Nanochannel structures in W enhance radiation tolerance

Qin, Wenjing; Ren, Feng; Doerner, Russell P.; Wei, Guo; Lv, Yawei; Chang, Sheng; Tang, Ming; Deng, Huiqiu; Jiang, Changzhong; Wang, Yongqiang

doi:10.1016/j.actamat.2018.04.048

Title: Nanochannel structures in W enhance radiation tolerance

Journal Article · Mon Apr 23 00:00:00 EDT 2018 · Acta Materialia

DOI:https://doi.org/10.1016/j.actamat.2018.04.048· OSTI ID:1440458

Qin, Wenjing ^[1];

^[1]; Doerner, Russell P. ^[2]; Wei, Guo ^[1]; Lv, Yawei ^[1]; Chang, Sheng ^[1]; Tang, Ming ^[3];

^[4]; Jiang, Changzhong ^[1];

^[3]

Wuhan Univ. (China). School of Physics and Technology. Center for Ion Beam Application. Center for Electron Microscopy
Univ. of California, San Diego, CA (United States). Center for Energy Research
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Hunan Univ., Changsha (China). Dept. of Applied Physics. School of Physics and Electronics

Developing high performance plasma facing materials (PFMs) is one of the greatest challenges for fusion reactors, because PFMs face unprecedented harsh environments including high flux plasma exposure, fast neutron irradiation and large transmutation gas. Tungsten (W) is considered as one of the most promising PFMs. Rapid accumulation of helium (He) atoms in such environments can lead to the He bubbles nucleation and even the formation of nano- to micro-scale “fuzz” on W surface, which greatly degrade the properties of W itself. The possible ejection of large W particulates into the core plasma can cause plasma instabilities. In this paper, we present a new strategy to address the root causes of bubble nucleation and “fuzz” formation by concurrently releasing He outside of W matrix through the nano-engineered channel structure (nanochannels). Comparing to ordinary bulk W, nanochannel W films with high surface-to-volume ratios are found to not only delay the growth of He bubbles, but also suppress the formation of “fuzz” (less than a half of the “fuzz” thickness formation in bulk W). Finally, molecular dynamic (MD) simulation results elucidate that low vacancy formation energy and high He binding energy in the nanochannel surface effectively help He release and affect He clusters distribution in W during He ion irradiation.

View Accepted Manuscript (DOE)

View Accepted Manuscript (Publisher)

Cite

Export

Save

Research Organization:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE; LANL Laboratory Directed Research and Development (LDRD) Program; National Natural Science Foundation of China (NSFC); Fundamental Research Funds for the Central Universities (China); Natural Science Foundation of Hubei Province (China); Univ. of California (United States)

Grant/Contract Number:: AC52-06NA25396; 11522543; 11475129; 51771073; 51571153; 2042017kf0194; 2016CFA080; 12-LR-237801; LDRD-20160567ER

OSTI ID:: 1440458

Alternate ID(s):: OSTI ID: 1548427

Report Number(s):: LA-UR-18-24035

Journal Information:: Acta Materialia, Vol. 153; ISSN 1359-6454

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

Citation Metrics:

Cited by: 48 works

Citation information provided by
Web of Science

References (40)

Materials research for fusion Knaster, J.; Moeslang, A.; Muroga, T. Nature Physics, Vol. 12, Issue 5 https://doi.org/10.1038/nphys3735	journal	May 2016
Material testing facilities and programs for plasma-facing component testing Linsmeier, Ch.; Unterberg, B.; Coenen, J. W. Nuclear Fusion, Vol. 57, Issue 9 https://doi.org/10.1088/1741-4326/aa4feb	journal	June 2017
Magnetic-confinement fusion Ongena, J.; Koch, R.; Wolf, R. Nature Physics, Vol. 12, Issue 5 https://doi.org/10.1038/nphys3745	journal	May 2016
Secondary electron emission from plasma-generated nanostructured tungsten fuzz Patino, M.; Raitses, Y.; Wirz, R. Applied Physics Letters, Vol. 109, Issue 20 https://doi.org/10.1063/1.4967830	journal	November 2016
Baseline high heat flux and plasma facing materials for fusion Ueda, Y.; Schmid, K.; Balden, M. Nuclear Fusion, Vol. 57, Issue 9 https://doi.org/10.1088/1741-4326/aa6b60	journal	June 2017
Period-thickness dependent responses of Cu/W multilayered nanofilms to ions irradiation under different ion energies Dong, Lan; Zhang, Hongxiu; Amekura, Hiroshi Journal of Nuclear Materials, Vol. 497 https://doi.org/10.1016/j.jnucmat.2017.07.064	journal	December 2017
Enhanced radiation tolerance of YSZ/Al2O3 multilayered nanofilms with pre-existing nanovoids Wang, Hui; Ren, Feng; Tang, Jun Acta Materialia, Vol. 144 https://doi.org/10.1016/j.actamat.2017.11.018	journal	February 2018
Deuterium retention in self-damaged tungsten Tyburska, B.; Alimov, V. Kh.; Ogorodnikova, O. V. Journal of Nuclear Materials, Vol. 395, Issue 1-3 https://doi.org/10.1016/j.jnucmat.2009.10.046	journal	December 2009
SRIM – The stopping and range of ions in matter (2010) Ziegler, James F.; Ziegler, M. D.; Biersack, J. P. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 268, Issue 11-12 https://doi.org/10.1016/j.nimb.2010.02.091	journal	June 2010
The influence of radiation damage on the plasma-induced deuterium retention in self-implanted tungsten Ogorodnikova, O. V.; Tyburska, B.; Alimov, V. Kh. Journal of Nuclear Materials, Vol. 415, Issue 1 https://doi.org/10.1016/j.jnucmat.2010.12.012	journal	August 2011
Formation process of tungsten nanostructure by the exposure to helium plasma under fusion relevant plasma conditions Kajita, Shin; Sakaguchi, Wataru; Ohno, Noriyasu Nuclear Fusion, Vol. 49, Issue 9 https://doi.org/10.1088/0029-5515/49/9/095005	journal	August 2009
Formation of helium induced nanostructure ‘fuzz’ on various tungsten grades Baldwin, M. J.; Doerner, R. P. Journal of Nuclear Materials, Vol. 404, Issue 3 https://doi.org/10.1016/j.jnucmat.2010.06.034	journal	September 2010
Sputtering properties of tungsten ‘fuzzy’ surfaces Nishijima, D.; Baldwin, M. J.; Doerner, R. P. Journal of Nuclear Materials, Vol. 415, Issue 1 https://doi.org/10.1016/j.jnucmat.2010.12.017	journal	August 2011
Fast Parallel Algorithms for Short-Range Molecular Dynamics Plimpton, Steve Journal of Computational Physics, Vol. 117, Issue 1 https://doi.org/10.1006/jcph.1995.1039	journal	March 1995
Interatomic potentials for simulation of He bubble formation in W Juslin, N.; Wirth, B. D. Journal of Nuclear Materials, Vol. 432, Issue 1-3 https://doi.org/10.1016/j.jnucmat.2012.07.023	journal	January 2013
Alpha- vs. beta-W nanocrystalline thin films: A comprehensive study of sputter parameters and resulting materials' properties Vüllers, F. T. N.; Spolenak, R. Thin Solid Films, Vol. 577 https://doi.org/10.1016/j.tsf.2015.01.030	journal	February 2015
The mechanism of texture formation during film growth: The roles of preferential sputtering and shadowing Ying, Feng; Smith, Richard W.; Srolovitz, David J. Applied Physics Letters, Vol. 69, Issue 20 https://doi.org/10.1063/1.116821	journal	November 1996
Migration of helium-pair in metals Cao, J. L.; Geng, W. T. Journal of Nuclear Materials, Vol. 478 https://doi.org/10.1016/j.jnucmat.2016.05.030	journal	September 2016
In situ TEM observation of helium bubble evolution in V/Ag multilayer during annealing Zhang, Hongxiu; Ren, Feng; Wang, Yongqiang Journal of Nuclear Materials, Vol. 467 https://doi.org/10.1016/j.jnucmat.2015.10.017	journal	December 2015
Self-organization of helium precipitates into elongated channels within metal nanolayers Chen, Di; Li, Nan; Yuryev, Dina Science Advances, Vol. 3, Issue 11 https://doi.org/10.1126/sciadv.aao2710	journal	November 2017
Magnetron sputter deposition of A-15 and bcc crystal structure tungsten thin films O’Keefe, M. J.; Grant, J. T.; Solomon, J. S. Journal of Electronic Materials, Vol. 24, Issue 8 https://doi.org/10.1007/BF02652968	journal	August 1995
Tungsten ‘fuzz’ growth re-examined: the dependence on ion fluence in non-erosive and erosive helium plasma Petty, T. J.; Baldwin, M. J.; Hasan, M. I. Nuclear Fusion, Vol. 55, Issue 9 https://doi.org/10.1088/0029-5515/55/9/093033	journal	August 2015
Nanostructure growth by helium plasma irradiation to tungsten in sputtering regime Noiri, Y.; Kajita, S.; Ohno, N. Journal of Nuclear Materials, Vol. 463 https://doi.org/10.1016/j.jnucmat.2015.01.036	journal	August 2015
Helium induced nanoscopic morphology on tungsten under fusion relevant plasma conditions Baldwin, M. J.; Doerner, R. P. Nuclear Fusion, Vol. 48, Issue 3 https://doi.org/10.1088/0029-5515/48/3/035001	journal	January 2008
Tungsten surface evolution by helium bubble nucleation, growth and rupture Sefta, Faiza; Hammond, Karl D.; Juslin, Niklas Nuclear Fusion, Vol. 53, Issue 7 https://doi.org/10.1088/0029-5515/53/7/073015	journal	June 2013
Molecular dynamics and Monte Carlo hybrid simulation for fuzzy tungsten nanostructure formation Ito, A. M.; Takayama, A.; Oda, Y. Nuclear Fusion, Vol. 55, Issue 7 https://doi.org/10.1088/0029-5515/55/7/073013	journal	June 2015
Quantitatively measuring the influence of helium in plasma-exposed tungsten Doerner, R. P.; Baldwin, M. J.; Simmonds, M. Nuclear Materials and Energy, Vol. 12 https://doi.org/10.1016/j.nme.2016.09.002	journal	August 2017
Experimental mechanistic investigation of the nanostructuring of tungsten with low energy helium plasmas Fiflis, P.; Connolly, N.; Ruzic, D. N. Journal of Nuclear Materials, Vol. 482 https://doi.org/10.1016/j.jnucmat.2016.10.015	journal	December 2016
First-principles study of vacancy, interstitial, noble gas atom interstitial and vacancy clusters in bcc-W Huang, Gui-Yang; Juslin, Niklas; Wirth, Brian D. Computational Materials Science, Vol. 123 https://doi.org/10.1016/j.commatsci.2016.06.022	journal	October 2016
Trapping of helium atom by vacancy in tungsten: a density functional theory study Zhang, Ningning; Zhang, Yujuan; Yang, Yu The European Physical Journal B, Vol. 90, Issue 5 https://doi.org/10.1140/epjb/e2017-80056-1	journal	May 2017
Depth dependence of vacancy formation energy at (100), (110), and (111) Al surfaces: A first-principles study Gupta, S. S.; van Huis, M. A.; Dijkstra, M. Physical Review B, Vol. 93, Issue 8 https://doi.org/10.1103/PhysRevB.93.085432	journal	February 2016
High hydrogen retention in the sub-surfaces of tungsten plasma facing materials: A theoretical insight Sun, Lu; Jin, Shuo; Lu, Guang-Hong Scripta Materialia, Vol. 122 https://doi.org/10.1016/j.scriptamat.2016.05.007	journal	September 2016
Trapping of He clusters by inert-gas impurities in tungsten: First-principles predictions and experimental validation Nguyen-Manh, Duc; Dudarev, S. L. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 352 https://doi.org/10.1016/j.nimb.2014.11.097	journal	June 2015
First-principles investigation of helium dissolution and clustering at a tungsten (1 1 0) surface Wang, Jinlong; Zhang, Ying; Zhou, Hong-Bo Journal of Nuclear Materials, Vol. 461 https://doi.org/10.1016/j.jnucmat.2015.03.026	journal	June 2015
Modeling and simulation of helium behavior in tungsten: A first-principles investigation Zhou, Hong-Bo; Li, Yu-Hao; Lu, Guang-Hong Computational Materials Science, Vol. 112 https://doi.org/10.1016/j.commatsci.2015.09.019	journal	February 2016
First-principles investigation of the orientation influenced He dissolution and diffusion behaviors on W surfaces Pan, G. Y.; Li, Y. G.; Zhang, Y. S. RSC Advances, Vol. 7, Issue 41 https://doi.org/10.1039/C7RA03281A	journal	January 2017
Helium nanobubble release from Pd surface: An atomic simulation Wang, Liang; Hu, Wangyu; Deng, Huiqiu Journal of Materials Research, Vol. 26, Issue 3 https://doi.org/10.1557/jmr.2010.49	journal	January 2011
A molecular dynamics simulation study of temperature and depth effect on helium bubble releasing from Ti surface Liang, Li; Ma, Mingwang; Xiang, Wei Journal of Alloys and Compounds, Vol. 645 https://doi.org/10.1016/j.jallcom.2015.01.084	journal	October 2015
A molecular dynamics study of helium bubble formation and gas release near titanium surfaces Zhang, B. L.; Wang, J.; Li, M. Journal of Nuclear Materials, Vol. 438, Issue 1-3 https://doi.org/10.1016/j.jnucmat.2013.03.033	journal	July 2013
Are Nanoporous Materials Radiation Resistant? Bringa, E. M.; Monk, J. D.; Caro, A. Nano Letters, Vol. 12, Issue 7 https://doi.org/10.1021/nl201383u	journal	June 2011

Cited By (4)

Helium flux effects on bubble growth and surface morphology in plasma-facing tungsten from large-scale molecular dynamics simulations Hammond, Karl D.; Naeger, Ian V.; Widanagamaachchi, Wathsala Nuclear Fusion, Vol. 59, Issue 6 https://doi.org/10.1088/1741-4326/ab12f6	journal	May 2019
Understanding the release of helium atoms from nanochannel tungsten: a molecular dynamics simulation Wei, Guo; Ren, Feng; Fang, Jingzhong Nuclear Fusion, Vol. 59, Issue 7 https://doi.org/10.1088/1741-4326/ab14c7	journal	June 2019
Ion beam analysis of fusion plasma-facing materials and components: facilities and research challenges Mayer, M.; Möller, S.; Rubel, M. Nuclear Fusion, Vol. 60, Issue 2 https://doi.org/10.1088/1741-4326/ab5817	journal	December 2019
Irradiation-Dependent Helium Gas Bubble Superlattice in Tungsten Sprouster, D. J.; Sun, C.; Zhang, Y. Scientific Reports, Vol. 9, Issue 1 https://doi.org/10.1038/s41598-019-39053-0	journal	February 2019

Similar Records

Influence of nanochannel structure on helium-vacancy cluster evolution and helium retention

Journal Article · Sun Sep 29 00:00:00 EDT 2019 · Journal of Nuclear Materials · OSTI ID:1440458

Qin, Wenjing; Jin, Shuoxue; Cao, Xingzhong; +5 more

Understanding the release of helium atoms from nanochannel tungsten: a molecular dynamics simulation

Journal Article · Wed Jun 05 00:00:00 EDT 2019 · Nuclear Fusion · OSTI ID:1440458

Wei, Guo; Ren, Feng; Fang, Jingzhong; +7 more

High Flux Helium Irradiation of Dispersion-Strengthened Tungsten Alloys and Effects of Heavy Metal Impurity Layer Deposition

Journal Article · Fri Nov 13 00:00:00 EST 2020 · Journal of Nuclear Materials · OSTI ID:1440458

Lang, E.; Kapat, A.; Morgan, T. W.; +1 more

Related Subjects

36 MATERIALS SCIENCE
tungsten
nanochannel formation
bubble
"fuzz"
simulation

Title: Nanochannel structures in W enhance radiation tolerance

Citation Formats

References (40)

Cited By (4)

Similar Records

Related Subjects