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A Comprehensive Set of High-Quality Point Charges for Simulations of Metal–Organic Frameworks

Journal Article · · Chemistry of Materials
 [1];  [2];  [2]
  1. Georgia Inst. of Technology, Atlanta, GA (United States); University of Minnesota Nanoporous Materials Genome Center
  2. Georgia Inst. of Technology, Atlanta, GA (United States)

Most classical simulations of metal-organic frameworks model electrostatic interactions using point charges on each atom in the structure. We report atomic point charges derived from periodic DFT electronic structure calculations for over 2,000 unique experimentally synthesized MOFs. These charges are publicly available as a supplement to the Computation-Ready Experimental MOF database. These DFT derived atomic point charges are compared to semi-empirical group contribution and charge equilibration methods for assigning charges. As an example of using these charges, we examined each MOF for usefulness in the adsorptive removal of tert-butyl mercaptan (TBM) from natural gas. Monte Carlo simulations revealed many candidate MOF structures with high selectivity for TBM over CH4 and high TBM capacity. As a result, we anticipate that this public dataset of atomic point charges for MOFs will facilitate high-throughput screening for a wide variety applications where electrostatic interactions must be considered.

Research Organization:
Univ. of Minnesota, Minneapolis, MN (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
Grant/Contract Number:
SC0008688; SC0008688
OSTI ID:
1459352
Journal Information:
Chemistry of Materials, Journal Name: Chemistry of Materials Journal Issue: 3 Vol. 28; ISSN 0897-4756
Publisher:
American Chemical Society (ACS)Copyright Statement
Country of Publication:
United States
Language:
English

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Cited By (23)

Distinguishing Metal–Organic Frameworks journal January 2018
Evaluating Charge Equilibration Methods To Generate Electrostatic Fields in Nanoporous Materials journal November 2018
Force-Field Prediction of Materials Properties in Metal-Organic Frameworks journal January 2017
In Silico Screening of Metal–Organic Frameworks for Adsorption-Driven Heat Pumps and Chillers journal July 2018
Computer-aided discovery of a metal–organic framework with superior oxygen uptake journal April 2018
Computation-Ready Experimental MOFs (CoRE MOFs) dataset January 2014
Materials Databases: The Need for Open, Interoperable Databases with Standardized Data and Rich Metadata journal September 2019
Design, Parameterization, and Implementation of Atomic Force Fields for Adsorption in Nanoporous Materials journal September 2019
Efficiently Exploring Adsorption Space to Identify Privileged Adsorbents for Chemical Separations of a Diverse Set of Molecules journal April 2018
Impact of H2O and CO2 on methane storage in metal–organic frameworks journal September 2019
The effect of atomic point charges on adsorption isotherms of CO2 and water in metal organic frameworks journal December 2019
Introducing DDEC6 atomic population analysis: part 4. Efficient parallel computation of net atomic charges, atomic spin moments, bond orders, and more journal January 2018
Establishing upper bounds on CO 2 swing capacity in sub-ambient pressure swing adsorption via molecular simulation of metal–organic frameworks journal January 2017
Methyl-rotation dynamics in metal–organic frameworks probed with terahertz spectroscopy journal January 2018
Structure–property relationship of metal–organic frameworks for alcohol-based adsorption-driven heat pumps via high-throughput computational screening journal January 2019
Role of partial charge assignment methods in high-throughput screening of MOF adsorbents and membranes for CO 2 /CH 4 separation journal January 2020
A collection of forcefield precursors for metal–organic frameworks journal January 2019
Large-scale evaluation of cascaded adsorption heat pumps based on metal/covalent–organic frameworks journal January 2019
Combining large-scale screening and machine learning to predict the metal-organic frameworks for organosulfurs removal from high-sour natural gas journal September 2019
Capture of pure toxic gases through porous materials from molecular simulations journal February 2018
iRASPA: GPU-accelerated visualization software for materials scientists journal January 2018
Modelling of framework materials at multiple scales: current practices and open questions
  • Fraux, Guillaume; Chibani, Siwar; Coudert, François-Xavier
  • Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 377, Issue 2149 https://doi.org/10.1098/rsta.2018.0220
journal May 2019
Computer-aided discovery of a metal-organic framework with superior oxygen uptake. text January 2018


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