A 15-year record of CO emissions constrained by MOPITT CO observations

Jiang, Zhe; Worden, John R.; Worden, Helen; Deeter, Merritt; Jones, Dylan B. A.; Arellano, Avelino F.; Henze, Daven K.

doi:10.5194/acp-17-4565-2017

A 15-year record of CO emissions constrained by MOPITT CO observations

Journal Article · Thu Apr 06 00:00:00 EDT 2017 · Atmospheric Chemistry and Physics (Online)

DOI:https://doi.org/10.5194/acp-17-4565-2017· OSTI ID:1479310

^[1]; Worden, John R. ^[2]; Worden, Helen ^[3]; Deeter, Merritt ^[3]; Jones, Dylan B. A. ^[4]; Arellano, Avelino F. ^[5]; Henze, Daven K. ^[6]

California Inst. of Technology (CalTech), Pasadena, CA (United States); National Center for Atmospheric Research, Boulder, CO (United States)
California Inst. of Technology (CalTech), Pasadena, CA (United States)
National Center for Atmospheric Research, Boulder, CO (United States)
Univ. of Toronto, Toronto, ON (Canada)
Univ. of Arizona, Tucson, AZ (United States)
Univ. of Colorado, Boulder, CO (United States)

Long-term measurements from satellites and surface stations have demonstrated a decreasing trend of tropospheric carbon monoxide (CO) in the Northern Hemisphere over the past decade. Likely explanations for this decrease include changes in anthropogenic, fires, and/or biogenic emissions or changes in the primary chemical sink hydroxyl radical (OH). Using remotely sensed CO measurements from the Measurement of Pollution in the Troposphere (MOPITT) satellite instrument, in situ methyl chloroform (MCF) measurements from the World Data Centre for Greenhouse Gases (WDCGG) and the adjoint of the GEOS-Chem model, we estimate the change in global CO emissions from 2001 to 2015. We show that the loss rate of MCF varied by 0.2 % in the past 15 years, indicating that changes in global OH distributions do not explain the recent decrease in CO. Our two-step inversion approach for estimating CO emissions is intended to mitigate the effect of bias errors in the MOPITT data as well as model errors in transport and chemistry, which are the primary factors contributing to the uncertainties when quantifying CO emissions using these remotely sensed data. Our results confirm that the decreasing trend of tropospheric CO in the Northern Hemisphere is due to decreasing CO emissions from anthropogenic and biomass burning sources. In particular, we find decreasing CO emissions from the United States and China in the past 15 years, and unchanged anthropogenic CO emissions from Europe since 2008. We find decreasing trends of biomass burning CO emissions from boreal North America, boreal Asia and South America, but little change over Africa. In contrast to prior results, we find that a positive trend in CO emissions is likely for India and southeast Asia.

View Accepted Manuscript (DOE)

Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: AC02-05CH11231

OSTI ID:: 1479310

Journal Information:: Atmospheric Chemistry and Physics (Online), Journal Name: Atmospheric Chemistry and Physics (Online) Journal Issue: 7 Vol. 17; ISSN 1680-7324

Publisher:: European Geosciences UnionCopyright Statement

Country of Publication:: United States

Language:: English

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Modeling Regional Pollution Transport Events During KORUS‐AQ: Progress and Challenges in Improving Representation of Land‐Atmosphere Feedbacks Huang, Min; Crawford, James H.; Diskin, Glenn S. Journal of Geophysical Research: Atmospheres, Vol. 123, Issue 18 https://doi.org/10.1029/2018jd028554	journal	September 2018
Quantifying Emissions of CO and NO _x Using Observations From MOPITT, OMI, TES, and OSIRIS Zhang, X.; Jones, D. B. A.; Keller, M. Journal of Geophysical Research: Atmospheres, Vol. 124, Issue 2 https://doi.org/10.1029/2018jd028670	journal	January 2019
Source Contributions to Carbon Monoxide Concentrations During KORUS‐AQ Based on CAM‐chem Model Applications Tang, Wenfu; Emmons, Louisa K.; Arellano Jr, Avelino F. Journal of Geophysical Research: Atmospheres, Vol. 124, Issue 5 https://doi.org/10.1029/2018jd029151	journal	March 2019
Multiconstituent Data Assimilation With WRF‐Chem/DART: Potential for Adjusting Anthropogenic Emissions and Improving Air Quality Forecasts Over Eastern China Ma, Chaoqun; Wang, Tijian; Mizzi, Arthur P. Journal of Geophysical Research: Atmospheres https://doi.org/10.1029/2019jd030421	journal	July 2019
Unexpected slowdown of US pollutant emission reduction in the past decade Jiang, Zhe; McDonald, Brian C.; Worden, Helen Proceedings of the National Academy of Sciences, Vol. 115, Issue 20 https://doi.org/10.1073/pnas.1801191115	journal	April 2018
Rapid decline in carbon monoxide emissions and export from East Asia between years 2005 and 2016 Zheng, Bo; Chevallier, Frederic; Ciais, Philippe Environmental Research Letters, Vol. 13, Issue 4 https://doi.org/10.1088/1748-9326/aab2b3	journal	March 2018
Detecting drought impact on terrestrial biosphere carbon fluxes over contiguous US with satellite observations Liu, Junjie; Bowman, Kevin; Parazoo, Nicholas C. Environmental Research Letters, Vol. 13, Issue 9 https://doi.org/10.1088/1748-9326/aad5ef	journal	September 2018
Impacts of Chemical and Synoptic Processes on Summer Tropospheric Ozone Trend in North China Zhou, Lihua; Zhang, Jing; Zheng, Xiaohui Advances in Meteorology, Vol. 2019 https://doi.org/10.1155/2019/3148432	journal	December 2019
Trends in China's anthropogenic emissions since 2010 as the consequence of clean air actions Zheng, Bo; Tong, Dan; Li, Meng Atmospheric Chemistry and Physics, Vol. 18, Issue 19 https://doi.org/10.5194/acp-18-14095-2018	journal	January 2018
New constraints on biogenic emissions using satellite-based estimates of carbon monoxide fluxes Worden, Helen M.; Bloom, A. Anthony; Worden, John R. Atmospheric Chemistry and Physics, Vol. 19, Issue 21 https://doi.org/10.5194/acp-19-13569-2019	journal	January 2019
Radiance-based retrieval bias mitigation for the MOPITT instrument: the version 8 product Deeter, Merritt N.; Edwards, David P.; Francis, Gene L. Atmospheric Measurement Techniques, Vol. 12, Issue 8 https://doi.org/10.5194/amt-12-4561-2019	journal	January 2019
Evaluation of MOPITT Version 7 joint TIR–NIR X_CO retrievals with TCCON Hedelius, Jacob K.; He, Tai-Long; Jones, Dylan B. A. Atmospheric Measurement Techniques, Vol. 12, Issue 10 https://doi.org/10.5194/amt-12-5547-2019	journal	January 2019
Global atmospheric carbon monoxide budget 2000–2017 inferred from multi-species atmospheric inversions Zheng, Bo; Chevallier, Frederic; Yin, Yi Earth System Science Data, Vol. 11, Issue 3 https://doi.org/10.5194/essd-11-1411-2019	journal	January 2019
Improved method for linear carbon monoxide simulation and source attribution in atmospheric chemistry models illustrated using GEOS-Chem v9 Fisher, Jenny A.; Murray, Lee T.; Jones, Dylan B. A. Geoscientific Model Development, Vol. 10, Issue 11 https://doi.org/10.5194/gmd-10-4129-2017	journal	January 2017

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