Enhancement of Light–Matter Interaction in Graphene Coupled to a Photonic Crystal Nanocavity journal October 2012
Tunable Graphene–Silicon Heterojunctions for Ultrasensitive Photodetection journal February 2013
Experimental Verification of Carrier Multiplication in Graphene journal August 2014
50 GBit/s Photodetectors Based on Wafer-Scale Graphene for Integrated Silicon Photonic Communication Systems journal August 2014
Integrating an electrically active colloidal quantum dot photodiode with a graphene phototransistor journal June 2016
Strong plasmonic enhancement of photovoltage in graphene journal August 2011
Plasmon resonance enhanced multicolour photodetection by graphene journal September 2011
Light–matter interaction in a microcavity-controlled graphene transistor journal January 2012
Photocurrent in graphene harnessed by tunable intrinsic plasmons journal June 2013
Photodetectors based on graphene, other two-dimensional materials and hybrid systems journal October 2014
Graphene photodetectors with ultra-broadband and high responsivity at room temperature journal March 2014
High-responsivity graphene/silicon-heterostructure waveguide photodetectors journal September 2013
Chip-integrated ultrafast graphene photodetector with high responsivity journal September 2013
Photoexcitation cascade and multiple hot-carrier generation in graphene journal February 2013
Electron mobility calculation for graphene on substrates journal August 2014
Optical antenna enhanced graphene photodetector journal December 2014
Graphene plasmonics text January 2013
CMOS-compatible graphene photodetector covering all optical communication bands text January 2013
Infrared Photodetectors Based on Reduced Graphene Oxide and Graphene Nanoribbons journal July 2011
Oxygen-Assisted Charge Transfer Between ZnO Quantum Dots and Graphene journal March 2013
Surface Plasmon Polariton Graphene Photodetectors journal December 2015
High-Responsivity Mid-Infrared Graphene Detectors with Antenna-Enhanced Photocarrier Generation and Collection journal June 2014
Photocurrent Imaging and Efficient Photon Detection in a Graphene Transistor journal March 2009
Controllable unzipping for intramolecular junctions of graphene nanoribbons and single-walled carbon nanotubes journal January 2013
Broadband high photoresponse from pure monolayer graphene photodetector journal May 2013
Ultrafast collinear scattering and carrier multiplication in graphene journal June 2013
Ultrafast graphene photodetector journal October 2009
Hybrid graphene–quantum dot phototransistors with ultrahigh gain journal May 2012
Graphene photonics and optoelectronics journal August 2010
Graphene photodetectors for high-speed optical communications journal March 2010
Graphene plasmonics journal November 2012
CMOS-compatible graphene photodetector covering all optical communication bands journal September 2013
Enhanced photodetection in graphene-integrated photonic crystal cavity journal December 2013
Role of contacts in graphene transistors: A scanning photocurrent study journal June 2009
Photoexcitation cascade and multiple hot carrier generation in graphene conference May 2013
Ultrahigh-mobility graphene devices from chemical vapor deposition on reusable copper journal July 2015
Intrinsic photocurrent characteristics of graphene photodetectors passivated with Al_2O_3 journal January 2013
Enhanced Graphene Photodetector with Fractal Metasurface conference January 2016
Surface Plasmon Polariton Graphene Photodetectors. text January 2016
Ultrafast collinear scattering and carrier multiplication in graphene. text January 2013
Strong plasmonic enhancement of photovoltage in graphene. text January 2011
Light-matter interaction in a microcavity-controlled graphene transistor. text January 2012
Ultrahigh-mobility graphene devices from chemical vapor deposition on reusable copper text January 2015
Ultrahigh electron mobility in suspended graphene text January 2008
The role of contacts in graphene transistors: A scanning photocurrent study text January 2009
Photocurrent imaging and efficient photon detection in a graphene transistor text January 2009
Ultrafast graphene photodetector text January 2009
Graphene Photonics and Optoelectronics text January 2010
Strong Plasmonic Enhancement of Photovoltage in Graphene text January 2011
Microcavity-integrated graphene photodetector text January 2011
Photo-excitation Cascade and Multiple Carrier Generation in Graphene text January 2012
Enhanced Photodetection in Graphene-Integrated Photonic Crystal Cavity text January 2013
Surface plasmon polariton graphene photodetectors text January 2015
Microcavity-integrated graphene photodetector text January 2012
Light–matter interaction in a microcavity-controlled graphene transistor text January 2012

Cited By (24)

A Review on the Development of Tunable Graphene Nanoantennas for Terahertz Optoelectronic and Plasmonic Applications journal March 2020
Unified benchmarking and characterization protocol for nanomaterial-based heterogeneous photodetector technologies preprint January 2020
Laser Fabrication of Graphene‐Based Flexible Electronics journal August 2019
Laser Programmable Patterning of RGO/GO Janus Paper for Multiresponsive Actuators journal August 2019
Engineering Optical Absorption in Graphene and Other 2D Materials: Advances and Applications journal July 2019
Polariton Photonics Using Structured Metals and 2D Materials journal October 2019
Graphene as a Transparent and Conductive Electrode for Organic Optoelectronic Devices journal June 2019
Mixing Properties of Room Temperature Patch‐Antenna Receivers in a Mid‐Infrared (λ ≈ 9 µm) Heterodyne System journal December 2019
Fabrication of highly stable CdS/g-C3N4 composite for enhanced photocatalytic degradation of RhB and reduction of CO2 journal November 2019
Trap engineering in solution processed PbSe quantum dots for high-speed MID-infrared photodetectors journal January 2019
Hybrid plasmonic gold-nanorod–platinum short-wave infrared photodetectors with fast response journal January 2019
Synthesis of bismuth sulfide nanobelts for high performance broadband photodetectors journal January 2020
High responsivity graphene photodetectors from visible to near-infrared by photogating effect journal November 2018
Two-dimensional infrared and terahertz detectors: Outlook and status journal June 2019
Illumination study of a quantum MIM diode for the mid-infrared journal August 2019
Graphene-based polarization-sensitive longwave infrared photodetector journal August 2019
Panchromatic organic photodetectors with SubPc as a non-fullerene acceptor journal September 2019
In2S3 Quantum Dots: Preparation, Properties and Optoelectronic Application journal May 2019
Graphene-based materials in the infrared and terahertz detector families: a tutorial journal January 2019
Ultra-compact integrated graphene plasmonic photodetector with bandwidth above 110 GHz journal February 2020
Theoretical Study of Plasmonically Induced Transparency Effect in Arrays of Graphene-Based Double Disk Resonators journal March 2019
A Grain Boundary Regulates the Friction Behaviors between Graphene and a Gold Substrate journal August 2019
Electronic and Thermal Properties of Graphene and Recent Advances in Graphene Based Electronics Applications journal March 2019
Two-Dimensional Hybrid Composites of SnS2 Nanosheets Array Film with Graphene for Enhanced Photoelectric Performance journal August 2019

Similar Records

Metallo-graphene nanocomposites and methods for using metallo-graphene nanocomposites for electromagnetic energy conversion
Patent · Tue Sep 27 00:00:00 EDT 2022 · OSTI ID:1925148

Enhanced photoresponsivity in graphene-silicon slow-light photonic crystal waveguides
Journal Article · Mon Mar 14 00:00:00 EDT 2016 · Applied Physics Letters · OSTI ID:22591431

High-Responsivity Graphene–Boron Nitride Photodetector and Autocorrelator in a Silicon Photonic Integrated Circuit
Journal Article · Tue Sep 15 00:00:00 EDT 2015 · Nano Letters · OSTI ID:1370894

Related Subjects