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Title: Numerical studies of CO2 and brine leakage into a shallow aquifer through an open wellbore

Journal Article · · Hydrogeology Journal
 [1];  [1];  [2];  [2]
  1. Beijing Normal Univ., Beijing (China). College of Water Sciences, Engineering Research Center of Groundwater Pollution Control and Remediation of Ministry of Education
  2. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Energy Geosciences Division

Industrial-scale geological storage of CO2 in saline aquifers may cause CO2 and brine leakage from abandoned wells into shallow fresh aquifers. This leakage problem involves the flow dynamics in both the wellbore and the storage reservoir. T2Well/ECO2N, a coupled wellbore-reservoir flow simulator, was used to analyze CO2 and brine leakage under different conditions with a hypothetical simulation model in water-CO2-brine systems. Parametric studies on CO2 and brine leakage, including the salinity, excess pore pressure (EPP) and initially dissolved CO2 mass fraction, are conducted to understand the mechanism of CO2 migration. The results show that brine leakage rates increase proportionally with EPP and inversely with the salinity when EPP varies from 0.5 to 1.5 MPa; however, there is no CO2 leakage into the shallow freshwater aquifer if EPP is less than 0.5 MPa. The dissolved CO2 mass fraction shows an important influence on the CO2 plume, as part of the dissolved CO2 becomes a free phase. Scenario simulation shows that the gas lifting effect will significantly increase the brine leakage rate into the shallow freshwater aquifer under the scenario of 3.89% dissolved CO2 mass fraction. The equivalent porous media (EPM) approach used to model the wellbore flow has been evaluated and results show that the EPM approach could either under- or over-estimate brine leakage rates under most scenarios. The discrepancies become more significant if a free CO2 phase evolves. Therefore, a model that can correctly describe the complex flow dynamics in the wellbore is necessary for investigating the leakage problems.

Research Organization:
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC)
Grant/Contract Number:
AC02-05CH11231
OSTI ID:
1476630
Journal Information:
Hydrogeology Journal, Vol. 26, Issue 2; ISSN 1431-2174
Publisher:
SpringerCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 6 works
Citation information provided by
Web of Science

References (36)

Brine flow up a well caused by pressure perturbation from geologic carbon sequestration: Static and dynamic evaluations journal July 2011
Analytical solutions for leakage rates through abandoned wells: ANALYTICAL SOLUTIONS FOR LEAKAGE RATES journal April 2004
Numerical Simulation of CO2 Leakage through Abandoned Wells: Model for an Abandoned Site with Observed Gas Migration in Alberta, Canada journal February 2009
Understanding the carbon dioxide sequestration in low-permeability saline aquifers in the Ordos Basin with numerical simulations journal May 2015
Model for CO 2 Leakage Including Multiple Geological Layers and Multiple Leaky Wells journal February 2009
CO2 flow through a fractured rock volume: Insights from field data, 3D fractures representation and fluid flow modeling journal October 2013
Modeling of CO2 Leakage up Through an Abandoned Well from Deep Saline Aquifer to Shallow Fresh Groundwaters journal August 2011
Modelling CO2-brine-rock interactions in the Upper Paleozoic formations of Ordos Basin used for CO2 sequestration journal August 2014
Modeling changes in pressure due to migration of fluids into the Above Zone Monitoring Interval of a geologic carbon storage site journal January 2017
CO 2 solubility measurements in brine under reservoir conditions: A comparison of experimental and geochemical modeling methods : CO journal February 2016
Evaluation of Potential Changes in Groundwater Quality in Response to CO2 Leakage from Deep Geologic Storage journal January 2010
Review of integrity of existing wells in relation to CO2 geological storage: What do we know? journal July 2011
Reduced order models of transient CO2 and brine leakage along abandoned wellbores from geologic carbon sequestration reservoirs journal February 2016
A full chain CCS demonstration project in northeast Ordos Basin, China: Operational experience and challenges journal July 2016
Well permeability estimation and CO2 leakage rates journal March 2014
Evaluation and development of options for remediation of CO2 leakage into groundwater aquifers from geologic carbon storage journal March 2012
Large-scale impact of CO2 storage in deep saline aquifers: A sensitivity study on pressure response in stratified systems journal March 2009
Analytical solution for two-phase flow in a wellbore using the drift-flux model journal December 2011
T2Well—An integrated wellbore–reservoir simulator journal April 2014
Estimating CO2 Fluxes Along Leaky Wellbores journal April 2014
Sequestration of CO2 in geological media: criteria and approach for site selection in response to climate change journal June 2000
Optimization of injection location based on simulations of CO 2 leakage through multiple leakage pathways : Optimization of Injection Location Based on CO2 Leakage journal March 2016
Simulation of groundwater flow within observation boreholes for confined aquifers journal February 2011
Large-scale numerical simulation of CO2 geologic storage and its impact on regional groundwater flow: A hypothetical case study at Tokyo Bay, Japan journal February 2009
Modeling brine leakage to shallow aquifer through an open wellbore using T2WELL/ECO2N journal July 2012
A new model for predicting the hydraulic conductivity of unsaturated porous media journal June 1976
An improved model calculating CO2 solubility in pure water and aqueous NaCl solutions from 273 to 533 K and from 0 to 2000 bar journal February 2003
An improved model for the calculation of CO2 solubility in aqueous solutions containing Na+, K+, Ca2+, Mg2+, Cl−, and SO42− journal February 2006
Leakage Calculator for Plugged and Abandoned Wells conference April 2017
A Closed-form Equation for Predicting the Hydraulic Conductivity of Unsaturated Soils1 journal January 1980
Early detection of brine and CO2 leakage through abandoned wells using pressure and surface-deformation monitoring data: Concept and demonstration journal December 2013
Benchmark modeling of the Sleipner CO2 plume: Calibration to seismic data for the uppermost layer and model sensitivity analysis journal December 2015
Semianalytical Solution for CO 2 Leakage through an Abandoned Well journal January 2005
An improved model to forecast CO2 leakage rates along a wellbore journal January 2011
On mobilization of lead and arsenic in groundwater in response to CO2 leakage from deep geological storage journal November 2009
Semi-analytical Solution for Brine Leakage Through Passive Abandoned Wells Taking Account of Brine Density Differences journal September 2013

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