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Title: Gd5Si4-PVDF nanocomposite films and their potential for triboelectric energy harvesting applications

Journal Article · · AIP Advances
DOI:https://doi.org/10.1063/1.5080116· OSTI ID:1503853
 [1];  [2];  [2];  [3];  [4];  [4];  [2]; ORCiD logo [5]
  1. Virginia Commonwealth Univ., Richmond, VA (United States)
  2. Univ. of Bolton (United Kingdom)
  3. Virginia Commonwealth Univ., Richmond, VA (United States); Univ. of Texas, El Paso, TX (United States)
  4. Ames Lab., Ames, IA (United States)
  5. Virginia Commonwealth Univ., Richmond, VA (United States); Iowa State Univ., Ames, IA (United States)

The triboelectric energy generators prepared using the combination of self-polarized, high β-phase nanocomposite films of Gd5Si4-PVDF and polyamide-6 (PA-6) films have generated significantly higher voltage of ~425 V, short-circuit current density of ~30 mA/m2 and a charge density of ~116.7 μC/m2 as compared to corresponding values of ~300 V, 30 mA/m2 and 94.7 μC/m2, respectively for the pristine PVDF-(PA-6) combination. The magnetic measurements of the Gd5Si4-PVDF films display a ferromagnetic behavior as compared to diamagnetic nature of pristine PVDF. The presence of magnetic nanoparticles in the polymeric matrix allows for some control over the microstructural properties during the preparation process. The results open new routes for multiferroic composite films to be suitable for multi-functional magnetic and triboelectric energy harvesting applications.

Research Organization:
Ames Lab., Ames, IA (United States)
Sponsoring Organization:
USDOE
Grant/Contract Number:
1357565; 1610967; 1726617; AC02-07CH11358
OSTI ID:
1503853
Report Number(s):
IS-J-9920
Journal Information:
AIP Advances, Vol. 9, Issue 3; ISSN 2158-3226
Publisher:
American Institute of Physics (AIP)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 5 works
Citation information provided by
Web of Science

References (9)

Multifunctional nanocomposites of poly(vinylidene fluoride) reinforced by carbon nanotubes and magnetite nanoparticles journal January 2015
Self-Powered Nanosensors and Nanosystems journal November 2011
Triboelectric nanogenerators as self-powered active sensors journal January 2015
Flexible triboelectric generator journal March 2012
Enhancement of 𝜷-phase in PVDF films embedded with ferromagnetic Gd 5 Si 4 nanoparticles for piezoelectric energy harvesting journal May 2017
A universal self-charging system driven by random biomechanical energy for sustainable operation of mobile electronics journal December 2015
Nanofibrous membrane constructed wearable triboelectric nanogenerator for high performance biomechanical energy harvesting journal June 2017
High performance triboelectric nanogenerators based on phase-inversion piezoelectric membranes of poly(vinylidene fluoride)-zinc stannate (PVDF-ZnSnO3) and polyamide-6 (PA6) journal December 2016
Enhancing the performance of triboelectric nanogenerator through prior-charge injection and its application on self-powered anticorrosion journal November 2014

Cited By (1)

Magnetocaloric Effect of Micro- and Nanoparticles of Gd5Si4 journal July 2019

Figures / Tables (5)


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