Real-Space Study of Charge and Orbital Ordering in La0.6Sr2.4Mn2O7 Manganite Single Crystal

Zheng, Qiang; Schreiber, Nate; Zheng, Hong; Yan, Jiaqiang; McGuire, Michael A.; Mitchell, J. F.; Chi, Miaofang; Sales, Brian C.

doi:10.1017/S1431927618001022

Title: Real-Space Study of Charge and Orbital Ordering in La_0.6Sr_2.4Mn₂O₇ Manganite Single Crystal

Journal Article · Wed Aug 01 00:00:00 EDT 2018 · Microscopy and Microanalysis

DOI:https://doi.org/10.1017/S1431927618001022· OSTI ID:1495973

Zheng, Qiang ^[1]; Schreiber, Nate ^[2]; Zheng, Hong ^[2]; Yan, Jiaqiang ^[1]; McGuire, Michael A. ^[1]; Mitchell, J. F. ^[2]; Chi, Miaofang ^[1]; Sales, Brian C. ^[1]

Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Argonne National Lab. (ANL), Argonne, IL (United States)

Charge and orbital ordering often occur in strongly correlated materials involving cations with multivalence states. This order is related to various interesting physical phenomena in perovskite-structured and related oxides, such as superconductivity and colossal magnetoresistance [1,2]. The n = 2 Ruddlesden-Popper phase La_2-2xSr_1+2xMn₂O₇ (LSMO), which is comprised of perovskite-like (La, Sr)MnO₃ bilayers separated by a rock-salt-like (La, Sr)O layer along [001], represents one of the most interesting manganites where its charge and orbital ordering can be tuned by varying x. In its phase diagram [3,4], previous studies revealed a narrow region with 0.66 ≤ x ≤ 0.72 that showed no long-range magnetic ordering, while the regions with x below 0.66 and above 0.72 exhibited clear different longrange magnetic ordering behaviors owing to charge/orbital ordering in the lattice.

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Research Organization:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1495973

Journal Information:: Microscopy and Microanalysis, Vol. 24, Issue S1; ISSN 1431-9276

Publisher:: Microscopy Society of America (MSA)Copyright Statement

Country of Publication:: United States

Language:: English

References (5)

Giant magnetoresistance of manganese oxides with a layered perovskite structure Moritomo, Y.; Asamitsu, A.; Kuwahara, H. Nature, Vol. 380, Issue 6570 https://doi.org/10.1038/380141a0	journal	March 1996
Interplay of spin and orbital ordering in the layered colossal magnetoresistance manganite ${La}_{2 - 2 x} {Sr}_{1 + 2 x} {Mn}_{2} O_{7} (0.5 <~ x <~ 1.0)$ Ling, C. D.; Millburn, J. E.; Mitchell, J. F. Physical Review B, Vol. 62, Issue 22 https://doi.org/10.1103/PhysRevB.62.15096	journal	December 2000
Magnetic phase diagram of layered manganites in the highly doped regime Mitchell, J. F.; Ling, C. D.; Millburn, J. E. Journal of Applied Physics, Vol. 89, Issue 11 https://doi.org/10.1063/1.1357135	journal	June 2001
Atomic-resolution imaging of oxidation states in manganites Varela, M.; Oxley, M. P.; Luo, W. Physical Review B, Vol. 79, Issue 8 https://doi.org/10.1103/PhysRevB.79.085117	journal	February 2009
Oxidation state and chemical shift investigation in transition metal oxides by EELS Tan, Haiyan; Verbeeck, Jo; Abakumov, Artem Ultramicroscopy, Vol. 116 https://doi.org/10.1016/j.ultramic.2012.03.002	journal	May 2012

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Title: Real-Space Study of Charge and Orbital Ordering in La0.6Sr2.4Mn2O7 Manganite Single Crystal

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Title: Real-Space Study of Charge and Orbital Ordering in La_0.6Sr_2.4Mn₂O₇ Manganite Single Crystal