Heating rate dependent ignition of Al/Pt nanolaminates through pulsed laser irradiation

Abere, Michael J.; Yarrington, Cole D.; Adams, David P.

doi:10.1063/1.5026507

Heating rate dependent ignition of Al/Pt nanolaminates through pulsed laser irradiation

Journal Article · Thu Jun 21 00:00:00 EDT 2018 · Journal of Applied Physics

DOI:https://doi.org/10.1063/1.5026507· OSTI ID:1457521

Abere, Michael J. ^[1]; Yarrington, Cole D. ^[1]; Adams, David P. ^[1]

Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

Direct laser irradiation of sputter deposited Al/Pt nanolaminate multilayers results in rapid local heating and exothermic mixing of reactant layers. Milli- and microsecond pulsed laser irradiation under certain test conditions leads to single-point ignition of rapid, self-propagating, formation reactions. Multilayers having bilayer thicknesses of 328 nm, 164 nm, and 65 nm are characterized by their ignition onset times and temperatures. Smaller bilayer thickness multilayers require less laser intensity for ignition compared with larger bilayer designs (when utilizing a particular pulse duration). The relationship between laser intensity and ignition onset time is used to calibrate an activation energy for ignition within a finite element reactive heat transport model. The local heating rate is varied from 10⁴ K/s to 10⁶ K/s by selecting a laser intensity. Kissinger analysis was performed on the heating rate-dependent ignition temperatures measured with high speed pyrometry to experimentally determine an activation energy in the foils of (6.2 ± 1.6 × 10⁴ J/mole atoms). Furthermore, this value is then compared to an activation energy produced from model fits to an ignition onset time of 7.2 × 10⁴ J/mole atoms.

View Accepted Manuscript (DOE)

Research Organization:: Sandia National Laboratories (SNL-NM), Albuquerque, NM (United States)

Sponsoring Organization:: USDOE; USDOE National Nuclear Security Administration (NNSA)

Grant/Contract Number:: AC04-94AL85000

OSTI ID:: 1457521

Alternate ID(s):: OSTI ID: 1456261

Report Number(s):: SAND--2018-6578J; 664565

Journal Information:: Journal of Applied Physics, Journal Name: Journal of Applied Physics Journal Issue: 23 Vol. 123; ISSN 0021-8979

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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