Phosphorus: An Anode of Choice for Sodium-Ion Batteries

Ni, Jiangfeng; Li, Liang; Lu, Jun

doi:10.1021/acsenergylett.8b00312

Title: Phosphorus: An Anode of Choice for Sodium-Ion Batteries

Journal Article · Fri Apr 06 00:00:00 EDT 2018 · ACS Energy Letters

DOI:https://doi.org/10.1021/acsenergylett.8b00312· OSTI ID:1484017

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Soochow Univ., Suzhou (People’s Republic of China). College of Physics, Optoelectronics and Energy, Center for Energy Conversion Materials & Physics (CECMP)
Argonne National Lab. (ANL), Argonne, IL (United States). Chemical Sciences and Engineering Division

Phosphorus (P) offers a high theoretical capacity of 2596 mAh g^-1 and thus has been intensively pursued as one of the most promising anodes for sodium-ion batteries. However, sodium storage in P anodes is facing significant technical challenges in terms of poor conductivity, large volume swelling, and an unstable solid-electrolyte interphase. These challenges need to be well mitigated before P material can be deployed in full batteries. In this Perspective, we summarize the latest research progress in the development of P anodes. Here, we focus on the design principle and criteria of efficient P anodes and materials strategies that mainly leverage the knowledge accumulated for the lithium anode of silicon. We also highlight the decisive role that theoretical simulation and in situ techniques play in addressing these difficulties associated with P materials.

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Research Organization:: Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Vehicle Technologies Office (EE-3V); National Natural Science Foundation of China (NSFC)

Grant/Contract Number:: AC02-06CH11357; 17KJA430013; BK20151219; BK20140009; 51672182; 51772197; 51422206

OSTI ID:: 1484017

Journal Information:: ACS Energy Letters, Vol. 3, Issue 5; ISSN 2380-8195

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 111 works

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