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Spatial and Temporal Correlations of XY Macro Spins

Journal Article · · Nano Letters
 [1];  [2];  [3];  [4];  [5];  [2]
  1. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Materials Sciences Division; Lawrence Berkeley National Laboratory
  2. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Materials Sciences Division; Univ. of California, Santa Cruz, CA (United States). Dept. of Physics
  3. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Molecular Foundry
  4. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS)
  5. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS); Univ. of Oregon, Eugene, OR (United States). Dept. of Physics
Here, we use nano disk arrays with square and honeycomb symmetry to investigate magnetic phases and spin correlations of XY dipolar systems at the micro scale. Utilizing magnetization sensitive x-ray photoemission electron microscopy, we probe magnetic ground states and the ”order-by-disorder” phenomenon predicted 30 years ago. We observe the antiferromagnetic striped ground state in square lattices, and six-fold symmetric structures, including trigonal vortex lattices and disordered floating vortices, in the honeycomb lattice. The spin frustration in the honeycomb lattice causes a phase transition from a long-range ordered locked phase over a floating phase with quasi long-range order and indications of a Berezinskii-Thouless-Kosterlitz-like character, to the thermally excited paramagnetic state. Absent spatial correlation and quasi periodic switching of isolated vortices in the quasi long-range ordered phase suggest a degeneracy of the vortex circulation.
Research Organization:
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Scientific User Facilities Division
Grant/Contract Number:
AC02-05CH11231
OSTI ID:
1473704
Alternate ID(s):
OSTI ID: 1530322
Journal Information:
Nano Letters, Journal Name: Nano Letters Journal Issue: 12 Vol. 18; ISSN 1530-6984
Publisher:
American Chemical SocietyCopyright Statement
Country of Publication:
United States
Language:
English

References (41)

Magnetic Microstructure of Rolled-Up Single-Layer Ferromagnetic Nanomembranes journal October 2013
Experimental Evidence of Chiral Ferrimagnetism in Amorphous GdCo Films journal May 2018
Resonating valence bonds: A new kind of insulator? journal February 1973
Hartmann characterization of the PEEM-3 aberration-corrected X-ray photoemission electron microscope journal May 2018
Zero-point entropy in ‘spin ice’ journal May 1999
Artificial ‘spin ice’ in a geometrically frustrated lattice of nanoscale ferromagnetic islands journal January 2006
Spontaneous skyrmion ground states in magnetic metals journal August 2006
Real-space observation of a two-dimensional skyrmion crystal journal June 2010
Multiply periodic states and isolated skyrmions in an anisotropic frustrated magnet journal September 2015
Static three-dimensional topological solitons in fluid chiral ferromagnets and colloids journal December 2016
Real-space observation of emergent magnetic monopoles and associated Dirac strings in artificial kagome spin ice journal October 2010
Thermal ground-state ordering and elementary excitations in artificial magnetic square ice journal November 2010
Skyrmion dynamics in a frustrated ferromagnetic film and current-induced helicity locking-unlocking transition journal November 2017
Collective magnetism in an artificial 2D XY spin system journal July 2018
Interaction modifiers in artificial spin ices journal February 2018
Order as an effect of disorder journal January 1980
Thermal transitions in nano-patterned XY-magnets journal July 2014
Vortex circulation patterns in planar microdisk arrays journal June 2017
Ordering, metastability and phase transitions in two-dimensional systems journal April 1973
Electron holography—basics and applications journal December 2007
Frustration and chiral orderings in correlated electron systems journal July 2016
Anisotropic Superexchange Interaction and Weak Ferromagnetism journal October 1960
Planar classical dipolar system on a honeycomb lattice journal February 1988
Ordering due to disorder in dipolar magnets on two-dimensional lattices journal October 1990
Soft-x-ray magnetic circular dichroism at the L 2 , 3 edges of nickel journal October 1990
Dipolar-induced planar anisotropy in ultrathin magnetic films journal June 1997
Nanoscale structure of the magnetic induction at monopole defects in artificial spin-ice lattices journal May 2011
Kosterlitz-Thouless transition of magnetic dipoles on the two-dimensional plane journal May 2011
Phase diagram of dipolar-coupled XY moments on disordered square lattices journal August 2018
Multiple- q States and the Skyrmion Lattice of the Triangular-Lattice Heisenberg Antiferromagnet under Magnetic Fields journal January 2012
Magnetic Dipole and Higher Pole Interaction on a Square Lattice journal April 2013
Skyrmion Knots in Frustrated Magnets journal June 2017
Solvable Model of a Spin-Glass journal December 1975
X-ray circular dichroism as a probe of orbital magnetization journal March 1992
Geometrical Frustration in the Ferromagnetic Pyrochlore Ho 2 Ti 2 O 7 journal September 1997
Multipolar Ordering and Magnetization Reversal in Two-Dimensional Nanomagnet Arrays journal November 2005
Glassy Spin Dynamics in Geometrically Frustrated Buckled Colloidal Crystals journal May 2017
Spin glasses: Experimental facts, theoretical concepts, and open questions journal October 1986
Dipolar effects in magnetic thin films and quasi-two-dimensional systems journal January 2000
Quantum spin liquid states journal April 2017
Spin Ice State in Frustrated Magnetic Pyrochlore Materials journal November 2001

Cited By (5)

Ice-rule made manifold: phase transitions, topological defects and manifold restoration in two-dimensional artificial spin systems text January 2019
Advances in artificial spin ice journal November 2019
Continuous ground-state degeneracy of classical dipoles on regular lattices journal July 2019
Continuous magnetic phase transition in artificial square ice journal June 2019
Reconfigurable ferromagnetic liquid droplets journal July 2019

Figures / Tables (5)