Chemical Feedback From Decreasing Carbon Monoxide Emissions

Gaubert, B.; Worden, H. M.; Arellano, A. F. J.; Emmons, L. K.; Tilmes, S.; Barré, J.; Martinez Alonso, S.; Vitt, F.; Anderson, J. L.; Alkemade, F.; Houweling, S.; Edwards, D. P.

doi:10.1002/2017GL074987

Chemical Feedback From Decreasing Carbon Monoxide Emissions

Journal Article · Wed Sep 13 00:00:00 EDT 2017 · Geophysical Research Letters

DOI:https://doi.org/10.1002/2017GL074987· OSTI ID:1479337

^[1]; ^[1]; ^[2]; ^[1]; ^[1]; Barré, J. ^[1]; Martinez Alonso, S. ^[1]; ^[1]; Anderson, J. L. ^[1]; Alkemade, F. ^[3]; ^[3]; ^[1]

National Center for Atmospheric Research, Boulder, CO (United States)
Univ. of Arizona, Tucson, AZ (United States)
SRON Netherlands Institute for Space Research, Utrecht (Netherlands); Utrecht Univ., Utrecht (Netherlands)

Understanding changes in the burden and growth rate of atmospheric methane (CH₄) has been the focus of several recent studies but still lacks scientific consensus. Here we investigate the role of decreasing anthropogenic carbon monoxide (CO) emissions since 2002 on hydroxyl radical (OH) sinks and tropospheric CH₄ loss. We quantify this impact by contrasting two model simulations for 2002–2013: (1) a Measurement of the Pollution in the Troposphere (MOPITT) CO reanalysis and (2) a Control-Run without CO assimilation. These simulations are performed with the Community Atmosphere Model with Chemistry of the Community Earth System Model fully coupled chemistry climate model with prescribed CH₄ surface concentrations. The assimilation of MOPITT observations constrains the global CO burden, which significantly decreased over this period by ~20%. We find that this decrease results to (a) increase in CO chemical production, (b) higher CH₄ oxidation by OH, and (c) ~8% shorter CH₄ lifetime. As a result, we elucidate this coupling by a surrogate mechanism for CO-OH-CH₄ that is quantified from the full chemistry simulations.

View Accepted Manuscript (DOE)

Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: AC02-05CH11231

OSTI ID:: 1479337

Journal Information:: Geophysical Research Letters, Journal Name: Geophysical Research Letters Journal Issue: 19 Vol. 44; ISSN 0094-8276

Publisher:: American Geophysical UnionCopyright Statement

Country of Publication:: United States

Language:: English

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Radiance-based Retrieval Bias Mitigation for the MOPITT Instrument: The Version 8 Product Deeter, Merritt N.; Edwards, David P.; Francis, Gene L. Atmospheric Measurement Techniques Discussions https://doi.org/10.5194/amt-2019-41	posted_content	March 2019
Global atmospheric carbon monoxide budget 2000–2017 inferred from multi-species atmospheric inversions Zheng, Bo; Chevallier, Frederic; Yin, Yi Earth System Science Data, Vol. 11, Issue 3 https://doi.org/10.5194/essd-11-1411-2019	journal	January 2019

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