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Interface engineering for a rational design of poison-free bimetallic CO oxidation catalysts

Journal Article · · Nanoscale
DOI:https://doi.org/10.1039/c7nr01382e· OSTI ID:1492966
 [1];  [2];  [3];  [3];  [3];  [1];  [2];  [3]
  1. Korea Advanced Inst. Science and Technology (KAIST), Daejeon (Korea, Republic of). Dept. of Materials Science and Engineering
  2. Univ. of Texas, Austin, TX (United States). Dept. of Chemistry
  3. Changnam National Univ, Daejeon (Korea). Dept. fo Materials Science and Engineering
We use density functional theory calculations of Pt@Cu core@shell nanoparticles (NPs) to design bifunctional poison-free CO oxidation catalysts. By calculating the adsorption chemistry under CO oxidation conditions, we find that the Pt@Cu NPs will be active for CO oxidation with resistance to CO-poisoning. The CO oxidation pathway at the Pt–Cu interface is determined on the Pt NP covered with a full- and partial-shell of Cu. The exposed portion of the Pt core preferentially binds CO and the Cu shell binds O2, supplying oxygen for the reaction. The Pt–Cu interface provides CO-oxidation sites that are not poisoned by either CO or O2. Additional computational screening shows that this separation of reactant binding sites is possible for several other core@shell NPs. Our results indicate that the metal–metal interface within a single NP can be optimized for design of bifunctional catalytic systems with improved performance.
Research Organization:
Lawrence Berkeley National Laboratory-National Energy Research Scientific Computing Center
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
DOE Contract Number:
SC0012704
OSTI ID:
1492966
Journal Information:
Nanoscale, Journal Name: Nanoscale Journal Issue: 16 Vol. 9; ISSN NANOHL; ISSN 2040-3364
Country of Publication:
United States
Language:
English

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  • Nilekar, Anand Udaykumar; Alayoglu, Selim; Eichhorn, Bryan
  • Journal of the American Chemical Society, Vol. 132, Issue 21, p. 7418-7428 https://doi.org/10.1021/ja101108w
journal June 2010

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