Reference Correlation for the Viscosity of Carbon Dioxide

Laesecke, Arno; Muzny, Chris D.

doi:10.1063/1.4977429

Title: Reference Correlation for the Viscosity of Carbon Dioxide

Journal Article · Tue Mar 21 00:00:00 EDT 2017 · Journal of Physical and Chemical Reference Data

DOI:https://doi.org/10.1063/1.4977429· OSTI ID:1463125

Laesecke, Arno ^[1]; Muzny, Chris D. ^[1]

National Inst. of Standards and Technology (NIST), Boulder, CO (United States)

A comprehensive database of experimental and computed data for the viscosity of carbon dioxide (CO₂) was compiled and a new reference correlation was developed. Literature results based on an ab initio potential energy surface were the foundation of the correlation of the viscosity in the limit of zero density in the temperature range from 100 K to 2000 K. Guided symbolic regression was employed to obtain a new functional form that extrapolates correctly to T → 0 K and to 10 000 K. Coordinated measurements at low density made it possible to implement the temperature dependence of the Rainwater-Friend theory in the linear-in-density viscosity term. The residual viscosity could be formulated with a scaling term ργ/T the significance of which was confirmed by symbolic regression. The final viscosity correlation covers temperatures from 100 K to 2000 K for gaseous CO₂, and from 220 K to 700 K with pressures along the melting line up to 8000 MPa for compressed and supercritical liquid states. The data representation is more accurate than with the previous correlations, and the covered pressure and temperature range is significantly extended. The critical enhancement of the viscosity of CO₂ is included in the new correlation.

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Research Organization:: National Inst. of Standards and Technology (NIST), Boulder, CO (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: FE0003931

OSTI ID:: 1463125

Journal Information:: Journal of Physical and Chemical Reference Data, Vol. 46, Issue 1; ISSN 0047-2689

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 75 works

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