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Title: Ultrahigh critical current densities, the vortex phase diagram, and the effect of granularity of the stoichiometric high-Tc superconductor CaKFe4As4

Journal Article · · Physical Review Materials

We present a comprehensive study of the critical current densities and the superconducting vortex phase diagram in the stoichiometric superconductor CaKFe4As4 which has a critical temperature of ~35 K. We performed detailed magnetization measurements both of high quality single crystals for different orientations in an applied magnetic field up to 16 T and for a powder sample. We find an extremely large critical current density, Jc, up to 108 A/cm2 for single crystals when H∥(ab) at 5 K, which remains robust in fields up to 16 T, being the largest of any other iron-based superconductor. The critical current density is reduced by a factor 10 in single crystals when H∥c at 5 K and significantly suppressed by the presence of grain boundaries in the powder sample. We also observe the presence of the fishtail effect in the magnetic hysteresis loops of single crystals when H∥c. The flux pinning force density and the pinning parameters suggest that the large critical current could be linked to the existence of point core and surface pinning. Based on the vortex phase diagram and the large critical current densities, CaKFe4As4 is now established as a potential iron-based superconductor candidate for practical applications.

Research Organization:
Ames Lab., Ames, IA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC02-07CH11358; GBMF4411; EP/I004475/1
OSTI ID:
1556119
Alternate ID(s):
OSTI ID: 1462138
Report Number(s):
is-j 9731; PRMHAR
Journal Information:
Physical Review Materials, Vol. 2, Issue 7; ISSN 2475-9953
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 44 works
Citation information provided by
Web of Science

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Cited By (10)

Unique defect structure and advantageous vortex pinning properties in superconducting CaKFe4As4 journal June 2019
Strong pinning in the hole-doped pnictide superconductor La 0.34 Na 0.66 Fe 2 As 2 journal March 2019
Chemical stability and superconductivity in Ag-sheathed CaKFe 4 As 4 superconducting tapes journal November 2018
Fe-based superconducting thin films—preparation and tuning of superconducting properties journal August 2019
Effects of core density and impurities on the critical current density of CaKFe 4 As 4 superconducting tapes journal September 2019
Optimization of superconducting properties of the stoichiometric CaKFe 4 As 4 journal December 2019
Enhancement of critical current density in CaKFe 4 As 4 single crystals through 3 MeV proton irradiation journal January 2020
Flux pinning and the vortex phase diagram in optimized CaKFe 4 As 4 single crystals fabricated by a one-step method journal February 2020
Strong pinning in the hole-doped pnictide superconductor La$_{0.34}$Na$_{0.66}$Fe$_2$As$_2$ text January 2019
Unique defect structure and advantageous vortex pinning properties in superconducting CaKFe4As4 text January 2019