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Fully differential single-photon double photoionization of atomic magnesium

Journal Article · · Physical Review A
 [1];  [2];  [3]
  1. California State Univ. Maritime Academy (Cal Maritime), Vallejo, CA (United States). Dept. of Science and Mathematics
  2. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Chemical Sciences Division
  3. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Chemical Sciences Division; Univ. of California, Davis, CA (United States). Dept. of Chemistry
The valence-shell double ionization of atomic magnesium is calculated using a grid-based representation of the 3s2 electron configuration in the presence of a fully occupied frozen-core configuration of the remaining ten electrons. Atomic orbitals are constructed from an underlying finite-element discrete variable representation that facilitates accurate representation of the interaction between the inner-shell electrons with those entering the continuum. Length and velocity gauge results are compared with recent theoretical calculations and experimental measurements for the total double-, single-, and triple-differential cross sections, particularly at the photon energy of 55.49 eV for the last one. Comparison between the similar processes of double ionization of the ns2 atoms helium, beryllium, and magnesium further illuminates the role of valence-shell electron correlation in atomic targets with heliumlike electronic configurations and symmetry.
Research Organization:
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Chemical Sciences, Geosciences & Biosciences Division
Grant/Contract Number:
AC02-05CH11231
OSTI ID:
1465405
Alternate ID(s):
OSTI ID: 1335726
Journal Information:
Physical Review A, Journal Name: Physical Review A Journal Issue: 6 Vol. 94; ISSN PLRAAN; ISSN 2469-9926
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

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Cited By (3)

Resonant single-photon double ionization driven by combined intra- and interatomic electron correlations journal January 2020
Dissociation dynamics of the water dication following one-photon double ionization. I. Theory journal November 2018
Resonant single-photon double ionization driven by combined intra- and interatomic electron correlations text January 2019

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