High-pressure-assisted X-ray-induced damage as a new route for materials synthesis

Evlyukhin, Egor; Kim, Eunja; Goldberger, David; Cifligu, Petrika; Weck, Philippe F.; Pravica, Michael

doi:10.1039/c8cp02119h

Title: High-pressure-assisted X-ray-induced damage as a new route for materials synthesis

Journal Article · Mon Jan 01 00:00:00 EST 2018 · Nature

DOI:https://doi.org/10.1039/c8cp02119h· OSTI ID:1457182

Evlyukhin, Egor ^[1]; Kim, Eunja ^[1]; Goldberger, David ^[1]; Cifligu, Petrika ^[1]; Weck, Philippe F. ^[2]; Pravica, Michael ^[1]

Univ. of Nevada, Las Vegas, NV (United States)
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

X-ray radiation induced damage has been known for decades and has largely been viewed as a tremendous nuisance; e.g., most X-ray-related studies of organic and inorganic materials suffer X-ray damage to varying degrees. Although, recent theoretical and experimental investigation of the response of simple chemical systems to X-rays offered better understanding of the mechanistic details of X-ray induced damage, the question about useful applicability of this technique is still unclear. Furthermore we experimentally demonstrate that by tuning pressure and X-ray energy, the radiation induced damage can be controlled and used for synthesis of novel materials.

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Research Organization:: Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA)

DOE Contract Number:: AC04-94AL85000

OSTI ID:: 1457182

Report Number(s):: SAND-2018-0378J; 659920

Journal Information:: Nature, Journal Name: Nature

Country of Publication:: United States

Language:: English

References (41)

Generalized Gradient Approximation Made Simple Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868 https://doi.org/10.1103/PhysRevLett.77.3865	journal	October 1996
Site- and energy-selective slow-electron production through intermolecular Coulombic decay Gokhberg, Kirill; Kolorenč, Přemysl; Kuleff, Alexander I. Nature, Vol. 505, Issue 7485 https://doi.org/10.1038/nature12936	journal	December 2013
Measurement of the Energy Dependence of X-ray-Induced Decomposition of Potassium Chlorate. Pravica, Michael; Bai, Ligang; Sneed, Daniel The Journal of Physical Chemistry A, Vol. 117, Issue 11 https://doi.org/10.1021/jp4008812	journal	March 2013
Projector augmented-wave method Blöchl, P. E. Physical Review B, Vol. 50, Issue 24, p. 17953-17979 https://doi.org/10.1103/PhysRevB.50.17953	journal	December 1994
Raman spectra of O−2 and O−3 ions in alkali-metal superoxides and ozonides Bates, J. B.; Brooker, M. H.; Boyd, G. E. Chemical Physics Letters, Vol. 16, Issue 2 https://doi.org/10.1016/0009-2614(72)80300-2	journal	October 1972
On the nature and origin of dicationic, charge-separated species formed in liquid water on X-ray irradiation Thürmer, Stephan; Ončák, Milan; Ottosson, Niklas Nature Chemistry, Vol. 5, Issue 7 https://doi.org/10.1038/nchem.1680	journal	June 2013
Oxalate minerals on Mars? Applin, D. M.; Izawa, M. R. M.; Cloutis, E. A. Earth and Planetary Science Letters, Vol. 420 https://doi.org/10.1016/j.epsl.2015.03.034	journal	June 2015
$K$ -edge x-ray absorption spectra of Cs and Xe Gomilšek, J. Padežnik; Kodre, A.; Arčon, I. Physical Review A, Vol. 68, Issue 4 https://doi.org/10.1103/PhysRevA.68.042505	journal	October 2003
Synthesis of stable cesium superoxide nanoparticles for gas sensing application by solution-processed spray pyrolysis method Nemade, K. R.; Waghuley, S. A. Applied Nanoscience, Vol. 7, Issue 8 https://doi.org/10.1007/s13204-017-0619-2	journal	October 2017
Measurement of the Energy and High-Pressure Dependence of X-ray-Induced Decomposition of Crystalline Strontium Oxalate Goldberger, David; Evlyukhin, Egor; Cifligu, Petrika The Journal of Physical Chemistry A, Vol. 121, Issue 38 https://doi.org/10.1021/acs.jpca.7b05604	journal	September 2017
Special points for Brillouin-zone integrations Monkhorst, Hendrik J.; Pack, James D. Physical Review B, Vol. 13, Issue 12, p. 5188-5192 https://doi.org/10.1103/PhysRevB.13.5188	journal	June 1976
Rapid structure determination of the hydrogen-containing compound Cs ₂ C ₂ O ₄ ·H ₂ O by joint single-crystal X-ray and powder neutron diffraction Weller, Mark T.; Henry, Paul F.; Light, Mark E. Acta Crystallographica Section B Structural Science, Vol. 63, Issue 3 https://doi.org/10.1107/S0108768107014826	journal	May 2007
X-ray induced synthesis of a novel material: Stable, doped solid CO at ambient conditions Pravica, Michael; Evlyukhin, Egor; Cifligu, Petrika Chemical Physics Letters, Vol. 686 https://doi.org/10.1016/j.cplett.2017.08.053	journal	October 2017
Ultrafast energy transfer between water molecules Jahnke, T.; Sann, H.; Havermeier, T. Nature Physics, Vol. 6, Issue 2 https://doi.org/10.1038/nphys1498	journal	January 2010
Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set Kresse, G.; Furthmüller, J. Physical Review B, Vol. 54, Issue 16, p. 11169-11186 https://doi.org/10.1103/PhysRevB.54.11169	journal	October 1996
The role of metal ions in X-ray-induced photochemistry Stumpf, V.; Gokhberg, K.; Cederbaum, L. S. Nature Chemistry, Vol. 8, Issue 3 https://doi.org/10.1038/nchem.2429	journal	January 2016
Reaction selectivity in an ionized water dimer: nonadiabatic ab initio dynamics simulations Svoboda, Ondřej; Hollas, Daniel; Ončák, Milan Physical Chemistry Chemical Physics, Vol. 15, Issue 27 https://doi.org/10.1039/c3cp51440d	journal	January 2013
Raman Spectroscopy and Dioxygen Adsorption on Cs-Loaded Zeolite Catalysts for Butene Isomerization Li, Junhui; Davis, Robert J. The Journal of Physical Chemistry B, Vol. 109, Issue 15 https://doi.org/10.1021/jp045092j	journal	April 2005
Chasing charge localization and chemical reactivity following photoionization in liquid water Marsalek, Ondrej; Elles, Christopher G.; Pieniazek, Piotr A. The Journal of Chemical Physics, Vol. 135, Issue 22 https://doi.org/10.1063/1.3664746	journal	December 2011
Experimental Observation of Interatomic Coulombic Decay in Neon Dimers Jahnke, T.; Czasch, A.; Schöffler, M. S. Physical Review Letters, Vol. 93, Issue 16 https://doi.org/10.1103/PhysRevLett.93.163401	journal	October 2004
Formation of cesium peroxide and cesium superoxide on InP photocathode activated by cesium and oxygen Sun, Yun; Liu, Zhi; Pianetta, Piero Journal of Applied Physics, Vol. 102, Issue 7 https://doi.org/10.1063/1.2786882	journal	October 2007
Strongly Enhanced Recombination via Two-Center Electronic Correlations Müller, C.; Voitkiv, A. B.; López-Urrutia, J. R. Crespo Physical Review Letters, Vol. 104, Issue 23 https://doi.org/10.1103/PhysRevLett.104.233202	journal	June 2010
Atoms, molecules, solids, and surfaces: Applications of the generalized gradient approximation for exchange and correlation Perdew, John P.; Chevary, J. A.; Vosko, S. H. Physical Review B, Vol. 46, Issue 11 https://doi.org/10.1103/PhysRevB.46.6671	journal	September 1992
Resonant Auger decay driving intermolecular Coulombic decay in molecular dimers Trinter, F.; Schöffler, M. S.; Kim, H. -K. Nature, Vol. 505, Issue 7485 https://doi.org/10.1038/nature12927	journal	December 2013
Characterization of Oxides of Cesium Band, A.; Albu-Yaron, A.; Livneh, T. The Journal of Physical Chemistry B, Vol. 108, Issue 33 https://doi.org/10.1021/jp036432o	journal	August 2004
Die Kristallstrukturen der Alkaliperoxyde F�ppl, Hermann Zeitschrift f�r anorganische und allgemeine Chemie, Vol. 291, Issue 1-4 https://doi.org/10.1002/zaac.19572910104	journal	September 1957
Imaging charge transfer in iodomethane upon x-ray photoabsorption Erk, B.; Boll, R.; Trippel, S. Science, Vol. 345, Issue 6194 https://doi.org/10.1126/science.1253607	journal	July 2014
When X-rays modify the protein structure: radiation damage at work Carugo, Oliviero; Carugo, Kristina Djinović Trends in Biochemical Sciences, Vol. 30, Issue 4 https://doi.org/10.1016/j.tibs.2005.02.009	journal	April 2005
Detection of the aromatic molecule benzonitrile ( c -C ₆ H ₅ CN) in the interstellar medium McGuire, Brett A.; Burkhardt, Andrew M.; Kalenskii, Sergei Science, Vol. 359, Issue 6372 https://doi.org/10.1126/science.aao4890	journal	January 2018
Auger processes in the 21st century Howell, Roger W. International Journal of Radiation Biology, Vol. 84, Issue 12 https://doi.org/10.1080/09553000802395527	journal	January 2008
The Vibrational Spectra of the Formate, Acetate, and Oxalate ions Ito, K.; Bernstein, H. J. Canadian Journal of Chemistry, Vol. 34, Issue 2 https://doi.org/10.1139/v56-021	journal	February 1956
DIOPTAS : a program for reduction of two-dimensional X-ray diffraction data and data exploration Prescher, Clemens; Prakapenka, Vitali B. High Pressure Research, Vol. 35, Issue 3 https://doi.org/10.1080/08957959.2015.1059835	journal	May 2015
The peroxide-ion fundamental frequency Evans, J. C. Journal of the Chemical Society D: Chemical Communications, Issue 12 https://doi.org/10.1039/c29690000682	journal	January 1969
Giant Intermolecular Decay and Fragmentation of Clusters Cederbaum, L. S.; Zobeley, J.; Tarantelli, F. Physical Review Letters, Vol. 79, Issue 24 https://doi.org/10.1103/PhysRevLett.79.4778	journal	December 1997
High-precision sampling for Brillouin-zone integration in metals Methfessel, M.; Paxton, A. T. Physical Review B, Vol. 40, Issue 6 https://doi.org/10.1103/PhysRevB.40.3616	journal	August 1989
Structure of Anhydrous Alkali-Metal Formates Wilson, Michael P.; Alcock, Nathaniel W.; Rodger, P. Mark Inorganic Chemistry, Vol. 45, Issue 11 https://doi.org/10.1021/ic051910q	journal	May 2006
Double-Strand Breaks in Dna Induced by the K-Shell Ionization of Calcium Atoms Takakura, Kaoru Acta Oncologica, Vol. 35, Issue 7 https://doi.org/10.3109/02841869609104041	journal	January 1996
New perspectives on basic zeolites as catalysts and catalyst supports Davis, Robert J. Journal of Catalysis, Vol. 216, Issue 1-2 https://doi.org/10.1016/S0021-9517(02)00034-9	journal	May 2003
Competitive charge transfer reactions in small [Mg(H2O)N]2+ clusters Barran, P. E.; Walker, N. R.; Stace, A. J. The Journal of Chemical Physics, Vol. 112, Issue 14 https://doi.org/10.1063/1.481218	journal	April 2000
Electronic decay in weakly bound heteroclusters: Energy transfer versus electron transfer Zobeley, Jürgen; Santra, Robin; Cederbaum, Lorenz S. The Journal of Chemical Physics, Vol. 115, Issue 11 https://doi.org/10.1063/1.1395555	journal	September 2001
Interatomic and intermolecular Coulombic decay: the coming of age story Jahnke, T. Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 48, Issue 8 https://doi.org/10.1088/0953-4075/48/8/082001	journal	March 2015

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