Tunable Infrared Devices via Ferroelectric Domain Reconfiguration

Beechem, Thomas E.; Goldflam, Michael D.; Sinclair, Michael B.; Peters, David W.; McDonald, Anthony E.; Paisley, Elizabeth A.; Kitahara, Andrew R.; Drury, Daniel E.; Burckel, D. Bruce; Finnegan, Patrick S.; Kim, Jong -Woo; Choi, Yongseong; Ryan, Philip J.; Ihlefeld, Jon F.

doi:10.1002/adom.201800862

Title: Tunable Infrared Devices via Ferroelectric Domain Reconfiguration

Journal Article · Sun Nov 04 00:00:00 EDT 2018 · Advanced Optical Materials

DOI:https://doi.org/10.1002/adom.201800862· OSTI ID:1505602

^[1]; Goldflam, Michael D. ^[1]; Sinclair, Michael B. ^[1]; Peters, David W. ^[1]; McDonald, Anthony E. ^[1]; Paisley, Elizabeth A. ^[1]; Kitahara, Andrew R. ^[2]; Drury, Daniel E. ^[3]; Burckel, D. Bruce ^[1]; Finnegan, Patrick S. ^[1]; Kim, Jong -Woo ^[4]; Choi, Yongseong ^[4]; Ryan, Philip J. ^[4]; Ihlefeld, Jon F. ^[5]

Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); Carnegie Mellon Univ., Pittsburgh, PA (United States)
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); Missouri Univ. of Science and Technology, Rolla, MO (United States)
Argonne National Lab. (ANL), Argonne, IL (United States)
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); Univ. of Virginia, Charlottesville, VA (United States)

Abstract Despite widespread use in sensing, electro‐optics, and catalysis, plasmonic elements are typically static in their spectral response. The subwavelength spatial confinement and enhanced electric fields intrinsic to plasmons provide a lever to realize dynamic spectral tunability—and thus multifunctional optical components—as small alterations in their dielectric environment are amplified by these effects. Here, electric‐field (DC) control of phonon modes is leveraged in lead zirconate titante (PZT) ferroelectric bilayers to create tunable long‐wave infrared (LWIR) plasmonic devices that demonstrate a combination of advantages—speed (>10 kHz), latching, and low‐power switching (<1 µJ mm ⁻² )—unavailable together in approaches reported heretofore. Mechanistically, bias‐induced domain reconfiguration alters the phonon energies defining PZT's optical permittivity, which determines the gap plasmon formed within the ferroelectric resting between patterned metal contacts. The utility of ferroelectrics for tunable plasmonic devices is thus demonstrated while highlighting the promise of leveraging phonons for these purposes.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE National Nuclear Security Administration (NNSA)

Grant/Contract Number:: AC02-06CH11357; DE‐NA0003525

OSTI ID:: 1505602

Alternate ID(s):: OSTI ID: 1480873

Journal Information:: Advanced Optical Materials, Vol. 6, Issue 24; ISSN 2195-1071

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 13 works

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Title: Tunable Infrared Devices via Ferroelectric Domain Reconfiguration

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