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Title: Three-stage decoherence dynamics of an electron spin qubit in an optically active quantum dot

Journal Article · · Nature Physics
DOI:https://doi.org/10.1038/nphys3470· OSTI ID:1492646

We report the control of solid-state qubits requires a detailed understanding of the decoherence mechanisms. Despite considerable progress in uncovering the qubit dynamics in strong magnetic fields, decoherence at very low magnetic fields remains puzzling, and the role of quadrupole coupling of nuclear spins is poorly understood. For spin qubits in semiconductor quantum dots, phenomenological models of decoherence include two basic types of spin relaxation: fast dephasing due to static but randomly distributed hyperfine fields (~2 ns) and a much slower process (>1 μs) of irreversible monotonic relaxation due either to nuclear spin co-flips or other complex many-body interaction effects. Here we show that this is an oversimplification; the spin qubit relaxation is determined by three rather than two distinct stages. Finally, the additional stage corresponds to the effect of coherent precession processes that occur in the nuclear spin bath itself, leading to a relatively fast but incomplete non-monotonic relaxation at intermediate timescales (~750 ns).

Research Organization:
Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
Sponsoring Organization:
USDOE Laboratory Directed Research and Development (LDRD) Program
Grant/Contract Number:
89233218CNA000001; AC52-06NA25396
OSTI ID:
1492646
Report Number(s):
LA-UR-15-24203
Journal Information:
Nature Physics, Vol. 11, Issue 12; ISSN 1745-2473
Publisher:
Nature Publishing Group (NPG)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 87 works
Citation information provided by
Web of Science

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Cited By (38)

Generation of Non‐Classical Light Using Semiconductor Quantum Dots journal January 2020
Quadrupolar and anisotropy effects on dephasing in two-electron spin qubits in GaAs journal April 2016
Material platforms for spin-based photonic quantum technologies journal April 2018
A self-sustaining atomic magnetometer with τ−1 averaging property journal June 2016
Magnetic field manipulation of spin current in a single-molecule magnet tunnel junction with two-electron Coulomb interaction journal April 2018
Electrically tunable dynamic nuclear spin polarization in GaAs quantum dots at zero magnetic field journal April 2018
A τ −1 measurement across three orders of magnitude based on an atomic spin precession magnetometer in self-sustaining mode journal May 2019
Environmental noise spectroscopy with qubits subjected to dynamical decoupling journal July 2017
Reviving the precision of multiple entangled probes in an open system by simple π -pulse sequences journal November 2016
Characterization of a quasistatic environment with a qubit journal June 2019
Coherent Optical Control of a Quantum-Dot Spin-Qubit in a Waveguide-Based Spin-Photon Interface journal March 2019
Correlations between optical properties and Voronoi-cell area of quantum dots journal October 2019
Complete state tomography of a quantum dot spin qubit journal January 2020
Vanishing electron g factor and long-lived nuclear spin polarization in weakly strained nanohole-filled GaAs/AlGaAs quantum dots journal April 2016
Hyperfine coupling of hole and nuclear spins in symmetric (111)-grown GaAs quantum dots journal September 2016
Quantum model for mode locking in pulsed semiconductor quantum dots journal December 2016
Cross calibration of deformation potentials and gradient-elastic tensors of GaAs using photoluminescence and nuclear magnetic resonance spectroscopy in GaAs/AlGaAs quantum dot structures journal June 2018
Decay and revival of electron spin polarization in an ensemble of (In,Ga)As quantum dots journal August 2018
Theory of spin inertia in singly charged quantum dots journal September 2018
Magnetic field dependence of the electron spin revival amplitude in periodically pulsed quantum dots journal October 2018
Quantum Effects in Higher-Order Correlators of a Quantum-Dot Spin Qubit journal July 2016
Spectrum of the Nuclear Environment for GaAs Spin Qubits journal April 2017
Phase-Tuned Entangled State Generation between Distant Spin Qubits journal July 2017
Fundamental Limits to Coherent Photon Generation with Solid-State Atomlike Transitions journal October 2019
Depolarization of Electronic Spin Qubits Confined in Semiconductor Quantum Dots journal December 2018
Quantum interface of an electron and a nuclear ensemble journal February 2019
Quantum interface of an electron and a nuclear ensemble. text January 2019
Correlations between optical properties and Voronoi-cell area of quantum dots text January 2019
Phase-Tuned Entangled State Generation between Distant Spin Qubits. text January 2017
Coherent Optical Control of a Quantum-Dot Spin-Qubit in a Waveguide-Based Spin-Photon Interface text January 2019
Phase-tuned entangled state generation between distant spin qubits conference June 2017
Quadrupolar and anisotropy effects on dephasing in two-electron spin qubits in GaAs text January 2016
Quantum model for mode locking in pulsed semiconductor quantum dots text January 2016
Spectrum of the Nuclear Environment for GaAs Spin Qubits text January 2017
Correlations between Optical Properties and Voronoi-Cell Area of Quantum Dots text January 2019
Characterization of a quasi-static environment with a qubit text January 2019
Fundamental Limits to Coherent Photon Generation with Solid-State Atomlike Transitions text January 2019
Pulse control protocols for preserving coherence in dipolar-coupled nuclear spin baths journal July 2019

Figures / Tables (7)


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