Low dimensional metal halide perovskites and hybrids

Zhou, Chenkun; Lin, Haoran; He, Qingquan; Xu, Liangjin; Worku, Michael; Chaaban, Maya; Lee, Sujin; Shi, Xiaoqin; Du, Mao-Hua; Ma, Biwu

doi:10.1016/j.mser.2018.12.001

Title: Low dimensional metal halide perovskites and hybrids

Journal Article · Thu Dec 20 00:00:00 EST 2018 · Materials Science and Engineering. R, Reports

DOI:https://doi.org/10.1016/j.mser.2018.12.001· OSTI ID:1493125

Zhou, Chenkun ^[1];

^[2]; He, Qingquan ^[2]; Xu, Liangjin ^[2]; Worku, Michael ^[3]; Chaaban, Maya ^[2]; Lee, Sujin ^[2]; Shi, Xiaoqin ^[4];

^[5];

^[6]

Florida A&M Univ. and Florida State Univ., Tallahassee, FL (United States). FAMU-FSU College of Engineering, Dept. of Chemical and Biomedical Engineering
Florida State Univ., Tallahassee, FL (United States). Dept. of Chemistry and Biochemistry
Florida State Univ., Tallahassee, FL (United States). Materials Science and Engineering Program
Florida State Univ., Tallahassee, FL (United States). Dept. of Chemistry and Biochemistry; Nanjing Univ. of Science and Technology, Nanjing (China). School of Materials Science and Engineering
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science & Technology Division
Florida A&M Univ. and Florida State Univ., Tallahassee, FL (United States). FAMU-FSU College of Engineering, Dept. of Chemical and Biomedical Engineering; Florida State Univ., Tallahassee, FL (United States). Dept. of Chemistry and Biochemistry; Florida State Univ., Tallahassee, FL (United States). Materials Science and Engineering Program

Organic-inorganic metal halide hybrids are an important class of crystalline materials with exceptional structural and property tunability. Recently metal halide perovskites with ABX₃ structure have been extensively investigated as new generation semiconductors for various optoelectronic devices, including photovoltaic cells, light emitting diodes, photodetectors, and lasers, for their exceptional optical and electronic properties. By controlling the morphological dimensionality, low dimensional metal halide perovskites, including 2D perovskite nanoplatelets, 1D perovskite nanowires, and 0D perovskite quantum dots, have been developed to exhibit distinct properties from their bulk counterparts, due to quantum size effects. Besides ABX₃ perovskites, organic-inorganic metal halide hybrids, containing the same fundamental building block of metal halide octahedra (BX₆), can also be assembled to possess other types of crystallographic structures. Using appropriate organic and inorganic components, low dimensional organic-inorganic metal halide hybrids with 2D, quasi-2D, corrugated-2D, 1D, and 0D structures at the molecular level have been developed and studied. Due to the strong quantum confinement and site isolation, these low dimensional metal halide hybrids at the molecular level exhibit remarkable and unique properties that are significantly different from those of ABX₃ perovskites. In light of the rapid development of low dimensional metal halide perovskites and hybrids, it is indeed timely to review the recent progress in these areas. Also, there is a need to clarify the difference between morphological low dimensional metal halide perovskites and molecular level low dimensional metal halide hybrids, as currently the terminologies of low dimensional perovskites are not appropriately used in many cases. Finally, in this review article, we discuss the synthesis, characterization, application, and computational studies of low dimensional metal halide perovskites and hybrids.

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Research Organization:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1493125

Journal Information:: Materials Science and Engineering. R, Reports, Vol. 137, Issue C; ISSN 0927-796X

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 199 works

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Ion Migration in Organometal Trihalide Perovskite and Its Impact on Photovoltaic Efficiency and Stability Yuan, Yongbo; Huang, Jinsong Accounts of Chemical Research, Vol. 49, Issue 2 https://doi.org/10.1021/acs.accounts.5b00420	journal	January 2016
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