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Tunable Infrared Devices via Ferroelectric Domain Reconfiguration

Journal Article · · Advanced Optical Materials
 [1];  [1];  [1];  [1];  [1];  [1];  [2];  [3];  [1];  [1];  [4];  [4];  [4];  [5]
  1. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
  2. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); Carnegie Mellon Univ., Pittsburgh, PA (United States)
  3. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); Missouri Univ. of Science and Technology, Rolla, MO (United States)
  4. Argonne National Lab. (ANL), Argonne, IL (United States)
  5. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); Univ. of Virginia, Charlottesville, VA (United States)
Despite widespread use in sensing, electro–optics, and catalysis, plasmonic elements are typically static in their spectral response. The subwavelength spatial confinement and enhanced electric fields intrinsic to plasmons provide a lever to realize dynamic spectral tunability—and thus multifunctional optical components—as small alterations in their dielectric environment are amplified by these effects. Here, electric–field (DC) control of phonon modes is leveraged in lead zirconate titante (PZT) ferroelectric bilayers to create tunable long–wave infrared (LWIR) plasmonic devices that demonstrate a combination of advantages—speed (>10 kHz), latching, and low–power switching (<1 µJ mm–2)—unavailable together in approaches reported heretofore. Mechanistically, bias–induced domain reconfiguration alters the phonon energies defining PZT's optical permittivity, which determines the gap plasmon formed within the ferroelectric resting between patterned metal contacts. Furthermore the utility of ferroelectrics for tunable plasmonic devices is thus demonstrated while highlighting the promise of leveraging phonons for these purposes.
Research Organization:
Argonne National Lab. (ANL), Argonne, IL (United States)
Sponsoring Organization:
USDOE; USDOE National Nuclear Security Administration (NNSA); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
Grant/Contract Number:
AC02-06CH11357; NA0003525
OSTI ID:
1505602
Alternate ID(s):
OSTI ID: 1480873
Journal Information:
Advanced Optical Materials, Journal Name: Advanced Optical Materials Journal Issue: 24 Vol. 6; ISSN 2195-1071
Publisher:
WileyCopyright Statement
Country of Publication:
United States
Language:
English

References (69)

Chemically Homogeneous Complex Oxide Thin Films Via Improved Substrate Metallization journal March 2012
Epitaxial PbZr x Ti 1− x O 3 Ferroelectric Bilayers with Giant Electromechanical Properties journal April 2015
Reversible Polarization Rotation in Epitaxial Ferroelectric Bilayers journal July 2016
Strip and gap plasmon polariton optical resonators journal January 2008
Bio-Inspired Evaporation Through Plasmonic Film of Nanoparticles at the Air-Water Interface journal May 2014
Determination of residual stress in PZT films produced by laser ablation with X-ray diffraction and Raman spectroscopy journal January 2010
Principles of Nano-Optics book January 2012
Principles of Nano-Optics book January 2006
Electronically Tunable Perfect Absorption in Graphene journal January 2018
Proton and carbon-13 NMR investigations of lead zirconate titanate (Pb(Zr,Ti)O3) thin-film precursor solutions journal April 1993
An Optofluidic Nanoplasmonic Biosensor for Direct Detection of Live Viruses from Biological Media journal December 2010
Reconfigurable Photonic Metamaterials journal May 2011
Radiation Engineering of Optical Antennas for Maximum Field Enhancement journal July 2011
Broad Electrical Tuning of Graphene-Loaded Plasmonic Antennas journal February 2013
Using Low-Loss Phase-Change Materials for Mid-Infrared Antenna Resonance Tuning journal July 2013
Wide Wavelength Tuning of Optical Antennas on Graphene with Nanosecond Response Time journal December 2013
Active Tunable Absorption Enhancement with Graphene Nanodisk Arrays journal December 2013
High-Responsivity Mid-Infrared Graphene Detectors with Antenna-Enhanced Photocarrier Generation and Collection journal June 2014
Electrically Tunable Metasurface Perfect Absorbers for Ultrathin Mid-Infrared Optical Modulators journal October 2014
Room-Temperature Voltage Tunable Phonon Thermal Conductivity via Reconfigurable Interfaces in Ferroelectric Thin Films journal February 2015
Gated Tunability and Hybridization of Localized Plasmons in Nanostructured Graphene journal February 2013
Photocurrent in graphene harnessed by tunable intrinsic plasmons journal June 2013
Strong coupling in the sub-wavelength limit using metamaterial nanocavities journal November 2013
Plasmonics for extreme light concentration and manipulation journal February 2010
Reversible optical switching of highly confined phonon–polaritons with an ultrathin phase-change material journal May 2016
Polaritons in layered two-dimensional materials journal November 2016
An electromechanically reconfigurable plasmonic metamaterial operating in the near-infrared journal March 2013
The case for plasmon-derived hot carrier devices journal January 2015
Colouring at the nanoscale journal January 2015
Reconfigurable nanomechanical photonic metamaterials journal January 2016
Atomic-scale photonic hybrids for mid-infrared and terahertz nanophotonics journal January 2016
Zero-power infrared digitizers based on plasmonically enhanced micromechanical photoswitches journal September 2017
Heat-assisted magnetic recording by a near-field transducer with efficient optical energy transfer journal March 2009
Electrical detection of confined gap plasmons in metal–insulator–metal waveguides journal April 2009
Optically reconfigurable metasurfaces and photonic devices based on phase change materials journal December 2015
Active tuning of surface phonon polariton resonances via carrier photoinjection journal December 2017
Maskless Plasmonic Lithography at 22 nm Resolution journal November 2011
Electrically Tunable Epsilon-Near-Zero (ENZ) Metafilm Absorbers journal November 2015
Recent progress in SERS biosensing journal January 2011
Electro‐optical characterization of Pb(Zr,Ti)O 3 thin films by waveguide refractometry journal October 1993
Determination of residual stresses in Pb(Zr0.53Ti0.47)O3 thin films with Raman spectroscopy journal December 2001
Domain distributions in tetragonal Pb(Zr,Ti)O3 thin films probed by polarized Raman spectroscopy journal December 2005
Large electro-optic effect in single-crystal Pb(Zr,Ti)O3 (001) measured by spectroscopic ellipsometry journal November 2008
Influence of poling on far-infrared response of lead zirconate titanate ceramics journal October 2009
Reconfigurable gradient index using VO 2 memory metamaterials journal July 2011
Ultrafast switching of ferroelastic nanodomains in bilayered ferroelectric thin films journal October 2011
Ultra-thin perfect absorber employing a tunable phase change material journal November 2012
Tunable metamaterials based on voltage controlled strong coupling journal December 2013
Optical and electro-optic anisotropy of epitaxial PZT thin films journal July 2015
Nano-optomechanical nonlinear dielectric metamaterials journal November 2015
Enhanced infrared detectors using resonant structures combined with thin type-II superlattice absorbers journal December 2016
Young's Modulus of Soft PZT from Partial Unloading Tests journal January 2002
Processing, Structure, Properties, and Applications of PZT Thin Films journal December 2007
Determination of the Young's modulus of pulsed laser deposited epitaxial PZT thin films journal June 2011
Polar lattice vibrations and phase transition dynamics in Pb(Zr 1 – x Ti x )O 3 journal November 2011
Compositional behavior of Raman-active phonons in Pb ( Z r 1 − x T i x ) O 3 ceramics journal January 2015
First-Principles Study of the Electro-Optic Effect in Ferroelectric Oxides journal October 2004
Longitudinal Electrooptic Effects and Photosensitivities of Lead Zirconate Titanate Thin Films journal November 1989
Angularly and Spectrally Resolved Light Scattering from Lead Zirconate Titanate Thin Films journal August 1995
Ferroelectric Ceramics: History and Technology journal April 1999
The Road Ahead for Metamaterials journal April 2010
Applying plasmonics to a sustainable future journal June 2017
Geometries and materials for subwavelength surface plasmon modes journal January 2004
Solving dielectric and plasmonic waveguide dispersion relations on a pocket calculator journal January 2009
Designing graphene absorption in a multispectral plasmon-enhanced infrared detector journal January 2017
Reconfigurable Photonic Metamaterials conference January 2011
Low-loss, infrared and terahertz nanophotonics using surface phonon polaritons journal January 2015
Reconfigurable Gradient Index using VO2 Memory Metamaterials text January 2011
Electronically Tunable Perfect Absorption in Graphene text January 2017

Cited By (3)

Controlling the Infrared Dielectric Function through Atomic-Scale Heterostructures journal June 2019
Internal‐Field‐Enhanced Charge Separation in a Single‐Domain Ferroelectric PbTiO 3 Photocatalyst journal November 2019
Simulation of tuning graphene plasmonic behaviors by ferroelectric domains for self-driven infrared photodetector applications journal January 2019

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