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Title: Low-energy inelastic response in the superconducting phases of PrOs4Sb12

Journal Article · · Physical Review B
 [1];  [1];  [1]
  1. Univ. of Illinois at Urbana-Champaign, IL (United States)

Recent ac susceptibility and polar Kerr effect measurements in the skutterudite superconductor PrOs4Sb12 (POS) uncovered the nature of the superconducting double transition from a high-temperature, high-field, time-reversal symmetric phase (or the A phase) to a low-temperature, low-field, time-reversal symmetry-broken phase (or the B phase). In this work, starting from a microscopic model, we derive a Ginzburg-Landau expansion relevant to POS that describes this entrance into the time-reversal symmetry-broken phase along the temperature axis. We also provide a study of the low-energy inelastic (Raman) response in both the A and B phases of POS, and seek additional signatures which could help reveal the exact form of the gap functions previously proposed in these phases. By appropriately manipulating the incoming and scattered light geometries, along with additional subtraction procedures and suitable assumptions, we show that one can access the various irreducible representations contained in the point group describing POS. We demonstrate how to use this technique on example order parameters proposed in POS. Depending on whether there exist nodes along the c axis, we find additional low-energy spectral weight within the superconducting gap in the $$E_g$$ geometry, a feature that could pinpoint the location of nodes on the Fermi surface.

Research Organization:
Energy Frontier Research Centers (EFRC) (United States). Center for Emergent Superconductivity (CES)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES); Gordon and Betty Moore Foundation
Grant/Contract Number:
AC02-98CH10886; GBMF4305; AC0298CH1088
OSTI ID:
1469835
Alternate ID(s):
OSTI ID: 1375258
Journal Information:
Physical Review B, Vol. 96, Issue 5; Related Information: CES partners with Brookhaven National Laboratory (BNL); Argonne National Laboratory; University of Illinois, Urbana-Champaign; Los Alamos National Laboratory; ISSN 2469-9950
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 1 work
Citation information provided by
Web of Science

References (40)

Possible Mass Enhancement by Multipole Fluctuations Excited via the Singlet–Triplet Crystal Electric Field States in PrOs 4 Sb 12 : Sb-NMR Studies Using a Single Crystal journal July 2011
Conservation laws, vertex corrections, and screening in Raman spectroscopy journal July 2017
Thermodynamical Study on the Heavy-Fermion Superconductor PrOs 4 Sb 12 : Evidence for Field-Induced Phase Transition journal September 2002
Evidence for Unconventional Strong-Coupling Superconductivity in P r O s 4 S b 12 : An Sb Nuclear Quadrupole Resonance Study journal January 2003
Magnetic Excitations in Heavy-Fermion Superconductor PrOs 4 Sb 12 journal June 2004
Crystal-Field Excitations, Magnetic-Field-Induced Phase Transition and Neutron-Scattering Spectra in PrOs 4 Sb 12 journal December 2004
Multiple Superconducting Phases in New Heavy Fermion Superconductor P r O s 4 S b 12 journal March 2003
Probing the Superconducting Gap Symmetry of P r O s 4 S b 12 : A Penetration Depth Study journal December 2003
Multiphase superconductivity in skutterudite PrOs 4 Sb 12 journal November 2003
Electronic Raman scattering in superconductors as a probe of anisotropic electron pairing journal June 1995
Heavy Fermion Superconductivity in the Filled Skutterudite Compound PrOs 4 Sb 12 journal January 2002
de Haas–van Alphen Study of the Pr-based Filled Skutterudite PrOs 4 P 12 journal January 2008
Magnetic Phase Diagram of the Heavy Fermion Superconductor PrOs 4 Sb 12 journal June 2003
Unconventional Superconductivity and Heavy Fermion Behavior in PrOs4Sb12 journal December 2006
Evidence for Point Nodes in the Superconducting Gap Function in the Filled Skutterudite Heavy-Fermion Compound PrOs 4 Sb 12 : 123 Sb-NQR Study under Pressure journal February 2007
Phenomenology for multiple phases in the heavy-fermion skutterudite superconductor PrOs 4 Sb 12 journal May 2003
High Magnetic Field Phase Diagram of P r O s 4 S b 12 journal January 2004
Theory of Field-Induced Phase Transition in PrOs 4 Sb 12 journal March 2004
Spin-triplet superconductivity in Pr Os 4 Sb 12 probed by muon Knight shift journal January 2007
Theory of a new type of heavy-electron superconductivity in PrOs 4 Sb 12 : quadrupolar-fluctuation mediated odd-parity pairings journal May 2003
Low-Temperature Specific Heat of the Heavy-Fermion Superconductor Pr  O s 4 S b 12 journal February 2003
s + i s state with broken time-reversal symmetry in Fe-based superconductors journal April 2013
Superconducting PrOs 4 Sb 12 : A Thermal Conductivity Study journal December 2006
Multiband electronic Raman scattering in bilayer superconductors journal November 1996
Superconducting gaps via Raman scattering in iron superconductors journal May 2014
Sb-NMR studies of single-crystal journal April 2005
Multipolar Moments in Pr-based Filled-Skutterudite Compounds with Singlet–Triplet Crystal-Field Levels journal August 2004
The Unconventional Superconductivity of Skutterudite PrOs 4 Sb 12 : Time-Reversal Symmetry Breaking and Adjacent Field-Induced Quadrupole Ordering journal May 2007
Evidence for Magnetic-Field-Induced Quadrupolar Ordering in the Heavy-Fermion Superconductor PrOs 4 Sb 12 journal May 2003
Superconductivity and heavy fermion behavior in PrOs 4 Sb 12 journal February 2002
Inelastic light scattering from correlated electrons journal January 2007
Theory of Raman scattering in superconductors journal May 1984
Muon Spin Relaxation and Isotropic Pairing in Superconducting P r O s 4 S b 12 journal September 2002
Time-Reversal Symmetry-Breaking Superconductivity in Heavy-Fermion P r O s 4 S b 12 Detected by Muon-Spin Relaxation journal August 2003
Triplet superconductivity in the skutterudite PrOs 4 Sb 12 journal December 2004
Fermi surface of the heavy-fermion superconductor PrOs 4 Sb 12 journal December 2002
Superconducting states in the tetrahedral compound PrOs 4 Sb 12 journal October 2004
Three-dimensional Majorana fermions in chiral superconductors journal December 2016
Fermi surface of the Pr-based filled skutterudite compound PrOs 4 P 12 journal January 2009
On Superconducting Double Transition in PrOs 4 Sb 12 journal June 2003

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