Measurement of the effective capacitance of solutions containing nanoscale uranyl peroxide cage clusters (U60) reveals cluster effects

Liu, Yi; Szymanowski, Jennifer E.  S.; Sigmon, Ginger E.; Morris, David E.; Hixon, Amy E.; Migliori, Albert; Burns, Peter C.

doi:10.1007/s10967-017-5659-2

Title: Measurement of the effective capacitance of solutions containing nanoscale uranyl peroxide cage clusters (U60) reveals cluster effects

Journal Article · Wed Dec 20 00:00:00 EST 2017 · Journal of Radioanalytical and Nuclear Chemistry

DOI:https://doi.org/10.1007/s10967-017-5659-2· OSTI ID:1470045

Liu, Yi; Szymanowski, Jennifer E. S.; Sigmon, Ginger E.; Morris, David E.; Hixon, Amy E.; Migliori, Albert; Burns, Peter C.

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Research Organization:: Energy Frontier Research Centers (EFRC) (United States). Materials Science of Actinides (MSA)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

DOE Contract Number:: SC0001089

OSTI ID:: 1470045

Journal Information:: Journal of Radioanalytical and Nuclear Chemistry, Vol. 315, Issue 2; Related Information: MSA partners with University of Notre Dame (lead); University of California, Davis; Florida State University; George Washington University; University of Michigan; University of Minnesota; Oak Ridge National Laboratory; Oregon state University; Rensselaer Polytechnic Institute; Savannah River National Laboratory; ISSN 0236-5731

Publisher:: Springer

Country of Publication:: United States

Language:: English

References (20)

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Simulations of Cyclic Voltammetry for Electric Double Layers in Asymmetric Electrolytes: A Generalized Modified Poisson–Nernst–Planck Model Wang, Hainan; Thiele, Alexander; Pilon, Laurent The Journal of Physical Chemistry C, Vol. 117, Issue 36 https://doi.org/10.1021/jp402181e	journal	August 2013
A comprehensive comparison of transition-metal and actinyl polyoxometalates Nyman, May; Burns, Peter C. Chemical Society Reviews, Vol. 41, Issue 22 https://doi.org/10.1039/c2cs35136f	journal	January 2012
Thermal Responsive Ion Selectivity of Uranyl Peroxide Nanocages: An Inorganic Mimic of K ⁺ Ion Channels Gao, Yunyi; Szymanowski, Jennifer E. S.; Sun, Xinyu Angewandte Chemie International Edition, Vol. 55, Issue 24 https://doi.org/10.1002/anie.201601852	journal	April 2016
Clusters of Actinides with Oxide, Peroxide, or Hydroxide Bridges Qiu, Jie; Burns, Peter C. Chemical Reviews, Vol. 113, Issue 2 https://doi.org/10.1021/cr300159x	journal	October 2012
Base-Driven Assembly of Large Uranium Oxo/Hydroxo Clusters Biswas, Biplab; Mougel, Victor; Pécaut, Jacques Angewandte Chemie International Edition, Vol. 50, Issue 25 https://doi.org/10.1002/anie.201101327	journal	May 2011
Influence of solvent nature on the electrochemical parameters of electrical double layer capacitors Lust, E.; Jänes, A.; Arulepp, M. Journal of Electroanalytical Chemistry, Vol. 562, Issue 1 https://doi.org/10.1016/j.jelechem.2003.07.034	journal	January 2004
Symmetry versus Minimal Pentagonal Adjacencies in Uranium-Based Polyoxometalate Fullerene Topologies Sigmon, Ginger E.; Unruh, Daniel K.; Ling, Jie Angewandte Chemie International Edition, Vol. 48, Issue 15 https://doi.org/10.1002/anie.200805870	journal	March 2009
Alkali-metal ion coordination in uranyl( vi ) poly-peroxide complexes in solution. Part 1: the Li ⁺ , Na ⁺ and K ⁺ – peroxide–hydroxide systems Zanonato, Pier Luigi; Di Bernardo, Plinio; Vallet, Valerie Dalton Transactions, Vol. 44, Issue 4 https://doi.org/10.1039/C4DT02104E	journal	January 2015
Comparing the differential capacitance of two ionic liquid electrolytes: Effects of specific adsorption Zhang, Qian; Han, Yining; Wang, Yonglong Electrochemistry Communications, Vol. 38 https://doi.org/10.1016/j.elecom.2013.10.027	journal	January 2014
Voltammetry at a de Levie brush electrode as a model for electrochemical supercapacitor behaviour Pell, W. G.; Conway, B. E. Journal of Electroanalytical Chemistry, Vol. 500, Issue 1-2 https://doi.org/10.1016/S0022-0728(00)00423-X	journal	March 2001
Selective Permeability of Uranyl Peroxide Nanocages to Different Alkali Ions: Influences from Surface Pores and Hydration Shells Gao, Yunyi; Haso, Fadi; Szymanowski, Jennifer E. S. Chemistry - A European Journal, Vol. 21, Issue 51 https://doi.org/10.1002/chem.201503773	journal	November 2015
Thickness of electrical double layer. Effect of ion size Bohinc, Klemen; Kralj-Iglič, Veronika; Iglič, Aleš Electrochimica Acta, Vol. 46, Issue 19 https://doi.org/10.1016/S0013-4686(01)00525-4	journal	June 2001
Actinyl Peroxide Nanospheres Burns, Peter C.; Kubatko, Karrie-Ann; Sigmon, Ginger Angewandte Chemie International Edition, Vol. 44, Issue 14 https://doi.org/10.1002/anie.200462445	journal	March 2005
Uranyl peroxide enhanced nuclear fuel corrosion in seawater Armstrong, C. R.; Nyman, M.; Shvareva, T. Proceedings of the National Academy of Sciences, Vol. 109, Issue 6 https://doi.org/10.1073/pnas.1119758109	journal	January 2012
Experimental measurements of U24Py nanocluster behavior in aqueous solution Flynn, Shannon L.; Szymanowski, Jennifer E. S.; Dembowski, Mateusz Radiochimica Acta, Vol. 104, Issue 12 https://doi.org/10.1515/ract-2015-2493	journal	January 2016
Uranyl Peroxide Cage Cluster Solubility in Water and the Role of the Electrical Double Layer Peruski, Kathryn M.; Bernales, Varinia; Dembowski, Mateusz Inorganic Chemistry, Vol. 56, Issue 3 https://doi.org/10.1021/acs.inorgchem.6b02435	journal	January 2017
Single-Crystal Time-of-Flight Neutron Diffraction and Magic-Angle-Spinning NMR Spectroscopy Resolve the Structure and ¹ H and ⁷ Li Dynamics of the Uranyl Peroxide Nanocluster U ₆₀ Olds, Travis A.; Dembowski, Mateusz; Wang, Xiaoping Inorganic Chemistry, Vol. 56, Issue 16 https://doi.org/10.1021/acs.inorgchem.7b01174	journal	July 2017
Influence of the solvent properties on the characteristics of a double layer capacitor Arulepp, M.; Permann, L.; Leis, J. Journal of Power Sources, Vol. 133, Issue 2 https://doi.org/10.1016/j.jpowsour.2004.03.026	journal	June 2004
Physical interpretation of cyclic voltammetry for measuring electric double layer capacitances Wang, Hainan; Pilon, Laurent Electrochimica Acta, Vol. 64 https://doi.org/10.1016/j.electacta.2011.12.118	journal	March 2012

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Title: Measurement of the effective capacitance of solutions containing nanoscale uranyl peroxide cage clusters (U60) reveals cluster effects

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