Chemical kinetics in an atmospheric pressure helium plasma containing humidity

Schröter, Sandra; Wijaikhum, Apiwat; Gibson, Andrew R.; West, Andrew; Davies, Helen L.; Minesi, Nicolas; Dedrick, James; Wagenaars, Erik; de Oliveira, Nelson; Nahon, Laurent; Kushner, Mark J.; Booth, Jean-Paul; Niemi, Kari; Gans, Timo; O'Connell, Deborah

doi:10.1039/C8CP02473A

Title: Chemical kinetics in an atmospheric pressure helium plasma containing humidity

Journal Article · Mon Jan 01 00:00:00 EST 2018 · Physical Chemistry Chemical Physics. PCCP

DOI:https://doi.org/10.1039/C8CP02473A· OSTI ID:1470577

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^[1]; Minesi, Nicolas ^[1];

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^[1]; de Oliveira, Nelson ^[2]; Nahon, Laurent ^[2];

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York Plasma Institute, Department of Physics, University of York, York YO10 5DD, UK
Synchrotron Soleil, l'Orme des Merisiers, 91192 Gif sur Yvette Cedex, France
Department of Electrical Engineering and Computer Science, University of Michigan, Ann Arbor, USA
LPP, CNRS, Ecole Polytechnique, UPMC Univ. Paris-Sud, Observatoire de Paris

Atmospheric pressure plasmas are sources of biologically active oxygen and nitrogen species, which makes them potentially suitable for the use as biomedical devices. Here, experiments and simulations are combined to investigate the formation of the key reactive oxygen species, atomic oxygen (O) and hydroxyl radicals (OH), in a radio-frequency driven atmospheric pressure plasma jet operated in humidified helium. Vacuum ultra-violet high-resolution Fourier-transform absorption spectroscopy and ultra-violet broad-band absorption spectroscopy are used to measure absolute densities of O and OH. These densities increase with increasing H₂O content in the feed gas, and approach saturation values at higher admixtures on the order of 3 × 10¹⁴ cm^-3 for OH and 3 × 10¹³ cm^-3 for O. Experimental results are used to benchmark densities obtained from zero-dimensional plasma chemical kinetics simulations, which reveal the dominant formation pathways. At low humidity content, O is formed from OH⁺ by proton transfer to H₂O, which also initiates the formation of large cluster ions. At higher humidity content, O is created by reactions between OH radicals, and lost by recombination with OH. OH is produced mainly from H₂O⁺ by proton transfer to H₂O and by electron impact dissociation of H₂O. It is lost by reactions with other OH molecules to form either H₂O + O or H₂O₂. Formation pathways change as a function of humidity content and position in the plasma channel. The understanding of the chemical kinetics of O and OH gained in this work will help in the development of plasma tailoring strategies to optimise their densities in applications.

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Research Organization:: Univ. of Michigan, Ann Arbor, MI (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: SC0001319; SC0014132

OSTI ID:: 1470577

Alternate ID(s):: OSTI ID: 1483482

Journal Information:: Physical Chemistry Chemical Physics. PCCP, Journal Name: Physical Chemistry Chemical Physics. PCCP Vol. 20 Journal Issue: 37; ISSN 1463-9076

Publisher:: Royal Society of Chemistry (RSC)Copyright Statement

Country of Publication:: United Kingdom

Language:: English

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Cited by: 56 works

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Figures / Tables (26)

Table 5: Part 1(p. 15)

Table 5: Part 2(p. 16)

Table 6(p. 17)

Table 7: Part 1(p. 17)

Table 7: Part 2(p. 18)

Table 8: Part 1(p. 19)

Table 8: Part 2(p. 20)

Table 9(p. 20)

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