Numerical studies of CO2 and brine leakage into a shallow aquifer through an open wellbore

Wang, Jingrui; Hu, Litang; Pan, Lehua; Zhang, Keni

doi:10.1007/s10040-017-1685-y

Numerical studies of CO₂ and brine leakage into a shallow aquifer through an open wellbore

Journal Article · Thu Nov 09 00:00:00 EST 2017 · Hydrogeology Journal

DOI:https://doi.org/10.1007/s10040-017-1685-y· OSTI ID:1476630

Wang, Jingrui ^[1]; Hu, Litang ^[1]; Pan, Lehua ^[2]; Zhang, Keni ^[2]

Beijing Normal Univ., Beijing (China). College of Water Sciences, Engineering Research Center of Groundwater Pollution Control and Remediation of Ministry of Education
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Energy Geosciences Division

Industrial-scale geological storage of CO₂ in saline aquifers may cause CO₂ and brine leakage from abandoned wells into shallow fresh aquifers. This leakage problem involves the flow dynamics in both the wellbore and the storage reservoir. T2Well/ECO2N, a coupled wellbore-reservoir flow simulator, was used to analyze CO₂ and brine leakage under different conditions with a hypothetical simulation model in water-CO₂-brine systems. Parametric studies on CO₂ and brine leakage, including the salinity, excess pore pressure (EPP) and initially dissolved CO₂ mass fraction, are conducted to understand the mechanism of CO₂ migration. The results show that brine leakage rates increase proportionally with EPP and inversely with the salinity when EPP varies from 0.5 to 1.5 MPa; however, there is no CO₂ leakage into the shallow freshwater aquifer if EPP is less than 0.5 MPa. The dissolved CO₂ mass fraction shows an important influence on the CO₂ plume, as part of the dissolved CO₂ becomes a free phase. Scenario simulation shows that the gas lifting effect will significantly increase the brine leakage rate into the shallow freshwater aquifer under the scenario of 3.89% dissolved CO₂ mass fraction. The equivalent porous media (EPM) approach used to model the wellbore flow has been evaluated and results show that the EPM approach could either under- or over-estimate brine leakage rates under most scenarios. The discrepancies become more significant if a free CO₂ phase evolves. Therefore, a model that can correctly describe the complex flow dynamics in the wellbore is necessary for investigating the leakage problems.

View Accepted Manuscript (DOE)

Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: AC02-05CH11231

OSTI ID:: 1476630

Journal Information:: Hydrogeology Journal, Journal Name: Hydrogeology Journal Journal Issue: 2 Vol. 26; ISSN 1431-2174

Publisher:: SpringerCopyright Statement

Country of Publication:: United States

Language:: English

References (36)

Optimization of injection location based on simulations of CO ₂ leakage through multiple leakage pathways : Optimization of Injection Location Based on CO2 Leakage Yu, Bo; Wang, Le; Liu, Yongzhong Asia-Pacific Journal of Chemical Engineering, Vol. 11, Issue 4 https://doi.org/10.1002/apj.1990	journal	March 2016
Understanding the carbon dioxide sequestration in low-permeability saline aquifers in the Ordos Basin with numerical simulations Xie, Jian; Zhang, Keni; Hu, Litang Greenhouse Gases: Science and Technology, Vol. 5, Issue 5 https://doi.org/10.1002/ghg.1499	journal	May 2015
CO ₂ solubility measurements in brine under reservoir conditions: A comparison of experimental and geochemical modeling methods : CO Steel, Luc; Liu, Qi; Mackay, Eric Greenhouse Gases: Science and Technology, Vol. 6, Issue 2 https://doi.org/10.1002/ghg.1590	journal	February 2016
Evaluation of Potential Changes in Groundwater Quality in Response to CO2 Leakage from Deep Geologic Storage Apps, J. A.; Zheng, L.; Zhang, Y. Transport in Porous Media, Vol. 82, Issue 1 https://doi.org/10.1007/s11242-009-9509-8	journal	January 2010
Modeling of CO2 Leakage up Through an Abandoned Well from Deep Saline Aquifer to Shallow Fresh Groundwaters Humez, Pauline; Audigane, Pascal; Lions, Julie Transport in Porous Media, Vol. 90, Issue 1 https://doi.org/10.1007/s11242-011-9801-2	journal	August 2011
Semi-analytical Solution for Brine Leakage Through Passive Abandoned Wells Taking Account of Brine Density Differences Réveillère, Arnaud Transport in Porous Media, Vol. 100, Issue 2 https://doi.org/10.1007/s11242-013-0221-3	journal	September 2013
Modelling CO2-brine-rock interactions in the Upper Paleozoic formations of Ordos Basin used for CO2 sequestration Liu, Hejuan; Hou, Zhengmeng; Were, Patrick Environmental Earth Sciences, Vol. 73, Issue 5 https://doi.org/10.1007/s12665-014-3571-4	journal	August 2014
An improved model calculating CO2 solubility in pure water and aqueous NaCl solutions from 273 to 533 K and from 0 to 2000 bar Duan, Zhenhao; Sun, Rui Chemical Geology, Vol. 193, Issue 3-4 https://doi.org/10.1016/S0009-2541(02)00263-2	journal	February 2003
Sequestration of CO2 in geological media: criteria and approach for site selection in response to climate change Bachu, Stefan Energy Conversion and Management, Vol. 41, Issue 9 https://doi.org/10.1016/S0196-8904(99)00149-1	journal	June 2000
Analytical solution for two-phase flow in a wellbore using the drift-flux model Pan, Lehua; Webb, Stephen W.; Oldenburg, Curtis M. Advances in Water Resources, Vol. 34, Issue 12 https://doi.org/10.1016/j.advwatres.2011.08.009	journal	December 2011
Early detection of brine and CO2 leakage through abandoned wells using pressure and surface-deformation monitoring data: Concept and demonstration Jung, Yoojin; Zhou, Quanlin; Birkholzer, Jens T. Advances in Water Resources, Vol. 62 https://doi.org/10.1016/j.advwatres.2013.06.008	journal	December 2013
T2Well—An integrated wellbore–reservoir simulator Pan, Lehua; Oldenburg, Curtis M. Computers & Geosciences, Vol. 65 https://doi.org/10.1016/j.cageo.2013.06.005	journal	April 2014
On mobilization of lead and arsenic in groundwater in response to CO2 leakage from deep geological storage Zheng, Liange; Apps, John A.; Zhang, Yingqi Chemical Geology, Vol. 268, Issue 3-4 https://doi.org/10.1016/j.chemgeo.2009.09.007	journal	November 2009
Large-scale numerical simulation of CO2 geologic storage and its impact on regional groundwater flow: A hypothetical case study at Tokyo Bay, Japan Yamamoto, Hajime; Zhang, Keni; Karasaki, Kenzi Energy Procedia, Vol. 1, Issue 1 https://doi.org/10.1016/j.egypro.2009.01.244	journal	February 2009
Numerical Simulation of CO2 Leakage through Abandoned Wells: Model for an Abandoned Site with Observed Gas Migration in Alberta, Canada Pawar, Rajesh J.; Watson, Theresa L.; Gable, Carl W. Energy Procedia, Vol. 1, Issue 1 https://doi.org/10.1016/j.egypro.2009.02.158	journal	February 2009
An improved model to forecast CO2 leakage rates along a wellbore Tao, Qing; Checkai, Dean; Huerta, Nicolas Energy Procedia, Vol. 4 https://doi.org/10.1016/j.egypro.2011.02.522	journal	January 2011
Large-scale impact of CO2 storage in deep saline aquifers: A sensitivity study on pressure response in stratified systems Birkholzer, J.; Zhou, Q.; Tsang, C. International Journal of Greenhouse Gas Control, Vol. 3, Issue 2 https://doi.org/10.1016/j.ijggc.2008.08.002	journal	March 2009
Review of integrity of existing wells in relation to CO2 geological storage: What do we know? Zhang, Min; Bachu, Stefan International Journal of Greenhouse Gas Control, Vol. 5, Issue 4 https://doi.org/10.1016/j.ijggc.2010.11.006	journal	July 2011
Brine flow up a well caused by pressure perturbation from geologic carbon sequestration: Static and dynamic evaluations Birkholzer, Jens T.; Nicot, Jean Philippe; Oldenburg, Curtis M. International Journal of Greenhouse Gas Control, Vol. 5, Issue 4 https://doi.org/10.1016/j.ijggc.2011.01.003	journal	July 2011
Evaluation and development of options for remediation of CO2 leakage into groundwater aquifers from geologic carbon storage Esposito, Ariel; Benson, Sally M. International Journal of Greenhouse Gas Control, Vol. 7 https://doi.org/10.1016/j.ijggc.2011.12.002	journal	March 2012
Modeling brine leakage to shallow aquifer through an open wellbore using T2WELL/ECO2N Hu, Litang; Pan, Lehua; Zhang, Keni International Journal of Greenhouse Gas Control, Vol. 9 https://doi.org/10.1016/j.ijggc.2012.05.010	journal	July 2012
CO2 flow through a fractured rock volume: Insights from field data, 3D fractures representation and fluid flow modeling Bigi, S.; Battaglia, M.; Alemanni, A. International Journal of Greenhouse Gas Control, Vol. 18 https://doi.org/10.1016/j.ijggc.2013.07.011	journal	October 2013
Well permeability estimation and CO2 leakage rates Tao, Qing; Bryant, Steven L. International Journal of Greenhouse Gas Control, Vol. 22 https://doi.org/10.1016/j.ijggc.2013.12.022	journal	March 2014
Benchmark modeling of the Sleipner CO2 plume: Calibration to seismic data for the uppermost layer and model sensitivity analysis Zhu, Chen; Zhang, Guanru; Lu, Peng International Journal of Greenhouse Gas Control, Vol. 43 https://doi.org/10.1016/j.ijggc.2014.12.016	journal	December 2015
Reduced order models of transient CO2 and brine leakage along abandoned wellbores from geologic carbon sequestration reservoirs Harp, Dylan R.; Pawar, Rajesh; Carey, J. William International Journal of Greenhouse Gas Control, Vol. 45 https://doi.org/10.1016/j.ijggc.2015.12.001	journal	February 2016
A full chain CCS demonstration project in northeast Ordos Basin, China: Operational experience and challenges Zhang, Keni; Xie, Jian; Li, Cai International Journal of Greenhouse Gas Control, Vol. 50 https://doi.org/10.1016/j.ijggc.2016.04.025	journal	July 2016
Modeling changes in pressure due to migration of fluids into the Above Zone Monitoring Interval of a geologic carbon storage site Namhata, Argha; Zhang, Liwei; Dilmore, Robert M. International Journal of Greenhouse Gas Control, Vol. 56 https://doi.org/10.1016/j.ijggc.2016.11.012	journal	January 2017
Simulation of groundwater flow within observation boreholes for confined aquifers Hu, Litang; Chen, Chongxi; Chen, Xunhong Journal of Hydrology, Vol. 398, Issue 1-2 https://doi.org/10.1016/j.jhydrol.2010.12.013	journal	February 2011
An improved model for the calculation of CO2 solubility in aqueous solutions containing Na+, K+, Ca2+, Mg2+, Cl−, and SO42− Duan, Zhenhao; Sun, Rui; Zhu, Chen Marine Chemistry, Vol. 98, Issue 2-4 https://doi.org/10.1016/j.marchem.2005.09.001	journal	February 2006
Semianalytical Solution for CO ₂ Leakage through an Abandoned Well Nordbotten, Jan Martin; Celia, Michael A.; Bachu, Stefan Environmental Science & Technology, Vol. 39, Issue 2 https://doi.org/10.1021/es035338i	journal	January 2005
Model for CO ₂ Leakage Including Multiple Geological Layers and Multiple Leaky Wells Nordbotten, Jan M.; Kavetski, Dmitri; Celia, Michael A. Environmental Science & Technology, Vol. 43, Issue 3 https://doi.org/10.1021/es801135v	journal	February 2009
Analytical solutions for leakage rates through abandoned wells: ANALYTICAL SOLUTIONS FOR LEAKAGE RATES Nordbotten, Jan Martin; Celia, Michael A.; Bachu, Stefan Water Resources Research, Vol. 40, Issue 4 https://doi.org/10.1029/2003WR002997	journal	April 2004
A new model for predicting the hydraulic conductivity of unsaturated porous media Mualem, Yechezkel Water Resources Research, Vol. 12, Issue 3 https://doi.org/10.1029/WR012i003p00513	journal	June 1976
Estimating CO2 Fluxes Along Leaky Wellbores Tao, Qing; Checkai, Dean; Huerta, Nicolas SPE Journal, Vol. 19, Issue 02 https://doi.org/10.2118/135483-PA	journal	April 2014
Leakage Calculator for Plugged and Abandoned Wells Ford, Eric P.; Moeinikia, Fatemeh; Lohne, Hans Petter SPE Bergen One Day Seminar https://doi.org/10.2118/185890-MS	conference	April 2017
A Closed-form Equation for Predicting the Hydraulic Conductivity of Unsaturated Soils1 van Genuchten, M. Th. Soil Science Society of America Journal, Vol. 44, Issue 5 https://doi.org/10.2136/sssaj1980.03615995004400050002x	journal	January 1980

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