Modeling, Simulation, and Implementation of Solar-Driven Water-Splitting Devices

Xiang, Chengxiang; Weber, Adam Z.; Ardo, Shane; Berger, Alan; Chen, YiKai; Coridan, Robert; Fountaine, Katherine T.; Haussener, Sophia; Hu, Shu; Liu, Rui; Lewis, Nathan S.; Modestino, Miguel A.; Shaner, Matthew M.; Singh, Meenesh R.; Stevens, John C.; Sun, Ke; Walczak, Karl

doi:10.1002/anie.201510463

Modeling, Simulation, and Implementation of Solar-Driven Water-Splitting Devices

Journal Article · Thu Oct 06 00:00:00 EDT 2016 · Angewandte Chemie (International Edition)

DOI:https://doi.org/10.1002/anie.201510463· OSTI ID:1506250

Xiang, Chengxiang ^[1]; ^[2]; Ardo, Shane ^[3]; Berger, Alan ^[4]; Chen, YiKai ^[1]; Coridan, Robert ^[5]; Fountaine, Katherine T. ^[6]; Haussener, Sophia ^[7]; Hu, Shu ^[1]; Liu, Rui ^[1]; Lewis, Nathan S. ^[8]; Modestino, Miguel A. ^[9]; Shaner, Matthew M. ^[8]; Singh, Meenesh R. ^[2]; Stevens, John C. ^[2]; Sun, Ke ^[8]; Walczak, Karl ^[2]

California Inst. of Technology, Pasadena CA (United States). Joint Center for Artificial Photosynthesis
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Joint Center for Artificial Photosynthesis
Univ. of California, Irvine, CA (United States). Dept. of Chemistry, and Dept. of Chemical Engineering and Materials Science
Air Products and Chemicals, Inc., Allentown, PA (United States)
Univ. of Arkansas, Fayetteville, AR (United States). Dept. of Chemistry and Biochemistry
Northrop Grumman Aerospace Systems, Redondo Beach, CA (United States). Nanophotonics and Plasmonics Lab.
Ecole Polytechnique Federale Lausanne (EPFL), Lausanne (Switzlerland). Lab. of Renewable Energy Science and Engineering
California Inst. of Technology, Pasadena CA (United States). Joint Center for Artificial Photosynthesis, Division of Chemistry and Chemical Engineering
Ecole Polytechnique Federale Lausanne (EPFL), Lausanne (Switzlerland). School of Engineering

An integrated cell for the solar-driven splitting of water consists of multiple functional components and couples various photoelectrochemical (PEC) processes at different length and time scales. The overall solar-to-hydrogen (STH) conversion efficiency of such a system depends on the performance and materials properties of the individual components as well as on the component integration, overall device architecture, and system operating conditions. This Review focuses on the modeling- and simulation-guided development and implementation of solar-driven water-splitting prototypes from a holistic viewpoint that explores the various interplays between the components. The underlying physics and interactions at the cell level is are reviewed and discussed, followed by an overview of the use of the cell model to provide target properties of materials and guide the design of a range of traditional and unique device architectures.

View Accepted Manuscript (DOE)

Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE; USDOE Office of Science (SC)

Grant/Contract Number:: AC02-05CH11231; EE0006963; SC0004993

OSTI ID:: 1506250

Alternate ID(s):: OSTI ID: 1401230

Journal Information:: Angewandte Chemie (International Edition), Journal Name: Angewandte Chemie (International Edition) Journal Issue: 42 Vol. 55; ISSN 1433-7851

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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