Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

Broadband ultrafast terahertz spectroscopy in the 25 T Split Florida-Helix

Journal Article · · Review of Scientific Instruments
DOI:https://doi.org/10.1063/1.5023384· OSTI ID:1467388
 [1];  [1];  [1];  [1];  [1];  [1];  [1];  [2];  [3];  [4];  [1]
  1. Univ. of Alabama, Birmingham, AL (United States). Dept. of Physics
  2. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States). Center for Integrated Nanotechnologies
  3. Florida State Univ., Tallahassee, FL (United States). National High Magnetic Field Lab. (MagLab)
  4. Univ. of South Florida, Tampa, FL (United States). Dept. of Physics

In this paper, we describe the development of a broadband (0.3–10 THz) optical pump-terahertz probe spectrometer with an unprecedented combination of temporal resolution (≤200 fs) operating in external magnetic fields as high as 25 T using the new Split Florida-Helix magnet system. Finally, using this new instrument, we measure the transient dynamics in a gallium arsenide four-quantum well sample after photoexcitation at 800 nm.

Research Organization:
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); Univ. of South Florida, Tampa, FL (United States); Univ. of Alabama, Birmingham, AL (United States); Florida State Univ., Tallahassee, FL (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22); National Science Foundation (NSF) (United States); Dept. of Education (ED) (United States)
Grant/Contract Number:
NA0003525; AC52-06NA25396; SC0012635
OSTI ID:
1467388
Alternate ID(s):
OSTI ID: 1460023
Report Number(s):
SAND--2018-1897J; 662901
Journal Information:
Review of Scientific Instruments, Journal Name: Review of Scientific Instruments Journal Issue: 7 Vol. 89; ISSN 0034-6748
Publisher:
American Institute of Physics (AIP)Copyright Statement
Country of Publication:
United States
Language:
English

References (83)

Exploring Dynamics in the Far-Infrared with Terahertz Spectroscopy journal June 2004
Observation of Ultrafast Free Carrier Dynamics in Single Layer MoS 2 journal August 2015
Exploring Dynamics in the Far-Infrared with Terahertz Spectroscopy journal April 2004
Time- and Polarization-Resolved Optical Spectroscopy of Colloidal CdSe Nanocrystal Quantum Dots in High Magnetic Fields journal August 2005
Quasi-phase-matched generation of coherent extreme-ultraviolet light journal January 2003
Metal wires for terahertz wave guiding journal November 2004
Ultrafast charge localization in a stripe-phase nickelate journal October 2013
Cooperative photoinduced metastable phase control in strained manganite films journal July 2016
Valley- and spin-polarized Landau levels in monolayer WSe2 journal October 2016
Cutting-edge terahertz technology journal February 2007
Coherent control of terahertz supercontinuum generation in ultrafast laser–gas interactions journal July 2008
High-temperature superconductivity in iron-based materials journal August 2010
Enhancement of superconductivity by a parallel magnetic field in two-dimensional superconductors journal August 2011
Long-lived nanosecond spin relaxation and spin coherence of electrons in monolayer MoS2 and WS2 journal August 2015
Evidence of an odd-parity hidden order in a spin–orbit coupled correlated iridate journal October 2015
Coherent cyclotron motion beyond Kohn’s theorem journal November 2015
Light-induced electron localization in a quantum Hall system journal April 2017
High power ultrafast lasers journal March 1998
Fiber-coupled antennas for ultrafast coherent terahertz spectroscopy in low temperatures and high magnetic fields journal September 2002
Pure Rotational Spectrum of Water Vapor journal October 1967
The Design of Powerful Electromagnets Part IV. The New Magnet Laboratory at M. I. T. journal December 1939
Algorithm for high-resolution single-shot THz measurement using in-line spectral interferometry with chirped pulses journal November 2005
GaAs, AlAs, and Al x Ga 1− x As: Material parameters for use in research and device applications journal August 1985
A table-top, repetitive pulsed magnet for nonlinear and ultrafast spectroscopy in high magnetic fields up to 30 T journal December 2013
Terahertz gas photonics journal June 2009
Ultrafast optical and far-infrared quasiparticle dynamics in correlated electron materials journal December 2002
Ultrafast dynamics of localized magnetic moments in the unconventional Mott insulator Sr 2 IrO 4 journal June 2016
Shubnikov–de Haas-like oscillations in millimeterwave photoconductivity in a high-mobility two-dimensional electron gas journal October 2001
Quantized Hall conductivity in two dimensions journal May 1981
Measurement of Fermi-surface distortion in double quantum wells from in-plane magnetic fields journal May 1991
Self-consistent density of states for a single- and double-quantum-well structure in a parallel magnetic field journal October 1996
Quasiparticle relaxation dynamics in superconductors with different gap structures: Theory and experiments on YBa 2 Cu 3 O 7 − δ journal January 1999
Liquid-crystal phases of quantum Hall systems journal March 1999
Femtosecond optical-pulse-induced absorption and refractive-index changes in GaAs in the midinfrared journal September 1999
Optical evidence for transient photoinduced magnetization in La 0.7 Ca 0.3 Mn O 3 journal February 2005
Terahertz magnetoconductivity of excitons and electrons in quantum cascade structures journal March 2008
Transient terahertz spectroscopy of excitons and unbound carriers in quasi-two-dimensional electron-hole gases journal January 2009
Shubnikov–de Haas oscillations in GaAs quantum wells in tilted magnetic fields journal June 2012
Reorientation of quantum Hall stripes within a partially filled Landau level journal March 2016
Cyclotron decay time of a two-dimensional electron gas from 0.4 to 100 K journal April 2016
Magnetic resonances of multiferroic TbFe 3 ( BO 3 ) 4 journal January 2017
Spatially resolved and time-resolved imaging of transport of indirect excitons in high magnetic fields journal June 2017
Scaling in Plateau-to-Plateau Transition: A Direct Connection of Quantum Hall Systems with the Anderson Localization Model journal May 2009
Two-Quantum Many-Body Coherences in Two-Dimensional Fourier-Transform Spectra of Exciton Resonances in Semiconductor Quantum Wells journal March 2010
Terahertz Spectroscopy of Spin Waves in Multiferroic BiFeO 3 in High Magnetic Fields journal June 2013
Optical Coherence in Atomic-Monolayer Transition-Metal Dichalcogenides Limited by Electron-Phonon Interactions journal March 2016
High-Temperature Terahertz Optical Diode Effect without Magnetic Order in Polar FeZnMo 3 O 8 journal January 2018
Anomalous Quantum Hall Effect: An Incompressible Quantum Fluid with Fractionally Charged Excitations journal May 1983
Spin beats and dynamical magnetization in quantum structures journal January 1994
Evidence for an Anisotropic State of Two-Dimensional Electrons in High Landau Levels journal January 1999
Nematic Phase of the Two-Dimensional Electron Gas in a Magnetic Field journal February 2000
Ultrafast Conductivity Dynamics in Colossal Magnetoresistance Manganites journal June 2001
Pair-Breaking and Superconducting State Recovery Dynamics in M g B 2 journal December 2003
Dynamic Kerr Effect and the Spectral Weight Transfer of the Manganites journal July 2004
Enhanced Photosusceptibility near T c for the Light-Induced Insulator-to-Metal Phase Transition in Vanadium Dioxide journal November 2007
Electrodynamics of correlated electron materials journal June 2011
Fabrication and Assembly of the NHMFL 25 T Resistive Split Magnet journal June 2012
Electronically controlled optical sampling using 100 MHz repetition rate fiber lasers conference February 2008
Optical Signatures of the Aharonov-Bohm Phase in Single-Walled Carbon Nanotubes journal May 2004
Light-Induced Superconductivity in a Stripe-Ordered Cuprate journal January 2011
Terahertz pulse propagation in the near field and the far field journal January 2000
Broadband terahertz detection with selected gases journal January 2009
Broadband Terahertz Detection with Selected Gases
  • Lu, Xiaofei; Karpowicz, Nicholas; Zhang, X. -C.
  • Nonlinear Optics: Materials, Fundamentals and Applications, Advances in Optical Sciences Congress https://doi.org/10.1364/nlo.2009.nwa4
conference January 2009
Direct measurement of cyclotron coherence times of high-mobility two-dimensional electron gases journal January 2010
Single-shot terahertz time-domain spectroscopy in pulsed high magnetic fields journal January 2016
Terahertz-pulse generation by photoionization of air with laser pulses composed of both fundamental and second-harmonic waves journal January 2004
Terahertz time-domain magnetospectroscopy of a high-mobility two-dimensional electron gas journal January 2007
Ultrafast pump–probe spectroscopy in gallium arsenide at 25 T journal January 2014
Ultrafast Conductivity Dynamics in Colossal Magnetoresistance Manganites text January 2001
Terahertz Time-Domain Magnetospectroscopy of a High-Mobility Two-Dimensional Electron Gas text January 2007
High-temperature superconductivity in iron-based materials text January 2010
Terahertz spectroscopy of spin waves in multiferroic BiFeO$_3$ in high magnetic fields text January 2013
Long-lived nanosecond spin relaxation and spin coherence of electrons in monolayer MoS_2 and WS_2 text January 2015
Observation of Ultrafast Free Carrier Dynamics in Single Layer MoS$_2$ text January 2015
Cooperative photoinduced metastable phase control in strained manganite films text January 2015
Reorientation of quantum Hall stripes within a partially filled Landau level text January 2016
Coherent cyclotron motion beyond Kohn's theorem text January 2016
Spatially and time-resolved imaging of transport of indirect excitons in high magnetic fields text January 2017
Dynamic Kerr Effect and Spectral Weight Transfer in the Manganites text January 2003
Time- and Polarization-Resolved Optical Spectroscopy of Colloidal CdSe Nanocrystal Quantum Dots in High Magnetic Fields text January 2005
Liquid Crystal Phases of Quantum Hall Systems text January 1998
Nematic phase of the two-dimensional electron gas in a magnetic field text January 1999
Fiber-coupled Antennas for Ultrafast Coherent Terahertz Spectroscopy in Low Temperatures and High Magnetic Fields text January 2002

Cited By (1)

Coherent two-dimensional Fourier transform spectroscopy using a 25 Tesla resistive magnet journal June 2019

Similar Records

Ultrafast terahertz Faraday rotation in graphene
Journal Article · Sat Dec 06 23:00:00 EST 2014 · Journal of Applied Physics · OSTI ID:22402735

Evaluation of DAST and zinc telluride nonlinear crystals for efficient terahertz generation
Journal Article · Fri Jul 31 00:00:00 EDT 2015 · AIP Conference Proceedings · OSTI ID:22488645